Nature Energy, volume 1, issue 4, publication number 16030
High-power all-solid-state batteries using sulfide superionic conductors
Yuki Kato
1, 2, 3
,
Satoshi Hori
2
,
Toshiya Saito
1
,
Kota Suzuki
2
,
Masaaki Hirayama
2
,
Akio Mitsui
4
,
Masao Yonemura
5
,
Hideki Iba
1
,
Ryoji Kanno
2
1
Battery Research Division, Higashifuji Technical Center, Toyota Motor Corporation, 1200 Mishuku, Susono, Shizuoka 410-1193, Japan
|
3
Battery AT, Advanced Technology 1, Toyota Motor Europe NV/SA, Hoge Wei 33A B-1930, Zaventem, Belgium
|
4
Material analysis Department, Material Engineering Division, Toyota Motor Corporation, 1 Toyota-cho, Toyota, Aichi 471-8572, Japan
|
Publication type: Journal Article
Publication date: 2016-03-21
Electronic, Optical and Magnetic Materials
Energy Engineering and Power Technology
Fuel Technology
Renewable Energy, Sustainability and the Environment
Abstract
Compared with lithium-ion batteries with liquid electrolytes, all-solid-state batteries offer an attractive option owing to their potential in improving the safety and achieving both high power and high energy densities. Despite extensive research efforts, the development of all-solid-state batteries still falls short of expectation largely because of the lack of suitable candidate materials for the electrolyte required for practical applications. Here we report lithium superionic conductors with an exceptionally high conductivity (25 mS cm−1 for Li9.54Si1.74P1.44S11.7Cl0.3), as well as high stability ( ∼0 V versus Li metal for Li9.6P3S12). A fabricated all-solid-state cell based on this lithium conductor is found to have very small internal resistance, especially at 100 ∘C. The cell possesses high specific power that is superior to that of conventional cells with liquid electrolytes. Stable cycling with a high current density of 18 C (charging/discharging in just three minutes; where C is the C-rate) is also demonstrated. The development of all-solid-state batteries requires fast lithium conductors. Here, the authors report a lithium compound, Li9.54Si1.74P1.44S11.7Cl0.3, with an exceptionally high conductivity and demonstrate that all-solid-state batteries based on the compound have high power densities.
Top-30
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Citations by publishers
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Elsevier
660 publications, 25.89%
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American Chemical Society (ACS)
532 publications, 20.87%
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American Physical Society (APS)
11 publications, 0.43%
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11 publications, 0.43%
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The Chemical Society of Japan
9 publications, 0.35%
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Japan Society of Applied Physics
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Chinese Physical Society
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Oxford University Press
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5 publications, 0.2%
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Taylor & Francis
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IEEE
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3 publications, 0.12%
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3 publications, 0.12%
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- We do not take into account publications without a DOI.
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- Statistics recalculated weekly.
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Kato Y. et al. High-power all-solid-state batteries using sulfide superionic conductors // Nature Energy. 2016. Vol. 1. No. 4. 16030
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Kato Y., Hori S., Saito T., Suzuki K., Hirayama M., Mitsui A., Yonemura M., Iba H., Kanno R. High-power all-solid-state batteries using sulfide superionic conductors // Nature Energy. 2016. Vol. 1. No. 4. 16030
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TY - JOUR
DO - 10.1038/nenergy.2016.30
UR - https://doi.org/10.1038/nenergy.2016.30
TI - High-power all-solid-state batteries using sulfide superionic conductors
T2 - Nature Energy
AU - Kato, Yuki
AU - Hori, Satoshi
AU - Saito, Toshiya
AU - Suzuki, Kota
AU - Hirayama, Masaaki
AU - Mitsui, Akio
AU - Yonemura, Masao
AU - Iba, Hideki
AU - Kanno, Ryoji
PY - 2016
DA - 2016/03/21 00:00:00
PB - Springer Nature
IS - 4
VL - 1
SN - 2058-7546
ER -
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@article{2016_Kato,
author = {Yuki Kato and Satoshi Hori and Toshiya Saito and Kota Suzuki and Masaaki Hirayama and Akio Mitsui and Masao Yonemura and Hideki Iba and Ryoji Kanno},
title = {High-power all-solid-state batteries using sulfide superionic conductors},
journal = {Nature Energy},
year = {2016},
volume = {1},
publisher = {Springer Nature},
month = {mar},
url = {https://doi.org/10.1038/nenergy.2016.30},
number = {4},
doi = {10.1038/nenergy.2016.30}
}