Nature Energy, volume 2, issue 5, publication number 17035

Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires

Wei Liu ¹

Seok-Woo Lee ²

Dingchang Lin ¹

Feifei Shi ¹

Shuang Wang ³

Austin D Sendek ⁴

Yi Cui ^{1, 5}

Hide authors affiliations Show authors affiliations: 5 affiliations

Department of Materials Science and Engineering, Stanford University, Stanford, California 94305, USA |

Geballe Laboratory for Advanced Materials, Stanford University, Stanford, California 94305, USA |

Department of Electrical Engineering, Stanford University, Stanford, California 94305, USA |

⁴

Department of Applied Physics, Stanford University, Stanford, California 94305, USA |

⁵

Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA |

Publication type: Journal Article

Publication date: 2017-04-03

Springer Nature

Journal: Nature Energy

Quartile SCImago

Quartile WOS

Impact factor: 56.7

ISSN: 20587546

DOI: 10.1038/nenergy.2017.35

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Electronic, Optical and Magnetic Materials

Energy Engineering and Power Technology

Fuel Technology

Renewable Energy, Sustainability and the Environment

Abstract

In contrast to conventional organic liquid electrolytes that have leakage, flammability and chemical stability issues, solid electrolytes are widely considered as a promising candidate for the development of next-generation safe lithium-ion batteries. In solid polymer electrolytes that contain polymers and lithium salts, inorganic nanoparticles are often used as fillers to improve electrochemical performance, structure stability, and mechanical strength. However, such composite polymer electrolytes generally have low ionic conductivity. Here we report that a composite polymer electrolyte with well-aligned inorganic Li+-conductive nanowires exhibits an ionic conductivity of 6.05 × 10−5 S cm-1 at 30 ∘C, which is one order of magnitude higher than previous polymer electrolytes with randomly aligned nanowires. The large conductivity enhancement is ascribed to a fast ion-conducting pathway without crossing junctions on the surfaces of the aligned nanowires. Moreover, the long-term structural stability of the polymer electrolyte is also improved by the use of nanowires. Fast ionic conductivity of solid electrolytes is a must in the development of next-generation solid-electrolyte-based lithium-ion batteries. Here the authors report that composite polymer electrolytes with well-aligned inorganic nanowires can achieve much larger conductivities than those without.

By date By citations

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Citations by journals

	5 10 15 20 25 30 35 40 45
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 43, 5.25% Journal of Materials Chemistry A 43 publications, 5.25%
Energy Storage Materials	Energy Storage Materials, 42, 5.13% Energy Storage Materials 42 publications, 5.13%
Advanced Functional Materials	Advanced Functional Materials, 35, 4.27% Advanced Functional Materials 35 publications, 4.27%
ACS applied materials & interfaces	ACS applied materials & interfaces, 34, 4.15% ACS applied materials & interfaces 34 publications, 4.15%
Advanced Materials	Advanced Materials, 26, 3.17% Advanced Materials 26 publications, 3.17%
Advanced Energy Materials	Advanced Energy Materials, 25, 3.05% Advanced Energy Materials 25 publications, 3.05%
Chemical Engineering Journal	Chemical Engineering Journal, 22, 2.69% Chemical Engineering Journal 22 publications, 2.69%
Small	Small, 18, 2.2% Small 18 publications, 2.2%
Journal of Power Sources	Journal of Power Sources, 18, 2.2% Journal of Power Sources 18 publications, 2.2%
Advanced Science	Advanced Science, 15, 1.83% Advanced Science 15 publications, 1.83%
ACS Applied Energy Materials	ACS Applied Energy Materials, 15, 1.83% ACS Applied Energy Materials 15 publications, 1.83%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 14, 1.71% Journal of the Electrochemical Society 14 publications, 1.71%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 14, 1.71% Journal of Colloid and Interface Science 14 publications, 1.71%
Journal of Energy Chemistry	Journal of Energy Chemistry, 12, 1.47% Journal of Energy Chemistry 12 publications, 1.47%
Electrochimica Acta	Electrochimica Acta, 11, 1.34% Electrochimica Acta 11 publications, 1.34%
ACS Nano	ACS Nano, 10, 1.22% ACS Nano 10 publications, 1.22%
Ionics	Ionics, 10, 1.22% Ionics 10 publications, 1.22%
Nano Energy	Nano Energy, 10, 1.22% Nano Energy 10 publications, 1.22%
Energy and Environmental Science	Energy and Environmental Science, 10, 1.22% Energy and Environmental Science 10 publications, 1.22%
Journal of Membrane Science	Journal of Membrane Science, 9, 1.1% Journal of Membrane Science 9 publications, 1.1%
ACS Energy Letters	ACS Energy Letters, 9, 1.1% ACS Energy Letters 9 publications, 1.1%
Nature Communications	Nature Communications, 8, 0.98% Nature Communications 8 publications, 0.98%
Electrochemical Energy Reviews	Electrochemical Energy Reviews, 7, 0.85% Electrochemical Energy Reviews 7 publications, 0.85%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 7, 0.85% Journal of Alloys and Compounds 7 publications, 0.85%
Angewandte Chemie	Angewandte Chemie, 7, 0.85% Angewandte Chemie 7 publications, 0.85%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 7, 0.85% Angewandte Chemie - International Edition 7 publications, 0.85%
Nano Letters	Nano Letters, 7, 0.85% Nano Letters 7 publications, 0.85%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 7, 0.85% Journal of Physical Chemistry C 7 publications, 0.85%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 7, 0.85% Materials Chemistry Frontiers 7 publications, 0.85%
	5 10 15 20 25 30 35 40 45

Citations by publishers

	50 100 150 200 250 300
Elsevier	Elsevier, 273, 33.33% Elsevier 273 publications, 33.33%
Wiley	Wiley, 191, 23.32% Wiley 191 publications, 23.32%
American Chemical Society (ACS)	American Chemical Society (ACS), 130, 15.87% American Chemical Society (ACS) 130 publications, 15.87%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 87, 10.62% Royal Society of Chemistry (RSC) 87 publications, 10.62%
Springer Nature	Springer Nature, 57, 6.96% Springer Nature 57 publications, 6.96%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 21, 2.56% Multidisciplinary Digital Publishing Institute (MDPI) 21 publications, 2.56%
The Electrochemical Society	The Electrochemical Society, 14, 1.71% The Electrochemical Society 14 publications, 1.71%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 5, 0.61% American Institute of Physics (AIP) 5 publications, 0.61%
Frontiers Media S.A.	Frontiers Media S.A., 5, 0.61% Frontiers Media S.A. 5 publications, 0.61%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 4, 0.49% American Association for the Advancement of Science (AAAS) 4 publications, 0.49%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 3, 0.37% Nonferrous Metals Society of China 3 publications, 0.37%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 3, 0.37% Proceedings of the National Academy of Sciences (PNAS) 3 publications, 0.37%
Tsinghua University Press	Tsinghua University Press, 2, 0.24% Tsinghua University Press 2 publications, 0.24%
IOP Publishing	IOP Publishing, 2, 0.24% IOP Publishing 2 publications, 0.24%
Trans Tech Publications	Trans Tech Publications, 2, 0.24% Trans Tech Publications 2 publications, 0.24%
OAE Publishing Inc.	OAE Publishing Inc., 2, 0.24% OAE Publishing Inc. 2 publications, 0.24%
Bentham Science	Bentham Science, 1, 0.12% Bentham Science 1 publication, 0.12%
Tech Science Press	Tech Science Press, 1, 0.12% Tech Science Press 1 publication, 0.12%
Chemical Industry Press	Chemical Industry Press, 1, 0.12% Chemical Industry Press 1 publication, 0.12%
KeAi Communications Co.	KeAi Communications Co., 1, 0.12% KeAi Communications Co. 1 publication, 0.12%
Taylor & Francis	Taylor & Francis, 1, 0.12% Taylor & Francis 1 publication, 0.12%
Chinese Physical Society	Chinese Physical Society, 1, 0.12% Chinese Physical Society 1 publication, 0.12%
Oxford University Press	Oxford University Press, 1, 0.12% Oxford University Press 1 publication, 0.12%
Research Square Platform LLC	Research Square Platform LLC, 1, 0.12% Research Square Platform LLC 1 publication, 0.12%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.12% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.12%
	50 100 150 200 250 300

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Liu W. et al. Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires // Nature Energy. 2017. Vol. 2. No. 5. 17035

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Liu W., Lee S., Lin D., Shi F., Wang S., Sendek A. D., Cui Y. Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires // Nature Energy. 2017. Vol. 2. No. 5. 17035

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TY - JOUR

DO - 10.1038/nenergy.2017.35

UR - https://doi.org/10.1038/nenergy.2017.35

TI - Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires

T2 - Nature Energy

AU - Liu, Wei

AU - Lee, Seok-Woo

AU - Lin, Dingchang

AU - Shi, Feifei

AU - Wang, Shuang

AU - Sendek, Austin D

AU - Cui, Yi

PY - 2017

DA - 2017/04/03 00:00:00

PB - Springer Nature

IS - 5

VL - 2

SN - 2058-7546

ER -

BibTex

Cite this

BibTex Copy

@article{2017_Liu,

author = {Wei Liu and Seok-Woo Lee and Dingchang Lin and Feifei Shi and Shuang Wang and Austin D Sendek and Yi Cui},

title = {Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires},

journal = {Nature Energy},

year = {2017},

volume = {2},

publisher = {Springer Nature},

month = {apr},

url = {https://doi.org/10.1038/nenergy.2017.35},

number = {5},

doi = {10.1038/nenergy.2017.35}

}

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Publisher

Springer Nature

Journal

Nature Energy

Quartile SCImago

Quartile WOS

Impact factor

56.7

ISSN

20587546 (Electronic)