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Light: Science and Applications, volume 12, issue 1, publication number 2

High-operating-temperature mid-infrared photodetectors via quantum dot gradient homojunction

Xiaomeng Xue 1
Meng-Lu Chen 1, 2, 3
Yuning Luo 1
Tianling Qin 1
Xin Tang 1, 2, 3
Qun Hao 1, 2, 3
Publication typeJournal Article
Publication date2023-01-01
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor19.4
ISSN20477538
Electronic, Optical and Magnetic Materials
Atomic and Molecular Physics, and Optics
Abstract

Due to thermal carriers generated by a narrow mid-infrared energy gap, cooling is always necessary to achieve ideal photodetection. In quantum dot (QD), the electron thermal generation should be reduced with quantum confinement in all three dimensions. As a result, there would be a great potential to realize high-operating-temperature (HOT) QD mid-IR photodetectors, though not yet achieved. Taking the advantages of colloidal nanocrystals’ solution processability and precise doping control by surface dipoles, this work demonstrates a HOT mid-infrared photodetector with a QD gradient homojunction. The detector achieves background-limited performance with D* = 2.7 × 1011 Jones on 4.2 μm at 80 K, above 1011 Jones until 200 K, above 1010 Jones until 280 K, and 7.6 × 109 Jones on 3.5 μm at 300 K. The external quantum efficiency also achieves more than 77% with responsivity 2.7 A/W at zero bias. The applications such as spectrometers, chemical sensors, and thermal cameras, are also approved, which motivate interest in low-cost, solution-processed and high-performance mid-infrared photodetection beyond epitaxial growth bulk photodetectors.

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GOST Copy
Xue X. et al. High-operating-temperature mid-infrared photodetectors via quantum dot gradient homojunction // Light: Science and Applications. 2023. Vol. 12. No. 1. 2
GOST all authors (up to 50) Copy
Xue X., Chen M., Luo Y., Qin T., Tang X., Hao Q. High-operating-temperature mid-infrared photodetectors via quantum dot gradient homojunction // Light: Science and Applications. 2023. Vol. 12. No. 1. 2
RIS |
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RIS Copy
TY - JOUR
DO - 10.1038/s41377-022-01014-0
UR - https://doi.org/10.1038/s41377-022-01014-0
TI - High-operating-temperature mid-infrared photodetectors via quantum dot gradient homojunction
T2 - Light: Science and Applications
AU - Xue, Xiaomeng
AU - Chen, Meng-Lu
AU - Luo, Yuning
AU - Qin, Tianling
AU - Tang, Xin
AU - Hao, Qun
PY - 2023
DA - 2023/01/01 00:00:00
PB - Springer Nature
IS - 1
VL - 12
SN - 2047-7538
ER -
BibTex
Cite this
BibTex Copy
@article{2023_Xue,
author = {Xiaomeng Xue and Meng-Lu Chen and Yuning Luo and Tianling Qin and Xin Tang and Qun Hao},
title = {High-operating-temperature mid-infrared photodetectors via quantum dot gradient homojunction},
journal = {Light: Science and Applications},
year = {2023},
volume = {12},
publisher = {Springer Nature},
month = {jan},
url = {https://doi.org/10.1038/s41377-022-01014-0},
number = {1},
doi = {10.1038/s41377-022-01014-0}
}
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