Open Access
Nature Communications, volume 12, issue 1, publication number 5075
Superconductivity up to 243 K in the yttrium-hydrogen system under high pressure
Kong Panpan
1
,
Minkov Vasily S.
1
,
Kuzovnikov Mikhail A
2
,
Drozdov Alexander P
1
,
Besedin Stanislav P.
1
,
Mozaffari Shirin
3
,
Balicas Luis
3
,
Balakirev F.
4
,
Prakapenka V.
5
,
Chariton Stella
5
,
Knyazev Dmitry A
6
,
Greenberg E.
5
,
1
Max-Planck-Institut für Chemie, Mainz, Germany
|
4
NHMFL, Los Alamos National Laboratory, MS E536, Los Alamos, USA
|
5
Center for Advanced Radiation Sources, University of Chicago, Chicago, USA
|
6
Max-Planck-Institut für Mikrostrukturphysik, Halle (Saale), Germany
|
Publication type: Journal Article
Publication date: 2021-08-20
Journal:
Nature Communications
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 16.6
ISSN: 20411723
PubMed ID:
34417471
General Chemistry
General Biochemistry, Genetics and Molecular Biology
General Physics and Astronomy
Abstract
The discovery of superconducting H3S with a critical temperature Tc∼200 K opened a door to room temperature superconductivity and stimulated further extensive studies of hydrogen-rich compounds stabilized by high pressure. Here, we report a comprehensive study of the yttrium-hydrogen system with the highest predicted Tcs among binary compounds and discuss the contradictions between different theoretical calculations and experimental data. We synthesized yttrium hydrides with the compositions of YH3, YH4, YH6 and YH9 in a diamond anvil cell and studied their crystal structures, electrical and magnetic transport properties, and isotopic effects. We found superconductivity in the Im-3m YH6 and P63/mmc YH9 phases with maximal Tcs of ∼220 K at 183 GPa and ∼243 K at 201 GPa, respectively. Fm-3m YH10 with the highest predicted Tc > 300 K was not observed in our experiments, and instead, YH9 was found to be the hydrogen-richest yttrium hydride in the studied pressure and temperature range up to record 410 GPa and 2250 K. The discovery of high temperature superconductivity in hydrogen-rich compounds stimulates further extensive studies. Here, the authors report superconductivity in pressurized yttrium-hydrogen system with highest predicted Tc among binary compounds.
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Kong P. et al. Superconductivity up to 243 K in the yttrium-hydrogen system under high pressure // Nature Communications. 2021. Vol. 12. No. 1. 5075
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Kong P., Minkov V. S., Kuzovnikov M. A., Drozdov A. P., Besedin S. P., Mozaffari S., Balicas L., Balakirev F., Prakapenka V., Chariton S., Knyazev D. A., Greenberg E., Eremets M. Superconductivity up to 243 K in the yttrium-hydrogen system under high pressure // Nature Communications. 2021. Vol. 12. No. 1. 5075
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TY - JOUR
DO - 10.1038/s41467-021-25372-2
UR - https://doi.org/10.1038%2Fs41467-021-25372-2
TI - Superconductivity up to 243 K in the yttrium-hydrogen system under high pressure
T2 - Nature Communications
AU - Kong, Panpan
AU - Minkov, Vasily S.
AU - Kuzovnikov, Mikhail A
AU - Drozdov, Alexander P
AU - Besedin, Stanislav P.
AU - Mozaffari, Shirin
AU - Balicas, Luis
AU - Balakirev, F.
AU - Prakapenka, V.
AU - Chariton, Stella
AU - Knyazev, Dmitry A
AU - Greenberg, E.
AU - Eremets, M.I.
PY - 2021
DA - 2021/08/20 00:00:00
PB - Springer Nature
IS - 1
VL - 12
PMID - 34417471
SN - 2041-1723
ER -
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@article{2021_Kong,
author = {Panpan Kong and Vasily S. Minkov and Mikhail A Kuzovnikov and Alexander P Drozdov and Stanislav P. Besedin and Shirin Mozaffari and Luis Balicas and F. Balakirev and V. Prakapenka and Stella Chariton and Dmitry A Knyazev and E. Greenberg and M.I. Eremets},
title = {Superconductivity up to 243 K in the yttrium-hydrogen system under high pressure},
journal = {Nature Communications},
year = {2021},
volume = {12},
publisher = {Springer Nature},
month = {aug},
url = {https://doi.org/10.1038%2Fs41467-021-25372-2},
number = {1},
doi = {10.1038/s41467-021-25372-2}
}