Nature Energy, volume 5, issue 4, pages 299-308
High-energy long-cycling all-solid-state lithium metal batteries enabled by silver–carbon composite anodes
Yong-Gun Lee
1
,
Satoshi Fujiki
2
,
Changhoon Jung
1
,
Naoki Suzuki
2
,
Nobuyoshi Yashiro
2
,
Ryo Omoda
2
,
Dong-su Ko
1
,
Tomoyuki Shiratsuchi
2
,
Toshinori Sugimoto
1
,
Saebom Ryu
1
,
Jun-Hwan Ku
1
,
Taku Watanabe
2
,
Youngsin Park
1
,
Yuichi Aihara
2
,
D. Im
1
,
In Taek Han
1
2
Samsung R&D Institute Japan, Osaka, Japan
|
Publication type: Journal Article
Publication date: 2020-03-09
Electronic, Optical and Magnetic Materials
Energy Engineering and Power Technology
Fuel Technology
Renewable Energy, Sustainability and the Environment
Abstract
An all-solid-state battery with a lithium metal anode is a strong candidate for surpassing conventional lithium-ion battery capabilities. However, undesirable Li dendrite growth and low Coulombic efficiency impede their practical application. Here we report that a high-performance all-solid-state lithium metal battery with a sulfide electrolyte is enabled by a Ag–C composite anode with no excess Li. We show that the thin Ag–C layer can effectively regulate Li deposition, which leads to a genuinely long electrochemical cyclability. In our full-cell demonstrations, we employed a high-Ni layered oxide cathode with a high specific capacity (>210 mAh g−1) and high areal capacity (>6.8 mAh cm−2) and an argyrodite-type sulfide electrolyte. A warm isostatic pressing technique was also introduced to improve the contact between the electrode and the electrolyte. A prototype pouch cell (0.6 Ah) thus prepared exhibited a high energy density (>900 Wh l−1), stable Coulombic efficiency over 99.8% and long cycle life (1,000 times). Solid-state Li metal batteries represent one of the most promising rechargeable battery technologies. Here the authors report an exceptional high-performance prototype solid-state pouch cell made of a sulfide electrolyte, a high-Ni layered oxide cathode and, in particular, a silver–carbon composite anode with no excess Li.
Top-30
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Wiley
299 publications, 28.53%
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Elsevier
291 publications, 27.77%
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4 publications, 0.38%
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Chinese Physical Society
3 publications, 0.29%
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OAE Publishing Inc.
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1 publication, 0.1%
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1 publication, 0.1%
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1 publication, 0.1%
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1 publication, 0.1%
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1 publication, 0.1%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Lee Y. et al. High-energy long-cycling all-solid-state lithium metal batteries enabled by silver–carbon composite anodes // Nature Energy. 2020. Vol. 5. No. 4. pp. 299-308.
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Lee Y., Fujiki S., Jung C., Suzuki N., Yashiro N., Omoda R., Ko D., Shiratsuchi T., Sugimoto T., Ryu S., Ku J., Watanabe T., Park Y., Aihara Y., Im D., Han I. T. High-energy long-cycling all-solid-state lithium metal batteries enabled by silver–carbon composite anodes // Nature Energy. 2020. Vol. 5. No. 4. pp. 299-308.
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TY - JOUR
DO - 10.1038/s41560-020-0575-z
UR - https://www.nature.com/articles/s41560-020-0575-z
TI - High-energy long-cycling all-solid-state lithium metal batteries enabled by silver–carbon composite anodes
T2 - Nature Energy
AU - Lee, Yong-Gun
AU - Fujiki, Satoshi
AU - Jung, Changhoon
AU - Suzuki, Naoki
AU - Yashiro, Nobuyoshi
AU - Omoda, Ryo
AU - Ko, Dong-su
AU - Shiratsuchi, Tomoyuki
AU - Sugimoto, Toshinori
AU - Ryu, Saebom
AU - Ku, Jun-Hwan
AU - Watanabe, Taku
AU - Park, Youngsin
AU - Aihara, Yuichi
AU - Im, D.
AU - Han, In Taek
PY - 2020
DA - 2020/03/09 00:00:00
PB - Springer Nature
SP - 299-308
IS - 4
VL - 5
SN - 2058-7546
ER -
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@article{2020_Lee,
author = {Yong-Gun Lee and Satoshi Fujiki and Changhoon Jung and Naoki Suzuki and Nobuyoshi Yashiro and Ryo Omoda and Dong-su Ko and Tomoyuki Shiratsuchi and Toshinori Sugimoto and Saebom Ryu and Jun-Hwan Ku and Taku Watanabe and Youngsin Park and Yuichi Aihara and D. Im and In Taek Han},
title = {High-energy long-cycling all-solid-state lithium metal batteries enabled by silver–carbon composite anodes},
journal = {Nature Energy},
year = {2020},
volume = {5},
publisher = {Springer Nature},
month = {mar},
url = {https://www.nature.com/articles/s41560-020-0575-z},
number = {4},
pages = {299--308},
doi = {10.1038/s41560-020-0575-z}
}
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Lee, Yong-Gun, et al. “High-energy long-cycling all-solid-state lithium metal batteries enabled by silver–carbon composite anodes.” Nature Energy, vol. 5, no. 4, Mar. 2020, pp. 299-308. https://www.nature.com/articles/s41560-020-0575-z.