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, том 4 , издание 1 , номер публикации 5086

Efficient Thermolysis Route to Monodisperse Cu2ZnSnS4 Nanocrystals with Controlled Shape and Structure

Тип публикации: Journal Article

Дата публикации: 2014-05-28

Springer Nature

Scientific Reports

SCImago Q1

WOS Q1

БС1

SJR: 0.893

CiteScore: 6.4

Impact factor: 4.9

ISSN: 20452322

DOI: 10.1038/srep05086

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PubMed ID: 24866987

Multidisciplinary

Краткое описание

Monodisperse Cu2ZnSnS4 (CZTS) nanocrystals with tunable shape, crystalline phase and composition are synthesized by efficient thermolysis of a single source precursor of mixed metal-oleate complexes in hot organic solvents with dissolved sulfur sources. Suitable tuning of the synthetic conditions and the Cu/(Zn + Sn) ratio of the precursor has enabled precise control of the crystalline phase in the form of kesterite, or a newly observed wurtzite structure. Nanocrystals with morphology in the form of spherical, rice-like, or rod-like shapes are obtained over a wide range of compositions (0.5 ≤ Cu/(Zn + Sn) ≤ 1.2). Both the final products and intermediates for each shape exhibit consistent composition and structure, indicating homogenous nucleation and growth of single-phase nanocrystals. Thin films prepared from colloidal nanocrystal suspensions display interesting shape-dependent photoresponse behavior under white light illumination from a solar simulator.

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Zhang X. et al. Efficient Thermolysis Route to Monodisperse Cu2ZnSnS4 Nanocrystals with Controlled Shape and Structure // Scientific Reports. 2014. Vol. 4. No. 1. 5086

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Zhang X., Guo G., Ji C., Huang K., Zha C., Wang Y., Shen L., Gupta A., Bao N. Efficient Thermolysis Route to Monodisperse Cu2ZnSnS4 Nanocrystals with Controlled Shape and Structure // Scientific Reports. 2014. Vol. 4. No. 1. 5086

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TY - JOUR

DO - 10.1038/srep05086

UR - https://doi.org/10.1038/srep05086

TI - Efficient Thermolysis Route to Monodisperse Cu2ZnSnS4 Nanocrystals with Controlled Shape and Structure

T2 - Scientific Reports

AU - Zhang, Xiaoyan

AU - Guo, Guobiao

AU - Ji, Cheng

AU - Huang, Kai

AU - Zha, Chenyang

AU - Wang, Yifeng

AU - Shen, Liming

AU - Gupta, Arunava

AU - Bao, Ningzhong

PY - 2014

DA - 2014/05/28

PB - Springer Nature

IS - 1

VL - 4

PMID - 24866987

SN - 2045-2322

ER -

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@article{2014_Zhang,

author = {Xiaoyan Zhang and Guobiao Guo and Cheng Ji and Kai Huang and Chenyang Zha and Yifeng Wang and Liming Shen and Arunava Gupta and Ningzhong Bao},

title = {Efficient Thermolysis Route to Monodisperse Cu2ZnSnS4 Nanocrystals with Controlled Shape and Structure},

journal = {Scientific Reports},

year = {2014},

volume = {4},

publisher = {Springer Nature},

month = {may},

url = {https://doi.org/10.1038/srep05086},

number = {1},

pages = {5086},

doi = {10.1038/srep05086}

}

Издатель

Springer Nature

Журнал

Scientific Reports

SCImago Q1

WOS Q1

БС1

SJR

0.893

CiteScore

6.4

Impact factor

4.9

ISSN

20452322 (Print, Electronic)

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