Copper-catalyzed C-alkylation of secondary alcohols and methyl ketones with alcohols employing the aerobic relay race methodology
Shiheng Liao
1
,
Kangkang Yu
1
,
Qiang Li
1
,
Haiwen Tian
1
,
Zhengping Zhang
1
,
Xiaochun Yu
1
,
Qing Xu
1
1
College of Chemistry and Materials Engineering, WenZhou University, Wenzhou, China
|
Тип публикации: Journal Article
Дата публикации: 2012-01-20
scimago Q2
wos Q2
БС1
SJR: 0.600
CiteScore: 5.2
Impact factor: 2.7
ISSN: 14770520, 14770539
PubMed ID:
22261789
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Краткое описание
By employing aerobic oxidation to aldehydes as a more effective alcohol activation strategy, ligand-free copper catalysts were found to be superior catalysts than other metals in aerobic dehydrative β-alkylation of secondary alcohols and α-alkylation of methyl ketones using alcohols as the green alkylating reagents. Based on our mechanistic studies and also supported by the literature, we deduce that the newly-proposed relay race process rather than the conventional borrowing hydrogen-type mechanisms should be the most possible and a more rational mechanism for the aerobic C-alkylation reactions.
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Всего цитирований:
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ГОСТ
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Liao S. et al. Copper-catalyzed C-alkylation of secondary alcohols and methyl ketones with alcohols employing the aerobic relay race methodology // Organic and Biomolecular Chemistry. 2012. Vol. 10. No. 15. p. 2973.
ГОСТ со всеми авторами (до 50)
Скопировать
Liao S., Yu K., Li Q., Tian H., Zhang Z., Yu X., Xu Q. Copper-catalyzed C-alkylation of secondary alcohols and methyl ketones with alcohols employing the aerobic relay race methodology // Organic and Biomolecular Chemistry. 2012. Vol. 10. No. 15. p. 2973.
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RIS
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TY - JOUR
DO - 10.1039/c1ob06739g
UR - https://doi.org/10.1039/c1ob06739g
TI - Copper-catalyzed C-alkylation of secondary alcohols and methyl ketones with alcohols employing the aerobic relay race methodology
T2 - Organic and Biomolecular Chemistry
AU - Liao, Shiheng
AU - Yu, Kangkang
AU - Li, Qiang
AU - Tian, Haiwen
AU - Zhang, Zhengping
AU - Yu, Xiaochun
AU - Xu, Qing
PY - 2012
DA - 2012/01/20
PB - Royal Society of Chemistry (RSC)
SP - 2973
IS - 15
VL - 10
PMID - 22261789
SN - 1477-0520
SN - 1477-0539
ER -
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BibTex (до 50 авторов)
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@article{2012_Liao,
author = {Shiheng Liao and Kangkang Yu and Qiang Li and Haiwen Tian and Zhengping Zhang and Xiaochun Yu and Qing Xu},
title = {Copper-catalyzed C-alkylation of secondary alcohols and methyl ketones with alcohols employing the aerobic relay race methodology},
journal = {Organic and Biomolecular Chemistry},
year = {2012},
volume = {10},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://doi.org/10.1039/c1ob06739g},
number = {15},
pages = {2973},
doi = {10.1039/c1ob06739g}
}
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MLA
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Liao, Shiheng, et al. “Copper-catalyzed C-alkylation of secondary alcohols and methyl ketones with alcohols employing the aerobic relay race methodology.” Organic and Biomolecular Chemistry, vol. 10, no. 15, Jan. 2012, p. 2973. https://doi.org/10.1039/c1ob06739g.