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Zwitterionic iodonium species afford halogen bond-based porous organic frameworks
Тип публикации: Journal Article
Дата публикации: 2022-04-12
scimago Q1
wos Q1
БС1
SJR: 2.138
CiteScore: 12.6
Impact factor: 7.4
ISSN: 20416520, 20416539
PubMed ID:
35694330
General Chemistry
Краткое описание
Porous architectures characterized by parallel channels arranged in honeycomb or rectangular patterns are identified in two polymorphic crystals of a zwitterionic 4-(aryliodonio)-benzenesulfonate. The channels are filled with disordered water molecules which can be reversibly removed on heating. Consistent with the remarkable strength and directionality of the halogen bonds (XBs) driving the crystal packing formation, the porous structure is stable and fully preserved on almost quantitative removal and readsorption of water. The porous systems described here are the first reported cases of one-component 3D organic frameworks whose assembly is driven by XB only (XOFs). These systems are a proof of concept for the ability of zwitterionic aryliodonium tectons in affording robust one-component 3D XOFs. The high directionality and strength of the XBs formed by these zwitterions and the geometrical constraints resulting from the tendency of their hypervalent iodine atoms to act as bidentate XB donors might be key factors in determining this ability.
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ГОСТ
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Soldatova N. et al. Zwitterionic iodonium species afford halogen bond-based porous organic frameworks // Chemical Science. 2022. Vol. 13. No. 19. pp. 5650-5658.
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Soldatova N., Postnikov P. S., Ivanov D. M., Semyonov O. V., Kukurina O. S., Guselnikova O., YAMAUCHI Y., Wirth T., Zhdankin V. V., Yusubov M. S., Gomila R. M., Frontera A., Resnati G., Kukushkin V. Y. Zwitterionic iodonium species afford halogen bond-based porous organic frameworks // Chemical Science. 2022. Vol. 13. No. 19. pp. 5650-5658.
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TY - JOUR
DO - 10.1039/d2sc00892k
UR - https://xlink.rsc.org/?DOI=D2SC00892K
TI - Zwitterionic iodonium species afford halogen bond-based porous organic frameworks
T2 - Chemical Science
AU - Soldatova, Natalia
AU - Postnikov, Pavel S.
AU - Ivanov, Daniil M
AU - Semyonov, Oleg V
AU - Kukurina, Olga S
AU - Guselnikova, Olga
AU - YAMAUCHI, Yusuke
AU - Wirth, Thomas
AU - Zhdankin, Viktor V.
AU - Yusubov, Mekhman S.
AU - Gomila, Rosa M.
AU - Frontera, Antonio
AU - Resnati, Giuseppe
AU - Kukushkin, Vadim Yu.
PY - 2022
DA - 2022/04/12
PB - Royal Society of Chemistry (RSC)
SP - 5650-5658
IS - 19
VL - 13
PMID - 35694330
SN - 2041-6520
SN - 2041-6539
ER -
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BibTex (до 50 авторов)
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@article{2022_Soldatova,
author = {Natalia Soldatova and Pavel S. Postnikov and Daniil M Ivanov and Oleg V Semyonov and Olga S Kukurina and Olga Guselnikova and Yusuke YAMAUCHI and Thomas Wirth and Viktor V. Zhdankin and Mekhman S. Yusubov and Rosa M. Gomila and Antonio Frontera and Giuseppe Resnati and Vadim Yu. Kukushkin},
title = {Zwitterionic iodonium species afford halogen bond-based porous organic frameworks},
journal = {Chemical Science},
year = {2022},
volume = {13},
publisher = {Royal Society of Chemistry (RSC)},
month = {apr},
url = {https://xlink.rsc.org/?DOI=D2SC00892K},
number = {19},
pages = {5650--5658},
doi = {10.1039/d2sc00892k}
}
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MLA
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Soldatova, Natalia, et al. “Zwitterionic iodonium species afford halogen bond-based porous organic frameworks.” Chemical Science, vol. 13, no. 19, Apr. 2022, pp. 5650-5658. https://xlink.rsc.org/?DOI=D2SC00892K.