Chemical Communications, volume 60, issue 7, pages 881-884

Aluminyl Derived Ethene Functionalization with Heteroallenes, Leading to an Intramolecular Ligand Rearrangement

Publication type: Journal Article
Publication date: 2024-01-01
scimago Q1
SJR: 1.133
CiteScore: 8.6
Impact factor: 4.3
ISSN: 13597345, 1364548X
DOI:  10.1039/d3cc05785b
PubMed ID:  38165276
Materials Chemistry
Metals and Alloys
Surfaces, Coatings and Films
General Chemistry
Ceramics and Composites
Electronic, Optical and Magnetic Materials
Catalysis
Abstract

The aluminacyclopropane K[Al(NON)(η-C2H4)] ([NON]2– = [O(SiMe2NDipp)2]2–, Dipp = 2,6-iPr2C6H3) reacts with CO2 and iPrN=C=NiPr to afford ring-expanded products of C–C bond formation. The latter system undergoes a 1,3-silyl retro-Brook rearrangement...

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