Photochemical organocatalytic heteroarylation of anilines and secondary alicyclic amines in continuous-flow
Тип публикации: Journal Article
Дата публикации: 2024-04-03
SCImago Q2
WOS Q3
БС1
SJR: 0.571
CiteScore: 5.7
Impact factor: 2.9
ISSN: 20589883
Catalysis
Chemistry (miscellaneous)
Process Chemistry and Technology
Chemical Engineering (miscellaneous)
Fluid Flow and Transfer Processes
Краткое описание
C–N bond formation plays a crucial role in various chemical synthesis processes in both the chemical industry and nature. While numerous methods have been developed for the formation of C–N bonds, only a few meet the criteria of “green chemistry”. In this study, we present a continuous-flow procedure for the decyanative N-heteroarylation of anilines and secondary alicyclic amines using a photoorganocatalytic reaction. Through the synergistic combination of photochemistry, organocatalysis, and continuous-flow technology, we were able to achieve high and close to quantitative yields, while significantly reducing the reaction time from 12 hours in batch procedures to just 1 hour in continuous-flow conditions.
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Boronin E. N. et al. Photochemical organocatalytic heteroarylation of anilines and secondary alicyclic amines in continuous-flow // Reaction Chemistry and Engineering. 2024. Vol. 9. No. 7. pp. 1877-1882.
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Boronin E. N., Svetlakova M. M., Vorobyov I. I., Malysheva Y. B., Polushtaytsev Y. V., Mensov S. N., Vorotyntsev A. V., Fedorov A. Yu., Noel T. R., Nyuchev A. V. Photochemical organocatalytic heteroarylation of anilines and secondary alicyclic amines in continuous-flow // Reaction Chemistry and Engineering. 2024. Vol. 9. No. 7. pp. 1877-1882.
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TY - JOUR
DO - 10.1039/d4re00130c
UR - https://xlink.rsc.org/?DOI=D4RE00130C
TI - Photochemical organocatalytic heteroarylation of anilines and secondary alicyclic amines in continuous-flow
T2 - Reaction Chemistry and Engineering
AU - Boronin, Egor N.
AU - Svetlakova, Milena M.
AU - Vorobyov, Ilya I.
AU - Malysheva, Yulia B
AU - Polushtaytsev, Yuri V
AU - Mensov, Sergey N
AU - Vorotyntsev, A. V.
AU - Fedorov, Alexey Yu
AU - Noel, Timothy R.
AU - Nyuchev, Alexander V.
PY - 2024
DA - 2024/04/03
PB - Royal Society of Chemistry (RSC)
SP - 1877-1882
IS - 7
VL - 9
SN - 2058-9883
ER -
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@article{2024_Boronin,
author = {Egor N. Boronin and Milena M. Svetlakova and Ilya I. Vorobyov and Yulia B Malysheva and Yuri V Polushtaytsev and Sergey N Mensov and A. V. Vorotyntsev and Alexey Yu Fedorov and Timothy R. Noel and Alexander V. Nyuchev},
title = {Photochemical organocatalytic heteroarylation of anilines and secondary alicyclic amines in continuous-flow},
journal = {Reaction Chemistry and Engineering},
year = {2024},
volume = {9},
publisher = {Royal Society of Chemistry (RSC)},
month = {apr},
url = {https://xlink.rsc.org/?DOI=D4RE00130C},
number = {7},
pages = {1877--1882},
doi = {10.1039/d4re00130c}
}
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Boronin, Egor N., et al. “Photochemical organocatalytic heteroarylation of anilines and secondary alicyclic amines in continuous-flow.” Reaction Chemistry and Engineering, vol. 9, no. 7, Apr. 2024, pp. 1877-1882. https://xlink.rsc.org/?DOI=D4RE00130C.
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