Open Access
RSC Advances, volume 4, issue 7, pages 3188-3194
Functional poly(carbonate-co-ether) synthesis from glycidyl methacrylate/CO2copolymerization catalyzed by Zn–Co(iii ) double metal cyanide complex catalyst
Publication type: Journal Article
Publication date: 2014-01-01
Journal:
RSC Advances
Quartile SCImago
Q2
Quartile WOS
Q2
Impact factor: 3.9
ISSN: 20462069, 20462069
General Chemistry
General Chemical Engineering
Abstract
Polycarbonates with pendant functional groups have attracted much attention due to their capability for further chemical modification and post-polymerization. This work describes the synthesis of a poly(carbonate-co-ether) with massive pendant acrylate groups from the copolymerization of glycidyl methacrylate (GMA) with carbon dioxide (CO2), using a nanolamellar zinc-cobalt double metal cyanide complex (Zn–Co(III) DMCC) catalyst. The carbonate linkage content (FCO2) of the poly(carbonate-co-ether) could be varied from 42.2 to 68.0% by changing the polymerization conditions. Of importance, 4-methoxyphenol was applied for regulating the copolymerization. It could not only act as an inhibitor for completely depressing the self-polymerization of GMA via free radical polymerization of the double bond, but also modulate the molecular weight of the resultant copolymers. The obtained copolymer had two terminal hydroxyl groups, which were confirmed by the electrospray ionization-tandem mass spectrometry (ESI-MS) technique. A new thermoset with high glass transition temperature (Tg: 105 or 120 °C) and massive carbonate units as well as hydroxyl (or carboxylic) groups was prepared by the curing reaction of the GMA–CO2 copolymer with allyl alcohol or acrylic acid in the presence of 2,2′-azobisisobutyronitrile (AIBN).
Top-30
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1 publication, 3.85%
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1 publication, 3.85%
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1 publication, 3.85%
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1 publication, 3.85%
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1 publication, 3.85%
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1 publication, 3.85%
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Citations by publishers
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10
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Royal Society of Chemistry (RSC)
10 publications, 38.46%
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Elsevier
5 publications, 19.23%
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Wiley
5 publications, 19.23%
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Springer Nature
1 publication, 3.85%
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American Chemical Society (ACS)
1 publication, 3.85%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 3.85%
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Taylor & Francis
1 publication, 3.85%
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Pleiades Publishing
1 publication, 3.85%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 3.85%
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2
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Wei R. J. et al. Functional poly(carbonate-co-ether) synthesis from glycidyl methacrylate/CO2copolymerization catalyzed by Zn–Co(iii) double metal cyanide complex catalyst // RSC Advances. 2014. Vol. 4. No. 7. pp. 3188-3194.
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Wei R. J., Wei R., Zhang X., Zhang Y., Du B. Y., Fan Zhiqiang 范., Qi G. Functional poly(carbonate-co-ether) synthesis from glycidyl methacrylate/CO2copolymerization catalyzed by Zn–Co(iii) double metal cyanide complex catalyst // RSC Advances. 2014. Vol. 4. No. 7. pp. 3188-3194.
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TY - JOUR
DO - 10.1039/c3ra46046k
UR - https://doi.org/10.1039/c3ra46046k
TI - Functional poly(carbonate-co-ether) synthesis from glycidyl methacrylate/CO2copolymerization catalyzed by Zn–Co(iii) double metal cyanide complex catalyst
T2 - RSC Advances
AU - Wei, Ren Jian
AU - Qi, Guo-rong
AU - Zhang, Xinghong
AU - Zhang, Ying-Ying
AU - Du, B. Y.
AU - Fan Zhiqiang, 范志强
AU - Wei, Ren-jian
PY - 2014
DA - 2014/01/01 00:00:00
PB - Royal Society of Chemistry (RSC)
SP - 3188-3194
IS - 7
VL - 4
SN - 2046-2069
SN - 2046-2069
ER -
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@article{2014_Wei,
author = {Ren Jian Wei and Guo-rong Qi and Xinghong Zhang and Ying-Ying Zhang and B. Y. Du and 范志强 Fan Zhiqiang and Ren-jian Wei},
title = {Functional poly(carbonate-co-ether) synthesis from glycidyl methacrylate/CO2copolymerization catalyzed by Zn–Co(iii) double metal cyanide complex catalyst},
journal = {RSC Advances},
year = {2014},
volume = {4},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://doi.org/10.1039/c3ra46046k},
number = {7},
pages = {3188--3194},
doi = {10.1039/c3ra46046k}
}
Cite this
MLA
Copy
Wei, Ren Jian, et al. “Functional poly(carbonate-co-ether) synthesis from glycidyl methacrylate/CO2copolymerization catalyzed by Zn–Co(iii) double metal cyanide complex catalyst.” RSC Advances, vol. 4, no. 7, Jan. 2014, pp. 3188-3194. https://doi.org/10.1039/c3ra46046k.