Luminescent CuI thiocyanate complexes based on tris(2-pyridyl)phosphine and its oxide: from mono-, di- and trinuclear species to coordination polymers
Marianna I Rakhmanova
2
,
Anastasiya O Sutyrina
1
,
Irina Yu. Bagryanskaya
3, 4
,
Peter M. Tolstoy
5
,
Artem L Gushchin
2, 4
,
A. Mazur
5
,
Nina K. Gusarova
1
,
Publication type: Journal Article
Publication date: 2016-10-06
scimago Q2
wos Q3
SJR: 0.493
CiteScore: 5.0
Impact factor: 2.5
ISSN: 11440546, 13699261
Materials Chemistry
General Chemistry
Catalysis
Abstract
Tris(2-pyridyl)phosphine oxide reacts with CuSCN to form a variety of luminescent complexes, depending on the specified metal-to-ligand ratio and the solvent used, viz. mononuclear [Cu(N,N′,N′′-Py3PO)(NCS)], dinuclear (N,N′-Py3PO)Cu(SCNNCS)Cu[(N,N′-Py3PO)], their co-crystal (2:1, correspondingly) and trinuclear {Cu(NCS)[SCNCu(N,N′,N′′-Py3PO)]2}. In the solid state, these complexes feature red-orange emission upon UV photoexcitation. The reaction of tris(2-pyridyl)phosphine with CuSCN quantitatively produces an almost insoluble coordination polymer, [Cu(Py3P)NCS]n, which exhibits bright green emission. The synthesized compounds are the first members of the hitherto unknown family of Cu(I) thiocyanate complexes supported by tripodal ligands.
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Artem'ev A. V. et al. Luminescent CuI thiocyanate complexes based on tris(2-pyridyl)phosphine and its oxide: from mono-, di- and trinuclear species to coordination polymers // New Journal of Chemistry. 2016. Vol. 40. No. 12. pp. 10028-10040.
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Artem'ev A. V., Doronina E. P., Rakhmanova M. I., Sutyrina A. O., Bagryanskaya I. Y., Tolstoy P. M., Gushchin A. L., Mazur A., Gusarova N. K., Trofimov B. A. Luminescent CuI thiocyanate complexes based on tris(2-pyridyl)phosphine and its oxide: from mono-, di- and trinuclear species to coordination polymers // New Journal of Chemistry. 2016. Vol. 40. No. 12. pp. 10028-10040.
Cite this
RIS
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TY - JOUR
DO - 10.1039/C6NJ02087A
UR - https://xlink.rsc.org/?DOI=C6NJ02087A
TI - Luminescent CuI thiocyanate complexes based on tris(2-pyridyl)phosphine and its oxide: from mono-, di- and trinuclear species to coordination polymers
T2 - New Journal of Chemistry
AU - Artem'ev, Alexander V.
AU - Doronina, Evgeniya P
AU - Rakhmanova, Marianna I
AU - Sutyrina, Anastasiya O
AU - Bagryanskaya, Irina Yu.
AU - Tolstoy, Peter M.
AU - Gushchin, Artem L
AU - Mazur, A.
AU - Gusarova, Nina K.
AU - Trofimov, B. A.
PY - 2016
DA - 2016/10/06
PB - Royal Society of Chemistry (RSC)
SP - 10028-10040
IS - 12
VL - 40
SN - 1144-0546
SN - 1369-9261
ER -
Cite this
BibTex (up to 50 authors)
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@article{2016_Artem'ev,
author = {Alexander V. Artem'ev and Evgeniya P Doronina and Marianna I Rakhmanova and Anastasiya O Sutyrina and Irina Yu. Bagryanskaya and Peter M. Tolstoy and Artem L Gushchin and A. Mazur and Nina K. Gusarova and B. A. Trofimov},
title = {Luminescent CuI thiocyanate complexes based on tris(2-pyridyl)phosphine and its oxide: from mono-, di- and trinuclear species to coordination polymers},
journal = {New Journal of Chemistry},
year = {2016},
volume = {40},
publisher = {Royal Society of Chemistry (RSC)},
month = {oct},
url = {https://xlink.rsc.org/?DOI=C6NJ02087A},
number = {12},
pages = {10028--10040},
doi = {10.1039/C6NJ02087A}
}
Cite this
MLA
Copy
Artem'ev, Alexander V., et al. “Luminescent CuI thiocyanate complexes based on tris(2-pyridyl)phosphine and its oxide: from mono-, di- and trinuclear species to coordination polymers.” New Journal of Chemistry, vol. 40, no. 12, Oct. 2016, pp. 10028-10040. https://xlink.rsc.org/?DOI=C6NJ02087A.