Journal of Materials Chemistry A, volume 5, issue 10, pages 4940-4948
High-voltage and free-standing poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 composite solid electrolyte for wide temperature range and flexible solid lithium ion battery
Jian Jun Zhang
1, 2
,
Xiao Zang
1
,
Huijie Wen
1
,
Tiantian Dong
1
,
Jingchao Chai
1, 2
,
Yang Li
1, 2
,
Bingbing Chen
1
,
Jingwen Zhao
1
,
Shanmu Dong
1
,
Ying Sun
1
,
Liping Yue
1
,
Zhihong Liu
1
,
Xiangxin Guo
3
,
Guanglei Cui
1
,
Liquan Chen
4
1
Qingdao Industrial Energy Storage Technology Institute, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, P. R. China
|
Publication type: Journal Article
Publication date: 2017-02-01
Journal:
Journal of Materials Chemistry A
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 11.9
ISSN: 20507488, 20507496, 09599428, 13645501
General Chemistry
General Materials Science
Renewable Energy, Sustainability and the Environment
Abstract
Solid electrolyte is regarded as a perfect way to enhance safety issues and boost energy density of lithium batteries. Herein, we developed a type of free-standing poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 composite solid electrolyte for ambient temperature and flexible solid-state lithium batteries. The composite solid electrolyte exhibited excellent comprehensive performance in terms of high ionic conductivity (5.2 × 10−4 S cm−1) at 20 °C, a wide electrochemical window (4.6 V), high ionic transference number (0.75) and satisfactory mechanical strength (6.8 MPa). When evaluated as solid electrolyte for an ambient-temperature solid lithium battery, such a composite electrolyte delivered excellent rate capability (5C) at 20 °C. This superior performance can be comparable to a liquid electrolyte-soaked PP separator-based lithium battery at room temperature. To our knowledge, this is the best rate capability of a solid composite electrolyte for a solid lithium battery at ambient temperature. Moreover, such a composite electrolyte-based flexible LiFePO4/Li4Ti5O12 lithium ion battery delivered excellent rate capability and superior cycling stability. All these fascinating features make poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 a very promising all-solid-state electrolyte for flexible solid lithium batteries. Our study makes a big step into addressing the challenges of ambient-temperature solid lithium batteries.
Top-30
Citations by journals
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Citations by publishers
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20
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120
140
160
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Elsevier
147 publications, 40.38%
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Wiley
65 publications, 17.86%
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American Chemical Society (ACS)
51 publications, 14.01%
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Royal Society of Chemistry (RSC)
44 publications, 12.09%
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Springer Nature
21 publications, 5.77%
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The Electrochemical Society
7 publications, 1.92%
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Multidisciplinary Digital Publishing Institute (MDPI)
4 publications, 1.1%
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Frontiers Media S.A.
3 publications, 0.82%
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Tsinghua University Press
3 publications, 0.82%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
2 publications, 0.55%
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IOP Publishing
2 publications, 0.55%
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Bentham Science
1 publication, 0.27%
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The Chemical Society of Japan
1 publication, 0.27%
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World Scientific
1 publication, 0.27%
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Ceramic Society of Japan
1 publication, 0.27%
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Materials Research Society
1 publication, 0.27%
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Chinese Ceramic Society
1 publication, 0.27%
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Oxford University Press
1 publication, 0.27%
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Shanghai Institute of Ceramics
1 publication, 0.27%
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OAE Publishing Inc.
1 publication, 0.27%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhang J. J. et al. High-voltage and free-standing poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 composite solid electrolyte for wide temperature range and flexible solid lithium ion battery // Journal of Materials Chemistry A. 2017. Vol. 5. No. 10. pp. 4940-4948.
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Zhang J. J., Zang X., Wen H., Dong T., Chai J., Li Y., Chen B., Zhao J., Dong S., Sun Y., Yue L., Liu Z., Guo X., Cui G., Chen L. High-voltage and free-standing poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 composite solid electrolyte for wide temperature range and flexible solid lithium ion battery // Journal of Materials Chemistry A. 2017. Vol. 5. No. 10. pp. 4940-4948.
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TY - JOUR
DO - 10.1039/C6TA10066J
UR - https://doi.org/10.1039/C6TA10066J
TI - High-voltage and free-standing poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 composite solid electrolyte for wide temperature range and flexible solid lithium ion battery
T2 - Journal of Materials Chemistry A
AU - Zang, Xiao
AU - Wen, Huijie
AU - Dong, Tiantian
AU - Chai, Jingchao
AU - Chen, Bingbing
AU - Dong, Shanmu
AU - Yue, Liping
AU - Liu, Zhihong
AU - Cui, Guanglei
AU - Zhang, Jian Jun
AU - Li, Yang
AU - Zhao, Jingwen
AU - Sun, Ying
AU - Guo, Xiangxin
AU - Chen, Liquan
PY - 2017
DA - 2017/02/01 00:00:00
PB - Royal Society of Chemistry (RSC)
SP - 4940-4948
IS - 10
VL - 5
SN - 2050-7488
SN - 2050-7496
SN - 0959-9428
SN - 1364-5501
ER -
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@article{2017_Zhang,
author = {Xiao Zang and Huijie Wen and Tiantian Dong and Jingchao Chai and Bingbing Chen and Shanmu Dong and Liping Yue and Zhihong Liu and Guanglei Cui and Jian Jun Zhang and Yang Li and Jingwen Zhao and Ying Sun and Xiangxin Guo and Liquan Chen},
title = {High-voltage and free-standing poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 composite solid electrolyte for wide temperature range and flexible solid lithium ion battery},
journal = {Journal of Materials Chemistry A},
year = {2017},
volume = {5},
publisher = {Royal Society of Chemistry (RSC)},
month = {feb},
url = {https://doi.org/10.1039/C6TA10066J},
number = {10},
pages = {4940--4948},
doi = {10.1039/C6TA10066J}
}
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Zhang, Jian Jun, et al. “High-voltage and free-standing poly(propylene carbonate)/Li6.75La3Zr1.75Ta0.25O12 composite solid electrolyte for wide temperature range and flexible solid lithium ion battery.” Journal of Materials Chemistry A, vol. 5, no. 10, Feb. 2017, pp. 4940-4948. https://doi.org/10.1039/C6TA10066J.
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