Synthesis, photophysical properties and cation-binding studies of bipyridine-functionalized gold(I) complexes
Igor V Solovyev
1, 2, 3, 4, 5, 6, 7
,
Aleksandar Kondinski
8
,
Kirill Yu. Monakhov
8, 9, 10, 11, 12
,
Igor O Koshevoy
2, 7, 13, 14, 15
,
Elena V Grachova
1, 3, 4, 5, 6
3
Institute of Chemistry
5
198504 St. Petersburg
6
Russia
|
7
DEPARTMENT OF CHEMISTRY
9
Institut für Anorganische Chemie
11
52074 Aachen
|
12
GERMANY
|
14
80101 Joensuu
|
15
FINLAND
|
Publication type: Journal Article
Publication date: 2018-01-01
scimago Q1
wos Q1
SJR: 1.276
CiteScore: 9.9
Impact factor: 6.4
ISSN: 20521545, 20521553
Inorganic Chemistry
Abstract
Gold(I) has been used as an interlocking center to design five phenyl-bipyridine based complexes [LAu(L1)] and [RAu(L2)] where L1 = 5-(4-ethynylphenyl)-2,2′-bipyridine and L2 = 5-(4-(diphenylphosphino)phenyl)-2,2′-bipyridine (L = P(C6H11)3, 1; C6H3(CH3)2NC, 2; R = Ph2OHCC2, 3; PhC2, 4; C6F5, 5). The obtained compounds have been characterized by polynuclear NMR spectroscopy and X-ray crystallography. Investigation of their UV-Vis absorption and emission characteristics has been supported by density functional theory (DFT) calculations that rationalize the tunable electronic properties of these compounds. Complexation of the metal cations and the corresponding optical responses of [LAu(L1)], in particular for Cd(II) and Pb(II), indicate the important role of gold(I) ions in modulating the luminescence characteristics of these species upon binding the analyte cations.
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Solovyev I. V. et al. Synthesis, photophysical properties and cation-binding studies of bipyridine-functionalized gold(I) complexes // Inorganic Chemistry Frontiers. 2018. Vol. 5. No. 1. pp. 160-171.
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Solovyev I. V., Kondinski A., Monakhov K. Y., Koshevoy I. O., Grachova E. V. Synthesis, photophysical properties and cation-binding studies of bipyridine-functionalized gold(I) complexes // Inorganic Chemistry Frontiers. 2018. Vol. 5. No. 1. pp. 160-171.
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TY - JOUR
DO - 10.1039/C7QI00514H
UR - https://xlink.rsc.org/?DOI=C7QI00514H
TI - Synthesis, photophysical properties and cation-binding studies of bipyridine-functionalized gold(I) complexes
T2 - Inorganic Chemistry Frontiers
AU - Solovyev, Igor V
AU - Kondinski, Aleksandar
AU - Monakhov, Kirill Yu.
AU - Koshevoy, Igor O
AU - Grachova, Elena V
PY - 2018
DA - 2018/01/01
PB - Royal Society of Chemistry (RSC)
SP - 160-171
IS - 1
VL - 5
SN - 2052-1545
SN - 2052-1553
ER -
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@article{2018_Solovyev,
author = {Igor V Solovyev and Aleksandar Kondinski and Kirill Yu. Monakhov and Igor O Koshevoy and Elena V Grachova},
title = {Synthesis, photophysical properties and cation-binding studies of bipyridine-functionalized gold(I) complexes},
journal = {Inorganic Chemistry Frontiers},
year = {2018},
volume = {5},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://xlink.rsc.org/?DOI=C7QI00514H},
number = {1},
pages = {160--171},
doi = {10.1039/C7QI00514H}
}
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MLA
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Solovyev, Igor V., et al. “Synthesis, photophysical properties and cation-binding studies of bipyridine-functionalized gold(I) complexes.” Inorganic Chemistry Frontiers, vol. 5, no. 1, Jan. 2018, pp. 160-171. https://xlink.rsc.org/?DOI=C7QI00514H.
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