Open Access
A highly active non-precious transition metal catalyst for the hydrogenation of carbon dioxide to formates
Benjamin G Schieweck
1, 2, 3, 4, 5
,
Niklas F Westhues
1, 2, 3, 4, 5
,
Jürgen Klankermayer
1, 2, 3, 4, 5
2
Institut für Makromolekulare und Technische Chemie
4
52074 Aachen
|
5
GERMANY
|
Publication type: Journal Article
Publication date: 2019-05-31
scimago Q1
wos Q1
SJR: 2.138
CiteScore: 12.6
Impact factor: 7.4
ISSN: 20416520, 20416539
PubMed ID:
31341604
General Chemistry
Abstract
Herein a highly active non-precious transition metal catalyst system for homogeneous hydrogenation of carbon dioxide to formate is presented. The application of selected nickel(II) salts in combination with tailored multidentate ligands enabled the effective transformation of carbon dioxide with an exceptional TON of up to 4.65 × 106. This unprecedented productivity based on the novel nickel catalyst not only outmatches that of existing systems containing first row transition metals, but also established catalysts based on precious transition metals.
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Metrics
45
Total citations:
45
Citations from 2024:
18
(40%)
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MLA
Cite this
GOST
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Schieweck B. G. et al. A highly active non-precious transition metal catalyst for the hydrogenation of carbon dioxide to formates // Chemical Science. 2019. Vol. 10. No. 26. pp. 6519-6523.
GOST all authors (up to 50)
Copy
Schieweck B. G., Westhues N. F., Klankermayer J. A highly active non-precious transition metal catalyst for the hydrogenation of carbon dioxide to formates // Chemical Science. 2019. Vol. 10. No. 26. pp. 6519-6523.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1039/c8sc05230a
UR - https://xlink.rsc.org/?DOI=C8SC05230A
TI - A highly active non-precious transition metal catalyst for the hydrogenation of carbon dioxide to formates
T2 - Chemical Science
AU - Schieweck, Benjamin G
AU - Westhues, Niklas F
AU - Klankermayer, Jürgen
PY - 2019
DA - 2019/05/31
PB - Royal Society of Chemistry (RSC)
SP - 6519-6523
IS - 26
VL - 10
PMID - 31341604
SN - 2041-6520
SN - 2041-6539
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2019_Schieweck,
author = {Benjamin G Schieweck and Niklas F Westhues and Jürgen Klankermayer},
title = {A highly active non-precious transition metal catalyst for the hydrogenation of carbon dioxide to formates},
journal = {Chemical Science},
year = {2019},
volume = {10},
publisher = {Royal Society of Chemistry (RSC)},
month = {may},
url = {https://xlink.rsc.org/?DOI=C8SC05230A},
number = {26},
pages = {6519--6523},
doi = {10.1039/c8sc05230a}
}
Cite this
MLA
Copy
Schieweck, Benjamin G., et al. “A highly active non-precious transition metal catalyst for the hydrogenation of carbon dioxide to formates.” Chemical Science, vol. 10, no. 26, May. 2019, pp. 6519-6523. https://xlink.rsc.org/?DOI=C8SC05230A.