Unprecedented plasmon-induced nitroxide-mediated polymerization (PI-NMP): a method for preparation of functional surfaces
Тип публикации: Journal Article
Дата публикации: 2019-04-01
scimago Q1
wos Q1
БС1
SJR: 2.462
CiteScore: 16.7
Impact factor: 9.5
ISSN: 20507488, 20507496, 09599428, 13645501
General Chemistry
General Materials Science
Renewable Energy, Sustainability and the Environment
Краткое описание
A plasmon as a stimulus opens up new opportunities for selective and regulated “from-surface” polymerization and functionalization of surfaces. Here, the first example of plasmon-assisted nitroxide-mediated polymerization (NMP) of stimuli-responsive block copolymers poly(N-isopropylacrylamide)-co-4-vinylboronic acid is reported. The growth of a polymer film at room temperature was achieved via plasmon-induced homolysis of alkoxyamines covalently attached to the surface of plasmon-active gold gratings at room temperature. Control of temperature, finite-difference time-domain method simulation of plasmon intensity distribution shift during polymerization, electron paramagnetic resonance experiments and other assays provide strong support for the plasmon-initiated mechanism of NMP. We demonstrated not only the control of the resulting polymer thickness but also the preparation of a surface-enhanced Raman spectroscopy chip for the detection of glycoproteins as a powerful example of plasmon-assisted NMP potential.
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Guselnikova O. et al. Unprecedented plasmon-induced nitroxide-mediated polymerization (PI-NMP): a method for preparation of functional surfaces // Journal of Materials Chemistry A. 2019. Vol. 7. No. 20. pp. 12414-12419.
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Guselnikova O. et al. Unprecedented plasmon-induced nitroxide-mediated polymerization (PI-NMP): a method for preparation of functional surfaces // Journal of Materials Chemistry A. 2019. Vol. 7. No. 20. pp. 12414-12419.
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TY - JOUR
DO - 10.1039/C9TA01630A
UR - https://xlink.rsc.org/?DOI=C9TA01630A
TI - Unprecedented plasmon-induced nitroxide-mediated polymerization (PI-NMP): a method for preparation of functional surfaces
T2 - Journal of Materials Chemistry A
AU - Guselnikova, Olga
AU - Marque, Sylvain R. A.
AU - Tretyakov, Evgeny
AU - Mares, David
AU - Jerabek, Vitezslav
AU - Audran, Gérard
AU - Joly, Jean-Patrick
AU - Trusova, Marina
AU - Švorčík, Václav
AU - Svorcik, Vaclav
AU - Lyutakov, Oleksiy
AU - Postnikov, Pavel S.
PY - 2019
DA - 2019/04/01
PB - Royal Society of Chemistry (RSC)
SP - 12414-12419
IS - 20
VL - 7
SN - 2050-7488
SN - 2050-7496
SN - 0959-9428
SN - 1364-5501
ER -
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@article{2019_Guselnikova,
author = {Olga Guselnikova and Sylvain R. A. Marque and Evgeny Tretyakov and David Mares and Vitezslav Jerabek and Gérard Audran and Jean-Patrick Joly and Marina Trusova and Václav Švorčík and Vaclav Svorcik and Oleksiy Lyutakov and Pavel S. Postnikov and others},
title = {Unprecedented plasmon-induced nitroxide-mediated polymerization (PI-NMP): a method for preparation of functional surfaces},
journal = {Journal of Materials Chemistry A},
year = {2019},
volume = {7},
publisher = {Royal Society of Chemistry (RSC)},
month = {apr},
url = {https://xlink.rsc.org/?DOI=C9TA01630A},
number = {20},
pages = {12414--12419},
doi = {10.1039/C9TA01630A}
}
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MLA
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Guselnikova, Olga, et al. “Unprecedented plasmon-induced nitroxide-mediated polymerization (PI-NMP): a method for preparation of functional surfaces.” Journal of Materials Chemistry A, vol. 7, no. 20, Apr. 2019, pp. 12414-12419. https://xlink.rsc.org/?DOI=C9TA01630A.
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