Journal of Materials Chemistry A, volume 8, issue 4, pages 1557-1577
Single-ion conducting gel polymer electrolytes: design, preparation and application
Kuirong Deng
1
,
Qingguang Zeng
1
,
Da Wang
1
,
Zheng Liu
1, 2
,
Zhenping Qiu
1
,
Yangfan Zhang
3
,
Min Xiao
4
,
2
Jiangmen Advanced Battery Material Engineering and Technology Research Center, Jiangmen, Guangdong 529020, P. R. China
|
Publication type: Journal Article
Publication date: 2020-01-01
Journal:
Journal of Materials Chemistry A
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 11.9
ISSN: 20507488, 20507496, 09599428, 13645501
General Chemistry
General Materials Science
Renewable Energy, Sustainability and the Environment
Abstract
Electrolytes as pivotal components of lithium-ion batteries (LIBs) and lithium metal batteries (LMBs) influence the capacity, cycle stability, safety and operating conditions of the batteries. An ideal electrolyte should possess high ionic conductivity, enhanced safety, unity lithium ion transference number (LITN) and good electrochemical stability. Single-ion conducting solid polymer electrolytes (SIC-SPEs) have garnered considerable attention due to their unique unity LITNs. In SIC-SPEs, immobilization of anions gives rise to unity LITNs, the absences of anionic concentration polarization, low internal impedances, higher discharge voltages and suppressions of lithium dendrite growth. Single-ion conducting gel polymer electrolytes (SIC-GPEs) can be fabricated by adding plasticizers to SIC-SPEs to enhance the ionic conductivities. Meanwhile, the original feature of unity LITNs (∼0.98) remains. Therefore, SIC-GPEs have been widely applied in LFP cells, LTO cells, LMO cells and Li/S cells, which showed excellent cycle stabilities, good rate capabilities and high capacities at ambient temperature. Good compatibility with lithium metal anodes and suppression of lithium dendrites that benefited from immobilization of anions are also inherited for SIC-GPEs. The current status of SIC-GPEs in terms of designs, preparation methods, electrochemical performances and applications is described in this review. The development directions and future prospects of SIC-GPEs are also discussed.
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Deng K. et al. Single-ion conducting gel polymer electrolytes: design, preparation and application // Journal of Materials Chemistry A. 2020. Vol. 8. No. 4. pp. 1557-1577.
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Deng K., Zeng Q., Wang D., Liu Z., Qiu Z., Zhang Y., Xiao M., Meng Y. L. Single-ion conducting gel polymer electrolytes: design, preparation and application // Journal of Materials Chemistry A. 2020. Vol. 8. No. 4. pp. 1557-1577.
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TY - JOUR
DO - 10.1039/C9TA11178F
UR - https://doi.org/10.1039/C9TA11178F
TI - Single-ion conducting gel polymer electrolytes: design, preparation and application
T2 - Journal of Materials Chemistry A
AU - Deng, Kuirong
AU - Zeng, Qingguang
AU - Wang, Da
AU - Zhang, Yangfan
AU - Meng, Y. L.
AU - Liu, Zheng
AU - Qiu, Zhenping
AU - Xiao, Min
PY - 2020
DA - 2020/01/01 00:00:00
PB - Royal Society of Chemistry (RSC)
SP - 1557-1577
IS - 4
VL - 8
SN - 2050-7488
SN - 2050-7496
SN - 0959-9428
SN - 1364-5501
ER -
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@article{2020_Deng,
author = {Kuirong Deng and Qingguang Zeng and Da Wang and Yangfan Zhang and Y. L. Meng and Zheng Liu and Zhenping Qiu and Min Xiao},
title = {Single-ion conducting gel polymer electrolytes: design, preparation and application},
journal = {Journal of Materials Chemistry A},
year = {2020},
volume = {8},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://doi.org/10.1039/C9TA11178F},
number = {4},
pages = {1557--1577},
doi = {10.1039/C9TA11178F}
}
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MLA
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Deng, Kuirong, et al. “Single-ion conducting gel polymer electrolytes: design, preparation and application.” Journal of Materials Chemistry A, vol. 8, no. 4, Jan. 2020, pp. 1557-1577. https://doi.org/10.1039/C9TA11178F.
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