Journal of Materials Chemistry A

, volume 9 , issue 10 , pages 5952-5979

Interrelated interfacial issues between a Li₇La₃Zr₂O₁₂-based garnet electrolyte and Li anode in the solid-state lithium battery: a review

Lijie Yang ^{1, 2, 3, 4, 5, 6}

Zaili Lu ^{1, 2, 3, 4, 5, 6}

Yuanxue Qin ^{4, 5, 6, 7, 8}

Chen Wu ^{4, 5, 6, 7, 8}

Chuankai Fu ^{6, 9, 10, 11, 12}

Yunzhi Gao ^{6, 9, 10, 11, 12}

Jun Liu ¹

Liang Jiang ^{1, 2, 3, 4, 5, 6}

Zhongyu Du ^{1, 2, 3, 4, 5, 6}

Zengyang Xie ¹

Li Zhenquan ^{1, 2, 3, 4, 5, 6}

Fandong Kong ^{4, 6, 13, 14, 15}

Geping Yin ^{6, 9, 10, 11, 12}

Hide authors affiliations Show authors affiliations: 15 affiliations

Laboratory of New Antitumor Drug Molecular Design & Synthesis, College of Basic Medicine, Jining Medical University, Jining 272067, China |

Laboratory of New Antitumor Drug Molecular Design & Synthesis

College of Basic Medicine

⁴

Jining Medical University |

⁵

Jining 272067 |

⁶

CHINA |

⁷

Clinical Medical College, Jining Medical University, Jining 272067, China |

⁸

Clinical Medical College

⁹

School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, China |

¹⁰

School of chemistry and chemical engineering

¹¹

HarBin Institute of Technology |

¹²

Harbin 150001 |

¹³

College of Pharmacy, Jining Medical University, Rizhao 276826, China |

¹⁴

College of Pharmacy

¹⁵

Rizhao 276826 |

Publication type: Journal Article

Publication date: 2021-01-29

Royal Society of Chemistry (RSC)

Journal of Materials Chemistry A

scimago Q1

wos Q1

SJR: 2.462

CiteScore: 16.7

Impact factor: 9.5

ISSN: 20507488, 20507496, 09599428, 13645501

DOI: 10.1039/d0ta08179e

Copy DOI

General Chemistry

General Materials Science

Renewable Energy, Sustainability and the Environment

Abstract

The Li7La3Zr2O12-based garnet (LLZO-BG) electrolyte has the advantage of strong thermal stability and can, therefore, avoid the flammability problem of organic electrolyte solutions. However, the solid-state lithium battery with LLZO-BG electrolyte has a much larger electrochemical resistance and poorer performance than the battery with an organic electrolyte solution, which is mainly related to the electrolyte/electrode interface. From the perspective of the LLZO-BG/Li interface, this review explores several interrelated interfacial issues, including the air instability of LLZO-BG, poor LLZO-BG/Li interfacial contact, easily generated lithium dendrite and the instability of LLZO-BG with the Li anode. We elaborate on the forming mechanisms, affecting factors and measures for improving these issues, and prospects for the future research directions of the LLZO-BG/Li interface. This review can provide new ideas for producing a solid-state lithium battery with high safety and high energy density.

Found

1 citation

Voropaeva Daria

PhD in Chemistry

33 publications, 506 citations, 18 reviews

h-index: 13

Kurnakov Institute of General and Inorganic Chemistry of the Russian Academy of Sciences

Research interests

Green technologies

Lithium-ion batteries

Membrane materials

Sodium-ion batteries

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Yang L. et al. Interrelated interfacial issues between a Li7La3Zr2O12-based garnet electrolyte and Li anode in the solid-state lithium battery: a review // Journal of Materials Chemistry A. 2021. Vol. 9. No. 10. pp. 5952-5979.

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RIS |

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RIS Copy

TY - JOUR

DO - 10.1039/d0ta08179e

UR - https://xlink.rsc.org/?DOI=D0TA08179E

TI - Interrelated interfacial issues between a Li7La3Zr2O12-based garnet electrolyte and Li anode in the solid-state lithium battery: a review

T2 - Journal of Materials Chemistry A

AU - Yang, Lijie

AU - Lu, Zaili

AU - Qin, Yuanxue

AU - Wu, Chen

AU - Fu, Chuankai

AU - Gao, Yunzhi

AU - Liu, Jun

AU - Jiang, Liang

AU - Du, Zhongyu

AU - Xie, Zengyang

AU - Zhenquan, Li

AU - Kong, Fandong

AU - Yin, Geping

PY - 2021

DA - 2021/01/29

PB - Royal Society of Chemistry (RSC)

SP - 5952-5979

IS - 10

VL - 9

SN - 2050-7488

SN - 2050-7496

SN - 0959-9428

SN - 1364-5501

ER -

BibTex |

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BibTex (up to 50 authors) Copy

@article{2021_Yang,

author = {Lijie Yang and Zaili Lu and Yuanxue Qin and Chen Wu and Chuankai Fu and Yunzhi Gao and Jun Liu and Liang Jiang and Zhongyu Du and Zengyang Xie and Li Zhenquan and Fandong Kong and Geping Yin and others},

title = {Interrelated interfacial issues between a Li7La3Zr2O12-based garnet electrolyte and Li anode in the solid-state lithium battery: a review},

journal = {Journal of Materials Chemistry A},

year = {2021},

volume = {9},

publisher = {Royal Society of Chemistry (RSC)},

month = {jan},

url = {https://xlink.rsc.org/?DOI=D0TA08179E},

number = {10},

pages = {5952--5979},

doi = {10.1039/d0ta08179e}

}

MLA

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MLA Copy

Yang, Lijie, et al. “Interrelated interfacial issues between a Li7La3Zr2O12-based garnet electrolyte and Li anode in the solid-state lithium battery: a review.” Journal of Materials Chemistry A, vol. 9, no. 10, Jan. 2021, pp. 5952-5979. https://xlink.rsc.org/?DOI=D0TA08179E.

Publisher

Royal Society of Chemistry (RSC)

Journal

Journal of Materials Chemistry A

scimago Q1

wos Q1

SJR

2.462

CiteScore

16.7

Impact factor

9.5

ISSN

20507488 (Print)

20507496 (Electronic)

09599428 (Print)

13645501 (Electronic)