Chemical Communications

, том 57 , издание 42 , страницы 5195-5198

Acyl fluorides as direct precursors to fluoride ketyl radicals: reductive deuteration using SmI₂ and D₂O

Тип публикации: Journal Article

Дата публикации: 2021-04-21

Royal Society of Chemistry (RSC)

Chemical Communications

SCImago Q1

WOS Q2

БС1

SJR: 0.907

CiteScore: 7.2

Impact factor: 4.3

ISSN: 13597345, 1364548X

DOI: 10.1039/d1cc01381e

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PubMed ID: 33908475

Materials Chemistry

Metals and Alloys

Surfaces, Coatings and Films

General Chemistry

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Electronic, Optical and Magnetic Materials

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A highly chemoselective reductive deuteration of acyl fluorides to provide α,α-dideuterio alcohols with exquisite levels of deuterium incorporation was developed using SmI2 and D2O as the deuterium source. This method introduces acyl fluorides as attractive radical precursors for the generation of reactive acyl-type fluoride ketyls that should find widespread application in many synthetic strategies involving single electron transfer processes.

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Li H. et al. Acyl fluorides as direct precursors to fluoride ketyl radicals: reductive deuteration using SmI2 and D2O // Chemical Communications. 2021. Vol. 57. No. 42. pp. 5195-5198.

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Li H. et al. Acyl fluorides as direct precursors to fluoride ketyl radicals: reductive deuteration using SmI2 and D2O // Chemical Communications. 2021. Vol. 57. No. 42. pp. 5195-5198.

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TY - JOUR

DO - 10.1039/d1cc01381e

UR - https://xlink.rsc.org/?DOI=D1CC01381E

TI - Acyl fluorides as direct precursors to fluoride ketyl radicals: reductive deuteration using SmI2 and D2O

T2 - Chemical Communications

AU - Li, Hengzhao

AU - Peng, Mengqi

AU - Lai, Zemin

AU - Ning, Lei

AU - Chen, Xingyue

AU - Zhang, Xiaoxu

AU - Wang, Pengjie

AU - Szostak, R.

AU - Szostak, Michal

AU - AN, JIE

PY - 2021

DA - 2021/04/21

PB - Royal Society of Chemistry (RSC)

SP - 5195-5198

IS - 42

VL - 57

PMID - 33908475

SN - 1359-7345

SN - 1364-548X

ER -

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@article{2021_Li,

author = {Hengzhao Li and Mengqi Peng and Zemin Lai and Lei Ning and Xingyue Chen and Xiaoxu Zhang and Pengjie Wang and R. Szostak and Michal Szostak and JIE AN and others},

title = {Acyl fluorides as direct precursors to fluoride ketyl radicals: reductive deuteration using SmI2 and D2O},

journal = {Chemical Communications},

year = {2021},

volume = {57},

publisher = {Royal Society of Chemistry (RSC)},

month = {apr},

url = {https://xlink.rsc.org/?DOI=D1CC01381E},

number = {42},

pages = {5195--5198},

doi = {10.1039/d1cc01381e}

}

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Li, Hengzhao, et al. “Acyl fluorides as direct precursors to fluoride ketyl radicals: reductive deuteration using SmI2 and D2O.” Chemical Communications, vol. 57, no. 42, Apr. 2021, pp. 5195-5198. https://xlink.rsc.org/?DOI=D1CC01381E.

Издатель

Royal Society of Chemistry (RSC)

Журнал

Chemical Communications

SCImago Q1

WOS Q2

БС1