Open Access
Recent advances in single atom catalysts for the electrochemical carbon dioxide reduction reaction
Jincheng Zhang
1, 2, 3, 4
,
Weizheng Cai
1, 2, 3, 4
,
Fang Xin Hu
5, 6, 7, 8, 9
,
Yang Hongbin
5
,
Yang Hongbin
5, 6, 7, 8, 9
,
Bin Liu
1, 2, 3, 4
2
School of Chemical and Biomedical Engineering
4
Singapore
|
6
Institute for Materials Science and Devices
8
Suzhou
|
9
CHINA
|
Publication type: Journal Article
Publication date: 2021-04-26
scimago Q1
wos Q1
SJR: 2.138
CiteScore: 12.6
Impact factor: 7.4
ISSN: 20416520, 20416539
PubMed ID:
34123313
General Chemistry
Abstract
The electrochemical carbon dioxide reduction reaction (CO2RR) offers a promising solution to mitigate carbon emission and at the same time generate valuable carbonaceous chemicals/fuels. Single atom catalysts (SACs) are encouraging to catalyze the electrochemical CO2RR due to the tunable electronic structure of the central metal atoms, which can regulate the adsorption energy of reactants and reaction intermediates. Moreover, SACs form a bridge between homogeneous and heterogeneous catalysts, providing an ideal platform to explore the reaction mechanism of electrochemical reactions. In this review, we first discuss the strategies for promoting the CO2RR performance, including suppression of the hydrogen evolution reaction (HER), generation of C1 products and formation of C2+ products. Then, we summarize the recent developments in regulating the structure of SACs toward the CO2RR based on the above aspects. Finally, several issues regarding the development of SACs for the CO2RR are raised and possible solutions are provided.
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Metrics
239
Total citations:
239
Citations from 2024:
139
(58.16%)
Cite this
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MLA
Cite this
GOST
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Zhang J. et al. Recent advances in single atom catalysts for the electrochemical carbon dioxide reduction reaction // Chemical Science. 2021. Vol. 12. No. 20. pp. 6800-6819.
GOST all authors (up to 50)
Copy
Zhang J., Cai W., Hu F. X., Hongbin Y., Yang Hongbin, Liu B. Recent advances in single atom catalysts for the electrochemical carbon dioxide reduction reaction // Chemical Science. 2021. Vol. 12. No. 20. pp. 6800-6819.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1039/d1sc01375k
UR - https://xlink.rsc.org/?DOI=D1SC01375K
TI - Recent advances in single atom catalysts for the electrochemical carbon dioxide reduction reaction
T2 - Chemical Science
AU - Zhang, Jincheng
AU - Cai, Weizheng
AU - Hu, Fang Xin
AU - Hongbin, Yang
AU - Yang Hongbin
AU - Liu, Bin
PY - 2021
DA - 2021/04/26
PB - Royal Society of Chemistry (RSC)
SP - 6800-6819
IS - 20
VL - 12
PMID - 34123313
SN - 2041-6520
SN - 2041-6539
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2021_Zhang,
author = {Jincheng Zhang and Weizheng Cai and Fang Xin Hu and Yang Hongbin and Yang Hongbin and Bin Liu},
title = {Recent advances in single atom catalysts for the electrochemical carbon dioxide reduction reaction},
journal = {Chemical Science},
year = {2021},
volume = {12},
publisher = {Royal Society of Chemistry (RSC)},
month = {apr},
url = {https://xlink.rsc.org/?DOI=D1SC01375K},
number = {20},
pages = {6800--6819},
doi = {10.1039/d1sc01375k}
}
Cite this
MLA
Copy
Zhang, Jincheng, et al. “Recent advances in single atom catalysts for the electrochemical carbon dioxide reduction reaction.” Chemical Science, vol. 12, no. 20, Apr. 2021, pp. 6800-6819. https://xlink.rsc.org/?DOI=D1SC01375K.