Catalysis Science and Technology

, volume 12 , issue 16 , pages 5152-5161

Highly efficient and selective photocatalytic CO₂ reduction using MIL-125(Ti) and based on LiFePO₄ and CuO QDs surface–interface regulation

Jun Zhou ¹

Qinwei Jia ¹

Luyu Wang ¹

Yuhang Zhao ¹

Xiaofan Ma ¹

Lei Gong ¹

Haonan Zhang ¹

Tong ZUO ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

College of Environmental and Safety Engineering, Qingdao University of Science and Technology, 53 Zhengzhou Road, Qingdao, Shandong Province 266042, P. R. China |

Publication type: Journal Article

Publication date: 2022-06-24

Royal Society of Chemistry (RSC)

Catalysis Science and Technology

scimago Q2

wos Q2

SJR: 1.026

CiteScore: 8.0

Impact factor: 4.2

ISSN: 20444753, 20444761

DOI: 10.1039/d2cy00917j

Copy DOI

Catalysis

Abstract

In this study, CuO quantum dots were encapsulated in a MIL-125(Ti) MOF via a simple oxidation method. Upon loading of LiFePO4 the composite material LiFePO4/CuO@MIL-125(Ti) was formed. Due to the protection of the MIL-125(Ti) MOF, the composite photocatalyst exhibited stability in water. LiFePO4 provided transferable electrons to the CuO QDs which significantly improved the efficiency and selectivity of the photocatalytic CO2 reduction. Experiments showed that, at an optimal ratio of 2.5% LiFePO4/1.0% CuO@MIL-125(Ti), the photocatalyst had its highest photocatalytic reduction activity for CO2 conversion in the presence of water. The optimized photocatalyst gave yields of methanol, ethanol, and acetic acid of up to 445.38, 966.36, and 844.63 μmol g−1, respectively. This work delivered a robust route for embedding CuO QDs and lithium battery materials into the surface matrix of photocatalysts for the effective reduction of CO2.

Found

Top-30

Journals

	1
Applied Surface Science	Applied Surface Science, 1, 6.25% Applied Surface Science 1 publication, 6.25%
Inorganic Chemistry	Inorganic Chemistry, 1, 6.25% Inorganic Chemistry 1 publication, 6.25%
Nanoscale	Nanoscale, 1, 6.25% Nanoscale 1 publication, 6.25%
Journal of Industrial and Engineering Chemistry	Journal of Industrial and Engineering Chemistry, 1, 6.25% Journal of Industrial and Engineering Chemistry 1 publication, 6.25%
Molecular Catalysis	Molecular Catalysis, 1, 6.25% Molecular Catalysis 1 publication, 6.25%
Environmental Science and Pollution Research	Environmental Science and Pollution Research, 1, 6.25% Environmental Science and Pollution Research 1 publication, 6.25%
Russian Chemical Reviews	Russian Chemical Reviews, 1, 6.25% Russian Chemical Reviews 1 publication, 6.25%
Angewandte Chemie	Angewandte Chemie, 1, 6.25% Angewandte Chemie 1 publication, 6.25%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 1, 6.25% Angewandte Chemie - International Edition 1 publication, 6.25%
Batteries	Batteries, 1, 6.25% Batteries 1 publication, 6.25%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 1, 6.25% Coordination Chemistry Reviews 1 publication, 6.25%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 1, 6.25% Journal of Materials Chemistry A 1 publication, 6.25%
Green Chemistry	Green Chemistry, 1, 6.25% Green Chemistry 1 publication, 6.25%
Waste Management	Waste Management, 1, 6.25% Waste Management 1 publication, 6.25%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 1, 6.25% Journal of Alloys and Compounds 1 publication, 6.25%
	1

Publishers

	1 2 3 4 5
Elsevier	Elsevier, 5, 31.25% Elsevier 5 publications, 31.25%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 3, 18.75% Royal Society of Chemistry (RSC) 3 publications, 18.75%
Wiley	Wiley, 2, 12.5% Wiley 2 publications, 12.5%
American Chemical Society (ACS)	American Chemical Society (ACS), 1, 6.25% American Chemical Society (ACS) 1 publication, 6.25%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 6.25% Korean Society of Industrial Engineering Chemistry 1 publication, 6.25%
Springer Nature	Springer Nature, 1, 6.25% Springer Nature 1 publication, 6.25%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 6.25% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 6.25%
IntechOpen	IntechOpen, 1, 6.25% IntechOpen 1 publication, 6.25%
MDPI	MDPI, 1, 6.25% MDPI 1 publication, 6.25%
	1 2 3 4 5

We do not take into account publications without a DOI.
Statistics recalculated weekly.

Are you a researcher?

Create a profile to get free access to personal recommendations for colleagues and new articles.

Metrics

Cite this

GOST |

Cite this

GOST Copy

Zhou J. et al. Highly efficient and selective photocatalytic CO2 reduction using MIL-125(Ti) and based on LiFePO4 and CuO QDs surface–interface regulation // Catalysis Science and Technology. 2022. Vol. 12. No. 16. pp. 5152-5161.

GOST all authors (up to 50) Copy

Zhou J., Jia Q., Wang L., Zhao Y., Ma X., Gong L., Zhang H., ZUO T. Highly efficient and selective photocatalytic CO2 reduction using MIL-125(Ti) and based on LiFePO4 and CuO QDs surface–interface regulation // Catalysis Science and Technology. 2022. Vol. 12. No. 16. pp. 5152-5161.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1039/d2cy00917j

UR - https://xlink.rsc.org/?DOI=D2CY00917J

TI - Highly efficient and selective photocatalytic CO2 reduction using MIL-125(Ti) and based on LiFePO4 and CuO QDs surface–interface regulation

T2 - Catalysis Science and Technology

AU - Zhou, Jun

AU - Jia, Qinwei

AU - Wang, Luyu

AU - Zhao, Yuhang

AU - Ma, Xiaofan

AU - Gong, Lei

AU - Zhang, Haonan

AU - ZUO, Tong

PY - 2022

DA - 2022/06/24

PB - Royal Society of Chemistry (RSC)

SP - 5152-5161

IS - 16

VL - 12

SN - 2044-4753

SN - 2044-4761

ER -

BibTex |

Cite this

BibTex (up to 50 authors) Copy

@article{2022_Zhou,

author = {Jun Zhou and Qinwei Jia and Luyu Wang and Yuhang Zhao and Xiaofan Ma and Lei Gong and Haonan Zhang and Tong ZUO},

title = {Highly efficient and selective photocatalytic CO2 reduction using MIL-125(Ti) and based on LiFePO4 and CuO QDs surface–interface regulation},

journal = {Catalysis Science and Technology},

year = {2022},

volume = {12},

publisher = {Royal Society of Chemistry (RSC)},

month = {jun},

url = {https://xlink.rsc.org/?DOI=D2CY00917J},

number = {16},

pages = {5152--5161},

doi = {10.1039/d2cy00917j}

}

MLA

Cite this

MLA Copy

Zhou, Jun, et al. “Highly efficient and selective photocatalytic CO2 reduction using MIL-125(Ti) and based on LiFePO4 and CuO QDs surface–interface regulation.” Catalysis Science and Technology, vol. 12, no. 16, Jun. 2022, pp. 5152-5161. https://xlink.rsc.org/?DOI=D2CY00917J.

Publisher

Royal Society of Chemistry (RSC)

Journal

Catalysis Science and Technology

scimago Q2

wos Q2

SJR

1.026

CiteScore

8.0

Impact factor

4.2

ISSN

20444753 (Print)

20444761 (Electronic)