Organic and Biomolecular Chemistry

, volume 20 , issue 44 , pages 8756-8760

Visible-light-mediated aerobic Ritter-type C–H amination of diarylmethanes using DDQ/tert-butyl nitrite

Tianci Li ¹

Jiangyu Yang ^{1, 2}

Xin Yin ^{1, 2}

Jinhua Shi ¹

Qun Cao ³

Miaomiao Hu ¹

Xiaowen Xu ¹

Meichao Li ¹

Zhenlu Shen ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

College of Chemical Engineering, Zhejiang University of Technology, Hangzhou, 310014, China |

Zhejiang Jitai New Materials Co., Ltd, Shaoxing 312369, China |

School of Chemistry and Chemical Engineering, Queen's University Belfast, David Keir Building, Belfast, BT9 5AG, UK |

Publication type: Journal Article

Publication date: 2022-10-25

Royal Society of Chemistry (RSC)

Organic and Biomolecular Chemistry

scimago Q2

wos Q2

SJR: 0.600

CiteScore: 5.2

Impact factor: 2.7

ISSN: 14770520, 14770539

DOI: 10.1039/d2ob01713j

Copy DOI

PubMed ID: 36314247

Organic Chemistry

Biochemistry

Physical and Theoretical Chemistry

Abstract

A metal-free photocatalytic Ritter-type C–H amination of unactivated sp3 carbons using molecular oxygen as a terminal oxidant has been developed. By employing a co-catalytic system of 3-dichloro-4,5-dicyano-1,4-benzoquinone (DDQ) and tert-butyl nitrite (TBN), this novel strategy provides a low cost, sustainable and scalable way to synthesise a broad range of secondary amides in moderate to excellent yields under mild conditions.

Found

1 citation

Budnikova Yulia

DSc in Chemistry, professor

259 publications, 4 512 citations, 54 reviews

h-index: 34

A.E. Arbuzov Institute of Organic and Physical Chemistry of the Kazan Scientific Center of the Russian Academy of Sciences

Kazan Scientific Center of the Russian Academy of Sciences

Research interests

C-H functionalization

Catalysis

Charge transfer

Chemistry of organoelement compounds

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GOST |

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GOST Copy

Li T. et al. Visible-light-mediated aerobic Ritter-type C–H amination of diarylmethanes using DDQ/tert-butyl nitrite // Organic and Biomolecular Chemistry. 2022. Vol. 20. No. 44. pp. 8756-8760.

GOST all authors (up to 50) Copy

Li T., Yang J., Yin X., Shi J., Cao Q., Hu M., Xu X., Li M., Shen Z. Visible-light-mediated aerobic Ritter-type C–H amination of diarylmethanes using DDQ/tert-butyl nitrite // Organic and Biomolecular Chemistry. 2022. Vol. 20. No. 44. pp. 8756-8760.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1039/d2ob01713j

UR - https://xlink.rsc.org/?DOI=D2OB01713J

TI - Visible-light-mediated aerobic Ritter-type C–H amination of diarylmethanes using DDQ/tert-butyl nitrite

T2 - Organic and Biomolecular Chemistry

AU - Li, Tianci

AU - Yang, Jiangyu

AU - Yin, Xin

AU - Shi, Jinhua

AU - Cao, Qun

AU - Hu, Miaomiao

AU - Xu, Xiaowen

AU - Li, Meichao

AU - Shen, Zhenlu

PY - 2022

DA - 2022/10/25

PB - Royal Society of Chemistry (RSC)

SP - 8756-8760

IS - 44

VL - 20

PMID - 36314247

SN - 1477-0520

SN - 1477-0539

ER -

BibTex |

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BibTex (up to 50 authors) Copy

@article{2022_Li,

author = {Tianci Li and Jiangyu Yang and Xin Yin and Jinhua Shi and Qun Cao and Miaomiao Hu and Xiaowen Xu and Meichao Li and Zhenlu Shen},

title = {Visible-light-mediated aerobic Ritter-type C–H amination of diarylmethanes using DDQ/tert-butyl nitrite},

journal = {Organic and Biomolecular Chemistry},

year = {2022},

volume = {20},

publisher = {Royal Society of Chemistry (RSC)},

month = {oct},

url = {https://xlink.rsc.org/?DOI=D2OB01713J},

number = {44},

pages = {8756--8760},

doi = {10.1039/d2ob01713j}

}

MLA

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MLA Copy

Li, Tianci, et al. “Visible-light-mediated aerobic Ritter-type C–H amination of diarylmethanes using DDQ/tert-butyl nitrite.” Organic and Biomolecular Chemistry, vol. 20, no. 44, Oct. 2022, pp. 8756-8760. https://xlink.rsc.org/?DOI=D2OB01713J.

Publisher

Royal Society of Chemistry (RSC)

Journal

Organic and Biomolecular Chemistry

scimago Q2

wos Q2

SJR

0.600

CiteScore

5.2

Impact factor

2.7

ISSN

14770520 (Print)

14770539 (Electronic)