Physical Chemistry Chemical Physics, volume 16, issue 19, pages 8751

Thermodynamic and kinetic analysis of heterogeneous photocatalysis for semiconductor systems

Baoshun Liu ¹

Xiujian Zhao ¹

Chiaki Terashima ^{2, 3}

Akira Fujishima ²

K. Nakata ^{2, 3}

Hide authors affiliations Show authors affiliations: 3 affiliations

State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology, Luoshi road 122, Wuhan, Hubei, P. R. China |

Research Institute for Science and Technology, Energy and Environment Photocatalyst Research Division, Tokyo University of Science, 1-3 Kagurazaka, Shinjuku-ku, Tokyo 162-8601, Japan |

Department of Applied Biological Science, Faculty of Science and Technology, Tokyo University of Science, 2641 Yamazaki, Noda, Chiba 278-8510, Japan |

Publication type: Journal Article

Publication date: 2014-03-28

Royal Society of Chemistry (RSC)

Journal: Physical Chemistry Chemical Physics

Quartile SCImago

Quartile WOS

Impact factor: 3.3

ISSN: 14639076, 14639084

DOI: 10.1039/c3cp55317e

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Physical and Theoretical Chemistry

General Physics and Astronomy

Abstract

Since the report of the Honda-Fujishima effect, heterogeneous photocatalysis has attracted much attention around the world because of its potential energy and environmental applications. Although great progresses have been made in recent years, most were focused on preparing highly-active photocatalysts and investigating visible light utilization. In fact, we are still unclear on the thermodynamic and kinetic nature of photocatalysis to date, which sometimes leads to misunderstandings for experimental results. It is timely to give a review and discussion on the thermodynamics and kinetics of photocatalysis, so as to direct future researches. However, there is an absence of a detailed review on this topic until now. In this article, we tried to review and discuss the thermodynamics and kinetics of photocatalysis. We explained the thermodynamic driving force of photocatalysis, and distinguished the functions of light and heat in photocatalysis. The Langmuir-Hinshelwood kinetic model, the ˙OH oxidation mechanism, and the direct-indirect (D-I) kinetic model were reviewed and compared. Some applications of the D-I model to study photocatalytic kinetics were also discussed. The electron transport mode and its importance in photocatalysis were investigated. Finally, the intrinsic relation between the kinetics and the thermodynamics of photocatalytic reactions was discussed.

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Citations by journals

	2 4 6 8 10 12
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International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 8, 3.48% International Journal of Hydrogen Energy 8 publications, 3.48%
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Journal of Physical Chemistry C	Journal of Physical Chemistry C, 7, 3.04% Journal of Physical Chemistry C 7 publications, 3.04%
Chemosphere	Chemosphere, 6, 2.61% Chemosphere 6 publications, 2.61%
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Chemical Engineering Journal	Chemical Engineering Journal, 5, 2.17% Chemical Engineering Journal 5 publications, 2.17%
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Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 4, 1.74% Applied Catalysis B: Environmental 4 publications, 1.74%
Journal of Photochemistry and Photobiology A: Chemistry	Journal of Photochemistry and Photobiology A: Chemistry, 4, 1.74% Journal of Photochemistry and Photobiology A: Chemistry 4 publications, 1.74%
Nanomaterials	Nanomaterials, 3, 1.3% Nanomaterials 3 publications, 1.3%
Journal of Sol-Gel Science and Technology	Journal of Sol-Gel Science and Technology, 3, 1.3% Journal of Sol-Gel Science and Technology 3 publications, 1.3%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 3, 1.3% Journal of Materials Science: Materials in Electronics 3 publications, 1.3%
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Ceramics International	Ceramics International, 3, 1.3% Ceramics International 3 publications, 1.3%
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Chinese Journal of Catalysis	Chinese Journal of Catalysis, 3, 1.3% Chinese Journal of Catalysis 3 publications, 1.3%
Catalysis Today	Catalysis Today, 3, 1.3% Catalysis Today 3 publications, 1.3%
ACS Applied Nano Materials	ACS Applied Nano Materials, 3, 1.3% ACS Applied Nano Materials 3 publications, 1.3%
Catalysis Science and Technology	Catalysis Science and Technology, 3, 1.3% Catalysis Science and Technology 3 publications, 1.3%
Journal of Applied Physics	Journal of Applied Physics, 2, 0.87% Journal of Applied Physics 2 publications, 0.87%
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Sustainability	Sustainability, 2, 0.87% Sustainability 2 publications, 0.87%
Coordination Chemistry Reviews	Coordination Chemistry Reviews, 2, 0.87% Coordination Chemistry Reviews 2 publications, 0.87%
Journal of Environmental Management	Journal of Environmental Management, 2, 0.87% Journal of Environmental Management 2 publications, 0.87%
Nanotechnology	Nanotechnology, 2, 0.87% Nanotechnology 2 publications, 0.87%
Journal of CO2 Utilization	Journal of CO2 Utilization, 2, 0.87% Journal of CO2 Utilization 2 publications, 0.87%
	2 4 6 8 10 12

Citations by publishers

	10 20 30 40 50 60 70 80 90 100
Elsevier	Elsevier, 95, 41.3% Elsevier 95 publications, 41.3%
Springer Nature	Springer Nature, 30, 13.04% Springer Nature 30 publications, 13.04%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 23, 10% Royal Society of Chemistry (RSC) 23 publications, 10%
American Chemical Society (ACS)	American Chemical Society (ACS), 19, 8.26% American Chemical Society (ACS) 19 publications, 8.26%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 17, 7.39% Multidisciplinary Digital Publishing Institute (MDPI) 17 publications, 7.39%
Wiley	Wiley, 11, 4.78% Wiley 11 publications, 4.78%
IOP Publishing	IOP Publishing, 5, 2.17% IOP Publishing 5 publications, 2.17%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 4, 1.74% American Institute of Physics (AIP) 4 publications, 1.74%
Frontiers Media S.A.	Frontiers Media S.A., 2, 0.87% Frontiers Media S.A. 2 publications, 0.87%
Hindawi Limited	Hindawi Limited, 1, 0.43% Hindawi Limited 1 publication, 0.43%
Copernicus	Copernicus, 1, 0.43% Copernicus 1 publication, 0.43%
The Royal Society	The Royal Society, 1, 0.43% The Royal Society 1 publication, 0.43%
World Scientific	World Scientific, 1, 0.43% World Scientific 1 publication, 0.43%
The Electrochemical Society	The Electrochemical Society, 1, 0.43% The Electrochemical Society 1 publication, 0.43%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.43% Taiwan Institute of Chemical Engineers 1 publication, 0.43%
Chinese Society of Rare Earths	Chinese Society of Rare Earths, 1, 0.43% Chinese Society of Rare Earths 1 publication, 0.43%
Chinese Ceramic Society	Chinese Ceramic Society, 1, 0.43% Chinese Ceramic Society 1 publication, 0.43%
Taylor & Francis	Taylor & Francis, 1, 0.43% Taylor & Francis 1 publication, 0.43%
Heighten Science Publications Corporation	Heighten Science Publications Corporation, 1, 0.43% Heighten Science Publications Corporation 1 publication, 0.43%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.43% American Association for the Advancement of Science (AAAS) 1 publication, 0.43%
Materials Research Society of Korea	Materials Research Society of Korea, 1, 0.43% Materials Research Society of Korea 1 publication, 0.43%
Trans Tech Publications	Trans Tech Publications, 1, 0.43% Trans Tech Publications 1 publication, 0.43%
American Vacuum Society	American Vacuum Society, 1, 0.43% American Vacuum Society 1 publication, 0.43%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.43% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.43%
	10 20 30 40 50 60 70 80 90 100

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Liu B. et al. Thermodynamic and kinetic analysis of heterogeneous photocatalysis for semiconductor systems // Physical Chemistry Chemical Physics. 2014. Vol. 16. No. 19. p. 8751.

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Liu B., Zhao X., Terashima C., Fujishima A., Nakata K. Thermodynamic and kinetic analysis of heterogeneous photocatalysis for semiconductor systems // Physical Chemistry Chemical Physics. 2014. Vol. 16. No. 19. p. 8751.

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TY - JOUR

DO - 10.1039/c3cp55317e

UR - https://doi.org/10.1039/c3cp55317e

TI - Thermodynamic and kinetic analysis of heterogeneous photocatalysis for semiconductor systems

T2 - Physical Chemistry Chemical Physics

AU - Fujishima, Akira

AU - Liu, Baoshun

AU - Zhao, Xiujian

AU - Terashima, Chiaki

AU - Nakata, K.

PY - 2014

DA - 2014/03/28 00:00:00

PB - Royal Society of Chemistry (RSC)

SP - 8751

IS - 19

VL - 16

SN - 1463-9076

SN - 1463-9084

ER -

BibTex |

Cite this

BibTex Copy

@article{2014_Liu,

author = {Akira Fujishima and Baoshun Liu and Xiujian Zhao and Chiaki Terashima and K. Nakata},

title = {Thermodynamic and kinetic analysis of heterogeneous photocatalysis for semiconductor systems},

journal = {Physical Chemistry Chemical Physics},

year = {2014},

volume = {16},

publisher = {Royal Society of Chemistry (RSC)},

month = {mar},

url = {https://doi.org/10.1039/c3cp55317e},

number = {19},

pages = {8751},

doi = {10.1039/c3cp55317e}

}

MLA

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MLA Copy

Liu, Baoshun, et al. “Thermodynamic and kinetic analysis of heterogeneous photocatalysis for semiconductor systems.” Physical Chemistry Chemical Physics, vol. 16, no. 19, Mar. 2014, p. 8751. https://doi.org/10.1039/c3cp55317e.

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Publisher

Royal Society of Chemistry (RSC)

Journal

Physical Chemistry Chemical Physics

Quartile SCImago

Quartile WOS

Impact factor

3.3

ISSN

14639076 (Print)
14639084 (Electronic)

Profiles

Terashima, Chiaki