Effects of solvents, additives, and π-allyl ligand structures on the polymerization behavior of diazoacetates initiated by π-allylPd complexes
Hiroaki Shimomoto
1, 2, 3, 4, 5, 6
,
Moemi Nakajima
1, 2, 3, 4, 5, 6
,
Akihiro Watanabe
1, 2, 3, 4, 5, 6
,
Hirokazu Murakami
1, 2, 3, 4, 5, 6
,
Tomomichi Itoh
1, 2, 3, 4, 5, 6
,
Eiji Ihara
1, 2, 3, 4, 5, 6
2
Department of Materials Science and Biotechnology
3
Graduate school of science and engineering
5
Matsuyama 790-8577
|
6
JAPAN
|
Publication type: Journal Article
Publication date: 2020-01-22
scimago Q1
wos Q2
SJR: 0.842
CiteScore: 7.6
Impact factor: 3.9
ISSN: 17599954, 17599962
Organic Chemistry
Biochemistry
Polymers and Plastics
Bioengineering
Abstract
In the polymerization of diazoacetates initiated by π-allylPd-based initiating systems, the effects of solvents, additives, and π-allyl ligand structures on the polymerization behavior were investigated. As a result, the polymerization in the presence of pyridine or its derivatives as an additive was found to afford a polymer with relatively narrow molecular weight distribution compared to that with π-allylPdCl alone. Furthermore, we have demonstrated that Pd complexes with π-allyl ligands with a variety of substituents are capable of polymerizing diazoacetates in a similar manner to the parent unsubstituted π-allylPdCl, and the tacticity of the resulting polymers is affected by the structure of the π-allyl ligands.
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17
Total citations:
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Citations from 2025:
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(25%)
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Shimomoto H. et al. Effects of solvents, additives, and π-allyl ligand structures on the polymerization behavior of diazoacetates initiated by π-allylPd complexes // Polymer Chemistry. 2020. Vol. 11. No. 10. pp. 1774-1784.
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Shimomoto H., Nakajima M., Watanabe A., Murakami H., Itoh T., Ihara E. Effects of solvents, additives, and π-allyl ligand structures on the polymerization behavior of diazoacetates initiated by π-allylPd complexes // Polymer Chemistry. 2020. Vol. 11. No. 10. pp. 1774-1784.
Cite this
RIS
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TY - JOUR
DO - 10.1039/c9py01654f
UR - https://xlink.rsc.org/?DOI=C9PY01654F
TI - Effects of solvents, additives, and π-allyl ligand structures on the polymerization behavior of diazoacetates initiated by π-allylPd complexes
T2 - Polymer Chemistry
AU - Shimomoto, Hiroaki
AU - Nakajima, Moemi
AU - Watanabe, Akihiro
AU - Murakami, Hirokazu
AU - Itoh, Tomomichi
AU - Ihara, Eiji
PY - 2020
DA - 2020/01/22
PB - Royal Society of Chemistry (RSC)
SP - 1774-1784
IS - 10
VL - 11
SN - 1759-9954
SN - 1759-9962
ER -
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BibTex (up to 50 authors)
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@article{2020_Shimomoto,
author = {Hiroaki Shimomoto and Moemi Nakajima and Akihiro Watanabe and Hirokazu Murakami and Tomomichi Itoh and Eiji Ihara},
title = {Effects of solvents, additives, and π-allyl ligand structures on the polymerization behavior of diazoacetates initiated by π-allylPd complexes},
journal = {Polymer Chemistry},
year = {2020},
volume = {11},
publisher = {Royal Society of Chemistry (RSC)},
month = {jan},
url = {https://xlink.rsc.org/?DOI=C9PY01654F},
number = {10},
pages = {1774--1784},
doi = {10.1039/c9py01654f}
}
Cite this
MLA
Copy
Shimomoto, Hiroaki, et al. “Effects of solvents, additives, and π-allyl ligand structures on the polymerization behavior of diazoacetates initiated by π-allylPd complexes.” Polymer Chemistry, vol. 11, no. 10, Jan. 2020, pp. 1774-1784. https://xlink.rsc.org/?DOI=C9PY01654F.