Selective direct C–H polyfluoroarylation of electron-deficient N-heterocyclic compounds
Shun Li
1, 2, 3, 4, 5, 6
,
Wen-Jing Li
1, 2, 3, 4, 5, 6
,
Xiao Yang
1
,
Rui Sun
1, 2, 3, 4, 5, 6
,
Juan Tang
1, 2, 3, 4, 5, 6
,
Xueli Zheng
1, 2, 3, 4, 5, 6
,
Mao Ling Yuan
1
,
Mao-Ling Yuan
1, 2, 3, 4, 5, 6
,
Ruixiang Li
1, 2, 3, 4, 5, 6
,
Hua Chen
1
,
Haiyan Fu
1, 2, 3, 4, 5, 6
2
Key Laboratory of Green Chemistry & Technology
3
Ministry of Education College of Chemistry
5
Chengdu 610064
|
6
P. R. China
|
Тип публикации: Journal Article
Дата публикации: 2020-10-12
scimago Q1
wos Q1
БС1
SJR: 1.068
CiteScore: 8.2
Impact factor: 4.7
ISSN: 20524110, 20524129
Organic Chemistry
Краткое описание
The first C2-selective direct C–H polyfluoroarylation of electron-deficient N-heterocycles with polyfluorobenzoic acid via the decarboxylative arylation process was achieved by using CuBr2 as the mediator in the green solvent diglyme. The key to success is using the N-methylation activation strategy and TBAB as an important additive. The protocol features broad substrate scope, ligand- and base-free conditions, and good functional group compatibility, and offers a powerful synthetic tool for assembling various polyfluoroarylated N-heterocycles.
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Li S. et al. Selective direct C–H polyfluoroarylation of electron-deficient N-heterocyclic compounds // Organic Chemistry Frontiers. 2020. Vol. 7. No. 23. pp. 3887-3895.
ГОСТ со всеми авторами (до 50)
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Li S. et al. Selective direct C–H polyfluoroarylation of electron-deficient N-heterocyclic compounds // Organic Chemistry Frontiers. 2020. Vol. 7. No. 23. pp. 3887-3895.
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TY - JOUR
DO - 10.1039/d0qo00923g
UR - https://xlink.rsc.org/?DOI=D0QO00923G
TI - Selective direct C–H polyfluoroarylation of electron-deficient N-heterocyclic compounds
T2 - Organic Chemistry Frontiers
AU - Li, Shun
AU - Li, Wen-Jing
AU - Yang, Xiao
AU - Sun, Rui
AU - Tang, Juan
AU - Zheng, Xueli
AU - Yuan, Mao Ling
AU - Yuan, Mao-Ling
AU - Li, Ruixiang
AU - Chen, Hua
AU - Fu, Haiyan
PY - 2020
DA - 2020/10/12
PB - Royal Society of Chemistry (RSC)
SP - 3887-3895
IS - 23
VL - 7
SN - 2052-4110
SN - 2052-4129
ER -
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@article{2020_Li,
author = {Shun Li and Wen-Jing Li and Xiao Yang and Rui Sun and Juan Tang and Xueli Zheng and Mao Ling Yuan and Mao-Ling Yuan and Ruixiang Li and Hua Chen and Haiyan Fu and others},
title = {Selective direct C–H polyfluoroarylation of electron-deficient N-heterocyclic compounds},
journal = {Organic Chemistry Frontiers},
year = {2020},
volume = {7},
publisher = {Royal Society of Chemistry (RSC)},
month = {oct},
url = {https://xlink.rsc.org/?DOI=D0QO00923G},
number = {23},
pages = {3887--3895},
doi = {10.1039/d0qo00923g}
}
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MLA
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Li, Shun, et al. “Selective direct C–H polyfluoroarylation of electron-deficient N-heterocyclic compounds.” Organic Chemistry Frontiers, vol. 7, no. 23, Oct. 2020, pp. 3887-3895. https://xlink.rsc.org/?DOI=D0QO00923G.