Open Access
The impact of alicyclic substituents on the extraction ability of new family of 1,10-phenanthroline-2,9-diamides
Pavel S. Lemport
1, 2, 3, 4, 5
,
Petr I Matveev
1, 2, 3, 4, 5
,
Alexandr Yatsenko
1, 2, 3, 4, 5
,
M V Evsiunina
1, 2, 3, 4, 5
,
Valentine S Petrov
1, 2, 3, 4, 5
,
B.N. Tarasevich
1, 2, 3, 4, 5
,
Vitaly A Roznyatovsky
1, 2, 3, 4, 5
,
Pavel Dorovatovskii
5, 6, 7
,
Victor N. Khrustalev
5, 8, 9, 10, 11, 12
,
Sergey S Zhokhov
1, 2, 3, 4, 5
,
V. Solov'ev
5, 13, 14, 15
,
Leonid A. Aslanov
1, 2, 3, 4, 5
,
Vladimir G Petrov
1, 2, 3, 4, 5
,
Valentine G. Nenajdenko
1, 2, 3, 4, 5
,
Yu.A. Ustynyuk
1, 2, 3, 4, 5
2
Chemistry department
4
Moscow
5
Russia
|
10
Department of Inorganic Chemistry
13
15
RUSSIAN ACADEMY OF SCIENCES
Publication type: Journal Article
Publication date: 2020-07-10
scimago Q1
wos Q2
SJR: 0.777
CiteScore: 7.6
Impact factor: 4.6
ISSN: 20462069
PubMed ID:
35519740
General Chemistry
General Chemical Engineering
Abstract
Development of efficient extractants for the separation of actinides and lanthanides in the technologies of nuclear fuel cycle is one of the most urgent and complex tasks in modern nuclear energetics. New family of 4,7-dichloro-1,10-phenanthroline-2,9-dicarboxylic acid diamides based on cyclic amines was synthesized and shown to exhibit high selectivity in the La/Am pair separation (SF (Am/La ≈ 10)) and in the Am/Eu pair separation (SF (Am/Eu ≈ 12)). It was shown that pyrrolidine derived diamide is more efficient extractant for americium, curium and lanthanides from highly acidic HNO3 solution than its non-cyclic N,N,N',N'-tetraalkyl analogues. The structures of synthesized compounds were studied in details by IR, NMR spectroscopy, and single crystal X-ray diffraction. According to spectroscopy data, incorporation of aromatic rings to the amide fragment of ligand leads to complex dynamic behavior in solutions what is believed to strongly affect the extraction ability of synthesized ligands.
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Total citations:
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Citations from 2024:
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(42%)
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GOST
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Lemport P. S. et al. The impact of alicyclic substituents on the extraction ability of new family of 1,10-phenanthroline-2,9-diamides // RSC Advances. 2020. Vol. 10. No. 44. pp. 26022-26033.
GOST all authors (up to 50)
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Lemport P. S. et al. The impact of alicyclic substituents on the extraction ability of new family of 1,10-phenanthroline-2,9-diamides // RSC Advances. 2020. Vol. 10. No. 44. pp. 26022-26033.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1039/d0ra05182a
UR - https://xlink.rsc.org/?DOI=D0RA05182A
TI - The impact of alicyclic substituents on the extraction ability of new family of 1,10-phenanthroline-2,9-diamides
T2 - RSC Advances
AU - Lemport, Pavel S.
AU - Matveev, Petr I
AU - Yatsenko, Alexandr
AU - Evsiunina, M V
AU - Petrov, Valentine S
AU - Tarasevich, B.N.
AU - Roznyatovsky, Vitaly A
AU - Dorovatovskii, Pavel
AU - Khrustalev, Victor N.
AU - Zhokhov, Sergey S
AU - Solov'ev, V.
AU - Aslanov, Leonid A.
AU - Petrov, Vladimir G
AU - Kalmykov, Stepan N.
AU - Nenajdenko, Valentine G.
AU - Ustynyuk, Yu.A.
PY - 2020
DA - 2020/07/10
PB - Royal Society of Chemistry (RSC)
SP - 26022-26033
IS - 44
VL - 10
PMID - 35519740
SN - 2046-2069
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2020_Lemport,
author = {Pavel S. Lemport and Petr I Matveev and Alexandr Yatsenko and M V Evsiunina and Valentine S Petrov and B.N. Tarasevich and Vitaly A Roznyatovsky and Pavel Dorovatovskii and Victor N. Khrustalev and Sergey S Zhokhov and V. Solov'ev and Leonid A. Aslanov and Vladimir G Petrov and Stepan N. Kalmykov and Valentine G. Nenajdenko and Yu.A. Ustynyuk and others},
title = {The impact of alicyclic substituents on the extraction ability of new family of 1,10-phenanthroline-2,9-diamides},
journal = {RSC Advances},
year = {2020},
volume = {10},
publisher = {Royal Society of Chemistry (RSC)},
month = {jul},
url = {https://xlink.rsc.org/?DOI=D0RA05182A},
number = {44},
pages = {26022--26033},
doi = {10.1039/d0ra05182a}
}
Cite this
MLA
Copy
Lemport, Pavel S., et al. “The impact of alicyclic substituents on the extraction ability of new family of 1,10-phenanthroline-2,9-diamides.” RSC Advances, vol. 10, no. 44, Jul. 2020, pp. 26022-26033. https://xlink.rsc.org/?DOI=D0RA05182A.