Hydrogenation and Dehydrogenation of N-Heterocycles Under Cp*Co(III)-Catalysis
Publication type: Journal Article
Publication date: 2023-10-02
scimago Q2
wos Q1
SJR: 0.653
CiteScore: 6.0
Impact factor: 3.3
ISSN: 14779226, 14779234
PubMed ID:
37814805
Inorganic Chemistry
Abstract
To realize the goal of a carbon-free energy economy, it is crucial to discover reactions that utilize sustainable resources as alternatives to fossil feedstocks. In this study, a well-defined, air-stable Cp*Co(III)-catalyst for transfer hydrogenation of quinoline derivatives and oxidative dehydrogenation of cyclic amines in water is developed. While the former reaction is promoted by formic acid as a transfer hydrogenation reagent, the latter is mediated by molecular oxygen as the sole oxidant. These processes provide new avenues for the investigation of air-stable cobalt catalysts for environmentally benign hydrogenation and dehydrogenation reactions.
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Dahiya P. et al. Hydrogenation and Dehydrogenation of N-Heterocycles Under Cp*Co(III)-Catalysis // Dalton Transactions. 2023. Vol. 52. No. 41. pp. 14752-14756.
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Dahiya P., Garg N., Poli R., Sundararaju B. Hydrogenation and Dehydrogenation of N-Heterocycles Under Cp*Co(III)-Catalysis // Dalton Transactions. 2023. Vol. 52. No. 41. pp. 14752-14756.
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RIS
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TY - JOUR
DO - 10.1039/d3dt03161f
UR - https://xlink.rsc.org/?DOI=D3DT03161F
TI - Hydrogenation and Dehydrogenation of N-Heterocycles Under Cp*Co(III)-Catalysis
T2 - Dalton Transactions
AU - Dahiya, Pardeep
AU - Garg, Nidhi
AU - Poli, Rinaldo
AU - Sundararaju, Basker
PY - 2023
DA - 2023/10/02
PB - Royal Society of Chemistry (RSC)
SP - 14752-14756
IS - 41
VL - 52
PMID - 37814805
SN - 1477-9226
SN - 1477-9234
ER -
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BibTex (up to 50 authors)
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@article{2023_Dahiya,
author = {Pardeep Dahiya and Nidhi Garg and Rinaldo Poli and Basker Sundararaju},
title = {Hydrogenation and Dehydrogenation of N-Heterocycles Under Cp*Co(III)-Catalysis},
journal = {Dalton Transactions},
year = {2023},
volume = {52},
publisher = {Royal Society of Chemistry (RSC)},
month = {oct},
url = {https://xlink.rsc.org/?DOI=D3DT03161F},
number = {41},
pages = {14752--14756},
doi = {10.1039/d3dt03161f}
}
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MLA
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Dahiya, Pardeep, et al. “Hydrogenation and Dehydrogenation of N-Heterocycles Under Cp*Co(III)-Catalysis.” Dalton Transactions, vol. 52, no. 41, Oct. 2023, pp. 14752-14756. https://xlink.rsc.org/?DOI=D3DT03161F.
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