volume 53 issue 13 pages 2253-2259

Synthesis of Substituted β-Styrylmalonates by Sequential Isomerization of 2-Arylcyclopropane-1,1-dicarboxylates and (2-Arylethylidene)malonates

Publication typeJournal Article
Publication date2021-01-08
scimago Q2
wos Q2
SJR0.559
CiteScore4.6
Impact factor2.3
ISSN00397881, 1437210X
Catalysis
Organic Chemistry
Abstract

A method has been developed for the synthesis of substituted β-styrylmalonates by conversion of 2-arylcyclopropane-1,1-dicarboxylates (ACDCs) in the presence of gallium trichloride into the corresponding­ 1,2-zwitterionic intermediates or (2-arylethyl­idene)malonates, followed by treatment with pyridine at room temperature leading to an isomerization of the emerging double bond. This method allows one to expand these reactions to include ACDCs with acceptor substituents at the aromatic ring.

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Novikov R. A. et al. Synthesis of Substituted β-Styrylmalonates by Sequential Isomerization of 2-Arylcyclopropane-1,1-dicarboxylates and (2-Arylethylidene)malonates // Synthesis. 2021. Vol. 53. No. 13. pp. 2253-2259.
GOST all authors (up to 50) Copy
Novikov R. A., Tomilov Y. V., Borisov D. D., Chermashentsev G. R. Synthesis of Substituted β-Styrylmalonates by Sequential Isomerization of 2-Arylcyclopropane-1,1-dicarboxylates and (2-Arylethylidene)malonates // Synthesis. 2021. Vol. 53. No. 13. pp. 2253-2259.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1055/a-1348-4311
UR - https://doi.org/10.1055/a-1348-4311
TI - Synthesis of Substituted β-Styrylmalonates by Sequential Isomerization of 2-Arylcyclopropane-1,1-dicarboxylates and (2-Arylethylidene)malonates
T2 - Synthesis
AU - Novikov, Roman A
AU - Tomilov, Yury V
AU - Borisov, Denis D
AU - Chermashentsev, Grigorii R
PY - 2021
DA - 2021/01/08
PB - Georg Thieme Verlag KG
SP - 2253-2259
IS - 13
VL - 53
SN - 0039-7881
SN - 1437-210X
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2021_Novikov,
author = {Roman A Novikov and Yury V Tomilov and Denis D Borisov and Grigorii R Chermashentsev},
title = {Synthesis of Substituted β-Styrylmalonates by Sequential Isomerization of 2-Arylcyclopropane-1,1-dicarboxylates and (2-Arylethylidene)malonates},
journal = {Synthesis},
year = {2021},
volume = {53},
publisher = {Georg Thieme Verlag KG},
month = {jan},
url = {https://doi.org/10.1055/a-1348-4311},
number = {13},
pages = {2253--2259},
doi = {10.1055/a-1348-4311}
}
MLA
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MLA Copy
Novikov, Roman A., et al. “Synthesis of Substituted β-Styrylmalonates by Sequential Isomerization of 2-Arylcyclopropane-1,1-dicarboxylates and (2-Arylethylidene)malonates.” Synthesis, vol. 53, no. 13, Jan. 2021, pp. 2253-2259. https://doi.org/10.1055/a-1348-4311.