Electrochemical Benzylic C(sp3)−H Amidation via Ritter-type Reaction in the Absence of External Mediator and Oxidant
Publication type: Journal Article
Publication date: 2022-12-05
scimago Q2
wos Q2
SJR: 0.559
CiteScore: 4.6
Impact factor: 2.3
ISSN: 00397881, 1437210X
Catalysis
Organic Chemistry
Abstract
A straightforward method involving electrochemical Ritter-type amidation of alkylarenes in the absence of external mediator and oxidant is described. This direct benzylic C(sp3)–H amidation utilizes cheap CH3CN or other nitriles as the nitrogen source and trace amount of H2O in the solvent as the oxygen and hydrogen source. A wide range of alkylarenes were found to be compatible, providing a variety of N-benzyl-substituted amides in moderate to good yields.
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Total citations:
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Liu P. et al. Electrochemical Benzylic C(sp3)−H Amidation via Ritter-type Reaction in the Absence of External Mediator and Oxidant // Synthesis. 2022.
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Liu P., Sun P., Chu Q., Zhou Y., Ji C. Electrochemical Benzylic C(sp3)−H Amidation via Ritter-type Reaction in the Absence of External Mediator and Oxidant // Synthesis. 2022.
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TY - JOUR
DO - 10.1055/a-1992-7066
UR - https://doi.org/10.1055/a-1992-7066
TI - Electrochemical Benzylic C(sp3)−H Amidation via Ritter-type Reaction in the Absence of External Mediator and Oxidant
T2 - Synthesis
AU - Liu, Ping
AU - Sun, Peipei
AU - Chu, Qiao
AU - Zhou, Yeqin
AU - Ji, Ce
PY - 2022
DA - 2022/12/05
PB - Georg Thieme Verlag KG
SN - 0039-7881
SN - 1437-210X
ER -
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@article{2022_Liu,
author = {Ping Liu and Peipei Sun and Qiao Chu and Yeqin Zhou and Ce Ji},
title = {Electrochemical Benzylic C(sp3)−H Amidation via Ritter-type Reaction in the Absence of External Mediator and Oxidant},
journal = {Synthesis},
year = {2022},
publisher = {Georg Thieme Verlag KG},
month = {dec},
url = {https://doi.org/10.1055/a-1992-7066},
doi = {10.1055/a-1992-7066}
}