Translational and rotational dynamics of water in mesoporous silica materials: MCM-41-S and MCM-48-S
Тип публикации: Journal Article
Дата публикации: 2003-07-30
scimago Q1
wos Q2
БС2
SJR: 0.819
CiteScore: 5.3
Impact factor: 3.1
ISSN: 00219606, 10897690
Physical and Theoretical Chemistry
General Physics and Astronomy
Краткое описание
We investigated the translational and rotational dynamics of water molecules in mesoporous silica materials MCM-41-S and MCM-48-S using the incoherent quasielastic neutron scattering technique. The range of wave vector transfers Q covered in the measurements was from 0.27 to 1.93 Å−1 broad enough to detect both the translational and rotational contributions to the scattering. We used the relaxing-cage models for both translational and rotational motions which we developed earlier, to analyze the QENS spectra and investigated water dynamics in a supercooled range from 250 to 280 K. The results show a marked slowing down of both the translational and rotational relaxation times, and an increasing effect of confinement on the translational motion, as the temperature is lowered.
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ГОСТ
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Faraone A. et al. Translational and rotational dynamics of water in mesoporous silica materials: MCM-41-S and MCM-48-S // Journal of Chemical Physics. 2003. Vol. 119. No. 7. pp. 3963-3971.
ГОСТ со всеми авторами (до 50)
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Faraone A., Liu Li, Mou C., Shih P., Copley J. R. D., Chen S. Translational and rotational dynamics of water in mesoporous silica materials: MCM-41-S and MCM-48-S // Journal of Chemical Physics. 2003. Vol. 119. No. 7. pp. 3963-3971.
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TY - JOUR
DO - 10.1063/1.1584653
UR - https://doi.org/10.1063/1.1584653
TI - Translational and rotational dynamics of water in mesoporous silica materials: MCM-41-S and MCM-48-S
T2 - Journal of Chemical Physics
AU - Faraone, Antonio
AU - Liu Li
AU - Mou, Chung-Yuan
AU - Shih, Pei-Chun
AU - Copley, John R. D.
AU - Chen, Sow-Hsin
PY - 2003
DA - 2003/07/30
PB - AIP Publishing
SP - 3963-3971
IS - 7
VL - 119
SN - 0021-9606
SN - 1089-7690
ER -
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@article{2003_Faraone,
author = {Antonio Faraone and Liu Li and Chung-Yuan Mou and Pei-Chun Shih and John R. D. Copley and Sow-Hsin Chen},
title = {Translational and rotational dynamics of water in mesoporous silica materials: MCM-41-S and MCM-48-S},
journal = {Journal of Chemical Physics},
year = {2003},
volume = {119},
publisher = {AIP Publishing},
month = {jul},
url = {https://doi.org/10.1063/1.1584653},
number = {7},
pages = {3963--3971},
doi = {10.1063/1.1584653}
}
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MLA
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Faraone, Antonio, et al. “Translational and rotational dynamics of water in mesoporous silica materials: MCM-41-S and MCM-48-S.” Journal of Chemical Physics, vol. 119, no. 7, Jul. 2003, pp. 3963-3971. https://doi.org/10.1063/1.1584653.