volume 135 issue 10 pages 101103

Communication: Stabilization of radical anions with weakly bound electron in condensed media: A case study of diacetonyl radical anion

Publication typeJournal Article
Publication date2011-09-12
scimago Q1
wos Q2
SJR0.819
CiteScore5.3
Impact factor3.1
ISSN00219606, 10897690
PubMed ID:  21932869
Physical and Theoretical Chemistry
General Physics and Astronomy
Abstract

The radical anion resulting from electron capture by diacetonyl molecule has been characterized by EPR and optical absorption spectroscopy in glassy ether matrices at 77 K. In non-polar alkane glasses this species was not observed under the same conditions, which confirms the crucial role of matrix interactions in stabilizing this species. Calculations at the MP2 level show the vertical detachment energy to increase gradually from roughly zero for a bare anion to ∼1 eV for the complex involving six ether molecules.

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Saenko E. V. et al. Communication: Stabilization of radical anions with weakly bound electron in condensed media: A case study of diacetonyl radical anion // Journal of Chemical Physics. 2011. Vol. 135. No. 10. p. 101103.
GOST all authors (up to 50) Copy
Saenko E. V., Laikov D. N., Baranova I. A., Feldman V. I. Communication: Stabilization of radical anions with weakly bound electron in condensed media: A case study of diacetonyl radical anion // Journal of Chemical Physics. 2011. Vol. 135. No. 10. p. 101103.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1063/1.3638690
UR - https://pubs.aip.org/jcp/article/135/10/101103/983373/Communication-Stabilization-of-radical-anions-with
TI - Communication: Stabilization of radical anions with weakly bound electron in condensed media: A case study of diacetonyl radical anion
T2 - Journal of Chemical Physics
AU - Saenko, Elizaveta V
AU - Laikov, Dimitri N
AU - Baranova, Irina A
AU - Feldman, Vladimir I
PY - 2011
DA - 2011/09/12
PB - AIP Publishing
SP - 101103
IS - 10
VL - 135
PMID - 21932869
SN - 0021-9606
SN - 1089-7690
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2011_Saenko,
author = {Elizaveta V Saenko and Dimitri N Laikov and Irina A Baranova and Vladimir I Feldman},
title = {Communication: Stabilization of radical anions with weakly bound electron in condensed media: A case study of diacetonyl radical anion},
journal = {Journal of Chemical Physics},
year = {2011},
volume = {135},
publisher = {AIP Publishing},
month = {sep},
url = {https://pubs.aip.org/jcp/article/135/10/101103/983373/Communication-Stabilization-of-radical-anions-with},
number = {10},
pages = {101103},
doi = {10.1063/1.3638690}
}
MLA
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MLA Copy
Saenko, Elizaveta V., et al. “Communication: Stabilization of radical anions with weakly bound electron in condensed media: A case study of diacetonyl radical anion.” Journal of Chemical Physics, vol. 135, no. 10, Sep. 2011, p. 101103. https://pubs.aip.org/jcp/article/135/10/101103/983373/Communication-Stabilization-of-radical-anions-with.