Journal of Chemical Physics, volume 87, issue 12, pages 7315-7322
PbS in polymers. From molecules to bulk solids
1
E. I. du Pont de Nemours and Company, Central Research and Development Department Experimental Station, Wilmington, Deleware 19898
Publication type: Journal Article
Publication date: 1987-12-15
Journal:
Journal of Chemical Physics
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 4.4
ISSN: 00219606, 10897690
DOI:
10.1063/1.453325
Physical and Theoretical Chemistry
General Physics and Astronomy
Abstract
The transition of PbS from molecular to bulk form has been observed in polymer films. As the particle size decreases the band gap shifts to the blue and eventually approaches the transition energy of the first allowed excited state, X→A, of a PbS molecule. Discrete absorption bands also appear. The electron-hole-in-a-box model with effective mass approximation cannot explain the observed size dependence. We have developed two theoretical models, both including the effect of band nonparabolicity, that successfully explain the observed size dependence down to about 25 Å.
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Citations by publishers
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50
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Wang Y. et al. PbS in polymers. From molecules to bulk solids // Journal of Chemical Physics. 1987. Vol. 87. No. 12. pp. 7315-7322.
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Wang Y., Suna A., Mahler W., Kasowski R. PbS in polymers. From molecules to bulk solids // Journal of Chemical Physics. 1987. Vol. 87. No. 12. pp. 7315-7322.
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TY - JOUR
DO - 10.1063/1.453325
UR - https://doi.org/10.1063/1.453325
TI - PbS in polymers. From molecules to bulk solids
T2 - Journal of Chemical Physics
AU - Wang, Y.
AU - Suna, A.
AU - Mahler, W.
AU - Kasowski, R
PY - 1987
DA - 1987/12/15 00:00:00
PB - American Institute of Physics (AIP)
SP - 7315-7322
IS - 12
VL - 87
SN - 0021-9606
SN - 1089-7690
ER -
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@article{1987_Wang,
author = {Y. Wang and A. Suna and W. Mahler and R Kasowski},
title = {PbS in polymers. From molecules to bulk solids},
journal = {Journal of Chemical Physics},
year = {1987},
volume = {87},
publisher = {American Institute of Physics (AIP)},
month = {dec},
url = {https://doi.org/10.1063/1.453325},
number = {12},
pages = {7315--7322},
doi = {10.1063/1.453325}
}
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MLA
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Wang, Y., et al. “PbS in polymers. From molecules to bulk solids.” Journal of Chemical Physics, vol. 87, no. 12, Dec. 1987, pp. 7315-7322. https://doi.org/10.1063/1.453325.