Applied Physics Letters

, том 101 , издание 24 , страницы 241910

Site-specific mapping of transition metal oxygen coordination in complex oxides

S TURNER ¹

R Egoavil ¹

M Batuk ¹

A A Abakumov ¹

J. Hadermann ¹

J. Verbeeck ¹

G. Van Tendeloo ¹

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EMAT, Department of Physics, University of Antwerp , B-2020 Antwerp, Belgium |

Тип публикации: Journal Article

Дата публикации: 2012-12-10

AIP Publishing

Applied Physics Letters

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SJR: 0.896

CiteScore: 6.1

Impact factor: 3.6

ISSN: 00036951, 10773118

DOI: 10.1063/1.4770512

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Physics and Astronomy (miscellaneous)

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We demonstrate site-specific mapping of the oxygen coordination number for transition metals in complex oxides using atomically resolved electron energy-loss spectroscopy in an aberration-corrected scanning transmission electron microscope. Pb2Sr2Bi2Fe6O16 contains iron with a constant Fe3+ valency in both octahedral and tetragonal pyramidal coordination and is selected to demonstrate the principle of site-specific coordination mapping. Analysis of the site-specific Fe-L2,3 data reveals distinct variations in the fine structure that are attributed to Fe in a six-fold (octahedron) or five-fold (distorted tetragonal pyramid) oxygen coordination. Using these variations, atomic resolution coordination maps are generated that are in excellent agreement with simulations.

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TURNER S. et al. Site-specific mapping of transition metal oxygen coordination in complex oxides // Applied Physics Letters. 2012. Vol. 101. No. 24. p. 241910.

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TURNER S., Egoavil R., Batuk M., Abakumov A. A., Hadermann J., Verbeeck J., Van Tendeloo G. Site-specific mapping of transition metal oxygen coordination in complex oxides // Applied Physics Letters. 2012. Vol. 101. No. 24. p. 241910.

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TY - JOUR

DO - 10.1063/1.4770512

UR - https://doi.org/10.1063/1.4770512

TI - Site-specific mapping of transition metal oxygen coordination in complex oxides

T2 - Applied Physics Letters

AU - TURNER, S

AU - Egoavil, R

AU - Batuk, M

AU - Abakumov, A A

AU - Hadermann, J.

AU - Verbeeck, J.

AU - Van Tendeloo, G.

PY - 2012

DA - 2012/12/10

PB - AIP Publishing

SP - 241910

IS - 24

VL - 101

SN - 0003-6951

SN - 1077-3118

ER -

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@article{2012_TURNER,

author = {S TURNER and R Egoavil and M Batuk and A A Abakumov and J. Hadermann and J. Verbeeck and G. Van Tendeloo},

title = {Site-specific mapping of transition metal oxygen coordination in complex oxides},

journal = {Applied Physics Letters},

year = {2012},

volume = {101},

publisher = {AIP Publishing},

month = {dec},

url = {https://doi.org/10.1063/1.4770512},

number = {24},

pages = {241910},

doi = {10.1063/1.4770512}

}

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TURNER, S., et al. “Site-specific mapping of transition metal oxygen coordination in complex oxides.” Applied Physics Letters, vol. 101, no. 24, Dec. 2012, p. 241910. https://doi.org/10.1063/1.4770512.