Open Access
Proceedings of the National Academy of Sciences of the United States of America, volume 114, issue 42, pages 11069-11074
An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes
Chen-Zi Zhao
1
,
Xue-Qiang Zhang
1
,
Xin-Bing Cheng
1
,
Rui Zhang
1
,
Rui Xu
2
,
Peng-Yu Chen
1
,
Hong-Jie Peng
1
,
Jia-Qi Huang
2
,
Qiang Zhang
1
Publication type: Journal Article
Publication date: 2017-10-02
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 11.1
ISSN: 00278424, 10916490
PubMed ID:
28973945
Multidisciplinary
Abstract
Significance
The Li metal electrode is regarded as a “Holy Grail” anode for next-generation batteries due to its extremely high theoretical capacity and lowest reduction potential. Unfortunately, uncontrolled dendrite growth leads to serious safety issues. This work realizes a dendrite-free Li metal anode by introducing an anion-immobilized composite solid electrolyte, where anions are tethered to polymer chains and ceramic particles. Immobilized anions contribute to uniform distribution of Li ions and dendrite-free Li deposition. The flexible electrolyte can be applied in all–solid-state Li metal batteries with excellent specific capacities. This work demonstrates a concept to adjust ion distribution based on solid-state electrolytes for safe dendrite-free Li anodes, paving the way to practical Li metal batteries.
Top-30
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Citations by publishers
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Elsevier
274 publications, 37.9%
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Wiley
166 publications, 22.96%
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American Chemical Society (ACS)
120 publications, 16.6%
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Royal Society of Chemistry (RSC)
64 publications, 8.85%
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Springer Nature
53 publications, 7.33%
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10 publications, 1.38%
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9 publications, 1.24%
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Proceedings of the National Academy of Sciences (PNAS)
4 publications, 0.55%
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IOP Publishing
3 publications, 0.41%
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American Institute of Physics (AIP)
2 publications, 0.28%
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World Scientific
1 publication, 0.14%
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Frontiers Media S.A.
1 publication, 0.14%
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Tsinghua University Press
1 publication, 0.14%
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Materials Research Society
1 publication, 0.14%
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Chemical Industry Press
1 publication, 0.14%
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KeAi Communications Co.
1 publication, 0.14%
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Oxford University Press
1 publication, 0.14%
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1 publication, 0.14%
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Chinese Physical Society
1 publication, 0.14%
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Hans Publishers
1 publication, 0.14%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.14%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhao C. et al. An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes // Proceedings of the National Academy of Sciences of the United States of America. 2017. Vol. 114. No. 42. pp. 11069-11074.
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Zhao C., Zhang X., Cheng X., Zhang R., Xu R., Chen P., Peng H., Huang J., Zhang Q. An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes // Proceedings of the National Academy of Sciences of the United States of America. 2017. Vol. 114. No. 42. pp. 11069-11074.
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TY - JOUR
DO - 10.1073/pnas.1708489114
UR - https://doi.org/10.1073/pnas.1708489114
TI - An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes
T2 - Proceedings of the National Academy of Sciences of the United States of America
AU - Zhao, Chen-Zi
AU - Zhang, Xue-Qiang
AU - Cheng, Xin-Bing
AU - Zhang, Rui
AU - Xu, Rui
AU - Chen, Peng-Yu
AU - Peng, Hong-Jie
AU - Huang, Jia-Qi
AU - Zhang, Qiang
PY - 2017
DA - 2017/10/02 00:00:00
PB - Proceedings of the National Academy of Sciences (PNAS)
SP - 11069-11074
IS - 42
VL - 114
PMID - 28973945
SN - 0027-8424
SN - 1091-6490
ER -
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@article{2017_Zhao,
author = {Chen-Zi Zhao and Xue-Qiang Zhang and Xin-Bing Cheng and Rui Zhang and Rui Xu and Peng-Yu Chen and Hong-Jie Peng and Jia-Qi Huang and Qiang Zhang},
title = {An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
year = {2017},
volume = {114},
publisher = {Proceedings of the National Academy of Sciences (PNAS)},
month = {oct},
url = {https://doi.org/10.1073/pnas.1708489114},
number = {42},
pages = {11069--11074},
doi = {10.1073/pnas.1708489114}
}
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Zhao, Chen-Zi, et al. “An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes.” Proceedings of the National Academy of Sciences of the United States of America, vol. 114, no. 42, Oct. 2017, pp. 11069-11074. https://doi.org/10.1073/pnas.1708489114.