Open Access
,
volume 114
,
issue 42
,
pages 11069-11074
An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes
Chen-Zi Zhao
1
,
Xue-Qiang Zhang
1
,
Xin-Bing Cheng
1
,
Rui Zhang
1
,
Rui Xu
2
,
Peng-Yu Chen
1
,
Hong-Jie Peng
1
,
Jia-Qi Huang
2
,
Qiang Zhang
1
Publication type: Journal Article
Publication date: 2017-10-02
scimago Q1
wos Q1
SJR: 3.414
CiteScore: 16.5
Impact factor: 9.1
ISSN: 00278424, 10916490
PubMed ID:
28973945
Multidisciplinary
Abstract
Significance
The Li metal electrode is regarded as a “Holy Grail” anode for next-generation batteries due to its extremely high theoretical capacity and lowest reduction potential. Unfortunately, uncontrolled dendrite growth leads to serious safety issues. This work realizes a dendrite-free Li metal anode by introducing an anion-immobilized composite solid electrolyte, where anions are tethered to polymer chains and ceramic particles. Immobilized anions contribute to uniform distribution of Li ions and dendrite-free Li deposition. The flexible electrolyte can be applied in all–solid-state Li metal batteries with excellent specific capacities. This work demonstrates a concept to adjust ion distribution based on solid-state electrolytes for safe dendrite-free Li anodes, paving the way to practical Li metal batteries.
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Metrics
801
Total citations:
801
Citations from 2024:
142
(17%)
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GOST
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Zhao C. et al. An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes // Proceedings of the National Academy of Sciences of the United States of America. 2017. Vol. 114. No. 42. pp. 11069-11074.
GOST all authors (up to 50)
Copy
Zhao C., Zhang X., Cheng X., Zhang R., Xu R., Chen P., Peng H., Huang J., Zhang Q. An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes // Proceedings of the National Academy of Sciences of the United States of America. 2017. Vol. 114. No. 42. pp. 11069-11074.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1073/pnas.1708489114
UR - https://doi.org/10.1073/pnas.1708489114
TI - An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes
T2 - Proceedings of the National Academy of Sciences of the United States of America
AU - Zhao, Chen-Zi
AU - Zhang, Xue-Qiang
AU - Cheng, Xin-Bing
AU - Zhang, Rui
AU - Xu, Rui
AU - Chen, Peng-Yu
AU - Peng, Hong-Jie
AU - Huang, Jia-Qi
AU - Zhang, Qiang
PY - 2017
DA - 2017/10/02
PB - Proceedings of the National Academy of Sciences (PNAS)
SP - 11069-11074
IS - 42
VL - 114
PMID - 28973945
SN - 0027-8424
SN - 1091-6490
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2017_Zhao,
author = {Chen-Zi Zhao and Xue-Qiang Zhang and Xin-Bing Cheng and Rui Zhang and Rui Xu and Peng-Yu Chen and Hong-Jie Peng and Jia-Qi Huang and Qiang Zhang},
title = {An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
year = {2017},
volume = {114},
publisher = {Proceedings of the National Academy of Sciences (PNAS)},
month = {oct},
url = {https://doi.org/10.1073/pnas.1708489114},
number = {42},
pages = {11069--11074},
doi = {10.1073/pnas.1708489114}
}
Cite this
MLA
Copy
Zhao, Chen-Zi, et al. “An anion-immobilized composite electrolyte for dendrite-free lithium metal anodes.” Proceedings of the National Academy of Sciences of the United States of America, vol. 114, no. 42, Oct. 2017, pp. 11069-11074. https://doi.org/10.1073/pnas.1708489114.