Synthesis and binding ability of mono- and tetrasubstituted aminophosphonate Zn-tetraarylporphyrins towards N- and O-containing organic substrates
Publication type: Journal Article
Publication date: 2013-11-06
scimago Q3
wos Q2
SJR: 0.222
CiteScore: 2.3
Impact factor: 2.6
ISSN: 10610278, 10290478, 10267816
General Chemistry
Abstract
The 1,6-addition of mono- and tetra-amino 5,10,15,20-tetraphenylporphyrins with dimethyl-(3,5-di-tert-butyl-4-oxocyclohexa-2,5-dienylidenemethyl)phosphonate leads to the corresponding mono- and tetrasubstituted aminophosphonate porphyrin derivatives. The binding ability of their Zn(II)-complexes towards 1,4-diazabicyclo[2,2,2]octane, imidazole, 4-(1H-imidazole-1-yl)benzyl alcohol and 4-(1H-imidazole-1-ylmethyl)benzyl alcohol in toluene was investigated by spectrophotometric and 1H NMR titration. It has been determined that the monosubstituted Zn-tetraarylporphyrin is involved in a two-point selective binding of 4-(1H-imidazole-1-ylmethyl)benzyl alcohol. Taking into account the fact that this binding is accompanied by a clear and easily identifiable response in the UV–vis spectra of the reaction mixture, this metalloporphyrin could be considered as a molecular optical sensing device for selected bidentate N- and O-containing substrates.
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Mamardashvili N. et al. Synthesis and binding ability of mono- and tetrasubstituted aminophosphonate Zn-tetraarylporphyrins towards N- and O-containing organic substrates // Supramolecular Chemistry. 2013. Vol. 26. No. 5-6. pp. 427-434.
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Mamardashvili N., Shaekhov T., Gibadullina E., Voronina J. K., Burilov A., Koifman O. I., Dehaen W. Synthesis and binding ability of mono- and tetrasubstituted aminophosphonate Zn-tetraarylporphyrins towards N- and O-containing organic substrates // Supramolecular Chemistry. 2013. Vol. 26. No. 5-6. pp. 427-434.
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TY - JOUR
DO - 10.1080/10610278.2013.844819
UR - https://doi.org/10.1080/10610278.2013.844819
TI - Synthesis and binding ability of mono- and tetrasubstituted aminophosphonate Zn-tetraarylporphyrins towards N- and O-containing organic substrates
T2 - Supramolecular Chemistry
AU - Mamardashvili, N.Zh.
AU - Shaekhov, Timur
AU - Gibadullina, Elmira
AU - Voronina, Julia K.
AU - Burilov, Aleksander
AU - Koifman, Oskar I.
AU - Dehaen, Wim
PY - 2013
DA - 2013/11/06
PB - Taylor & Francis
SP - 427-434
IS - 5-6
VL - 26
SN - 1061-0278
SN - 1029-0478
SN - 1026-7816
ER -
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@article{2013_Mamardashvili,
author = {N.Zh. Mamardashvili and Timur Shaekhov and Elmira Gibadullina and Julia K. Voronina and Aleksander Burilov and Oskar I. Koifman and Wim Dehaen},
title = {Synthesis and binding ability of mono- and tetrasubstituted aminophosphonate Zn-tetraarylporphyrins towards N- and O-containing organic substrates},
journal = {Supramolecular Chemistry},
year = {2013},
volume = {26},
publisher = {Taylor & Francis},
month = {nov},
url = {https://doi.org/10.1080/10610278.2013.844819},
number = {5-6},
pages = {427--434},
doi = {10.1080/10610278.2013.844819}
}
Cite this
MLA
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Mamardashvili, N.Zh., et al. “Synthesis and binding ability of mono- and tetrasubstituted aminophosphonate Zn-tetraarylporphyrins towards N- and O-containing organic substrates.” Supramolecular Chemistry, vol. 26, no. 5-6, Nov. 2013, pp. 427-434. https://doi.org/10.1080/10610278.2013.844819.