volume 29 issue 9 pages 678-684

Radical character of non-IPR isomer 17418 (C1) of fullerene C76

Publication typeJournal Article
Publication date2021-02-03
scimago Q3
wos Q3
SJR0.362
CiteScore4.0
Impact factor1.8
ISSN1536383X, 15364046
Organic Chemistry
Physical and Theoretical Chemistry
Atomic and Molecular Physics, and Optics
General Materials Science
Abstract
Abstract Using a theoretical approach supported by DFT calculations, the features of molecular structure of isomer 17418 (C1) of fullerene C76 with the distribution of single, double and delocalized π-bonds has been determined for the first time. It is shown the radical nature together with the well-known overstrain due to pentalene fragment are the reasons for the instability of this fullerene as empty molecule. The synthesis of endohedral metallofulerenes is accompanied by the formation of an ion pair: the fullerene anion and a metal cation inside the molecule. It`s leading to the closure of the electron shell of the fullerene molecule and the removal of excess local strains. The previously experimentally determined cations sites inside the fullerene, which stabilize the molecule as a whole, are close to the disclosed radical clusters.
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Khamatgalimov A. et al. Radical character of non-IPR isomer 17418 (C1) of fullerene C76 // Fullerenes Nanotubes and Carbon Nanostructures. 2021. Vol. 29. No. 9. pp. 678-684.
GOST all authors (up to 50) Copy
Khamatgalimov A., Egorova A., Chachkov D., Kovalenko V. Radical character of non-IPR isomer 17418 (C1) of fullerene C76 // Fullerenes Nanotubes and Carbon Nanostructures. 2021. Vol. 29. No. 9. pp. 678-684.
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TY - JOUR
DO - 10.1080/1536383x.2021.1880393
UR - https://doi.org/10.1080/1536383x.2021.1880393
TI - Radical character of non-IPR isomer 17418 (C1) of fullerene C76
T2 - Fullerenes Nanotubes and Carbon Nanostructures
AU - Khamatgalimov, A.R
AU - Egorova, Anna
AU - Chachkov, D.V.
AU - Kovalenko, V.I.
PY - 2021
DA - 2021/02/03
PB - Taylor & Francis
SP - 678-684
IS - 9
VL - 29
SN - 1536-383X
SN - 1536-4046
ER -
BibTex |
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BibTex (up to 50 authors) Copy
@article{2021_Khamatgalimov,
author = {A.R Khamatgalimov and Anna Egorova and D.V. Chachkov and V.I. Kovalenko},
title = {Radical character of non-IPR isomer 17418 (C1) of fullerene C76},
journal = {Fullerenes Nanotubes and Carbon Nanostructures},
year = {2021},
volume = {29},
publisher = {Taylor & Francis},
month = {feb},
url = {https://doi.org/10.1080/1536383x.2021.1880393},
number = {9},
pages = {678--684},
doi = {10.1080/1536383x.2021.1880393}
}
MLA
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Khamatgalimov, A.R, et al. “Radical character of non-IPR isomer 17418 (C1) of fullerene C76.” Fullerenes Nanotubes and Carbon Nanostructures, vol. 29, no. 9, Feb. 2021, pp. 678-684. https://doi.org/10.1080/1536383x.2021.1880393.