Physical Review B, volume 71, issue 16, publication number 161302

Correlation between photoluminescence intermittency of CdSe quantum dots and self-trapped states in dielectric media

Publication typeJournal Article
Publication date2005-04-08
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor3.7
ISSN24699950, 24699969, 10980121, 1550235X
Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Abstract
We present evidence that the photoluminescence intermittency of $\mathrm{Cd}\mathrm{Se}∕\mathrm{Zn}\mathrm{S}$ core/shell quantum dots is correlated with the dielectric environment surrounding the quantum dots. The statistics of dark state lifetimes in the intermittency is found to be related to the stabilization energy of charges in the local dielectric surrounding of the quantum dot. This supports the model of an ionized quantum dot in the dark state. Charges ejected from the quantum dot are suggested to be self-trapped in mid-bandgap states of the surrounding matrix due to atomic and electronic relaxation processes. These trap states are inherent to disordered materials and proposed to be a general source of power law intermittency of various types of emitters such as quantum dots and dye molecules.

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Issac A., von Borczyskowski C., Cichos F. Correlation between photoluminescence intermittency of CdSe quantum dots and self-trapped states in dielectric media // Physical Review B. 2005. Vol. 71. No. 16. 161302
GOST all authors (up to 50) Copy
Issac A., von Borczyskowski C., Cichos F. Correlation between photoluminescence intermittency of CdSe quantum dots and self-trapped states in dielectric media // Physical Review B. 2005. Vol. 71. No. 16. 161302
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RIS Copy
TY - JOUR
DO - 10.1103/physrevb.71.161302
UR - https://doi.org/10.1103/physrevb.71.161302
TI - Correlation between photoluminescence intermittency of CdSe quantum dots and self-trapped states in dielectric media
T2 - Physical Review B
AU - Issac, Abey
AU - von Borczyskowski, Christian
AU - Cichos, Frank
PY - 2005
DA - 2005/04/08 00:00:00
PB - American Physical Society (APS)
IS - 16
VL - 71
SN - 2469-9950
SN - 2469-9969
SN - 1098-0121
SN - 1550-235X
ER -
BibTex
Cite this
BibTex Copy
@article{2005_Issac,
author = {Abey Issac and Christian von Borczyskowski and Frank Cichos},
title = {Correlation between photoluminescence intermittency of CdSe quantum dots and self-trapped states in dielectric media},
journal = {Physical Review B},
year = {2005},
volume = {71},
publisher = {American Physical Society (APS)},
month = {apr},
url = {https://doi.org/10.1103/physrevb.71.161302},
number = {16},
doi = {10.1103/physrevb.71.161302}
}
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