Physical Review B, volume 78, issue 12, publication number 125325
Carrier multiplication yields in PbS and PbSe nanocrystals measured by transient photoluminescence
Publication type: Journal Article
Publication date: 2008-09-29
Journal:
Physical Review B
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.7
ISSN: 24699950, 24699969, 10980121, 1550235X
Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Abstract
We report here an assessment of carrier multiplication (CM) yields in PbSe and PbS nanocrystals (NCs) by a quantitative analysis of biexciton and exciton dynamics in transient photoluminescence decays. Interest in CM, the generation of more than one electron and hole in a semiconductor after absorption of one photon, has renewed in recent years because of reports suggesting greatly increased efficiencies in nanocrystalline materials compared to the bulk form, in which CM was otherwise too weak to be of consequence in photovoltaic energy conversion devices. In our PbSe and PbS NC samples, however, we estimate using transient photoluminescence that at most 0.25 additional e-h pairs are generated per photon even at energies hv > 5Eg, instead of the much higher values reported in the literature. We argue by comparing NC CM estimates and reported bulk values on an absolute energy basis, which we justify as appropriate on physical grounds, that the data reported thus far are inconclusive with respect to the importance of nanoscale-specific phenomena in the CM process.
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Citations by publishers
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83 publications, 40.89%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
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Nair G. et al. Carrier multiplication yields in PbS and PbSe nanocrystals measured by transient photoluminescence // Physical Review B. 2008. Vol. 78. No. 12. 125325
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Nair G., Geyer S. M., Geyer S. M., Chang L., Bawendi M. G., Bawendi M. G. Carrier multiplication yields in PbS and PbSe nanocrystals measured by transient photoluminescence // Physical Review B. 2008. Vol. 78. No. 12. 125325
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TY - JOUR
DO - 10.1103/physrevb.78.125325
UR - https://doi.org/10.1103/physrevb.78.125325
TI - Carrier multiplication yields in PbS and PbSe nanocrystals measured by transient photoluminescence
T2 - Physical Review B
AU - Nair, Gautham
AU - Geyer, Scott M
AU - Chang, Liang-Yi
AU - Bawendi, Moungi G
AU - Geyer, Scott M.
AU - Bawendi, Moungi G.
PY - 2008
DA - 2008/09/29 00:00:00
PB - American Physical Society (APS)
IS - 12
VL - 78
SN - 2469-9950
SN - 2469-9969
SN - 1098-0121
SN - 1550-235X
ER -
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@article{2008_Nair,
author = {Gautham Nair and Scott M Geyer and Liang-Yi Chang and Moungi G Bawendi and Scott M. Geyer and Moungi G. Bawendi},
title = {Carrier multiplication yields in PbS and PbSe nanocrystals measured by transient photoluminescence},
journal = {Physical Review B},
year = {2008},
volume = {78},
publisher = {American Physical Society (APS)},
month = {sep},
url = {https://doi.org/10.1103/physrevb.78.125325},
number = {12},
doi = {10.1103/physrevb.78.125325}
}
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