Physical Review B, volume 82, issue 12, publication number 125320
Temperature-dependent photoluminescence of PbS quantum dots in glass: Evidence of exciton state splitting and carrier trapping
Maxim S. Gaponenko
1
,
Andrey A. Lutich
2
,
Nikolai A. Tolstik
1
,
Alexei A. Onushchenko
3
,
Alexander M. Malyarevich
1
,
Eugene P Petrov
4
,
E.P Petrov
4
,
Konstantin V. Yumashev
1
3
Research and Technological Institute of Optical Materials Science, 193171 St. Petersburg, Russia
|
Publication type: Journal Article
Publication date: 2010-09-17
Journal:
Physical Review B
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.7
ISSN: 24699950, 24699969, 10980121, 1550235X
Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Abstract
We report experimental evidence of the lowest exciton state splitting and carrier trapping in PbS quantum dots (QDs) in glass matrix. Our measurements of photoluminescence (PL) of PbS QDs using steady-state and time-resolved PL spectroscopy reveal strong temperature dependences of the PL intensity and decay kinetics. We find that consistent quantitative description of our experimental results can be achieved using a simple model taking into account the lowest 1S-1S exciton state splitting and multiphonon-assisted carrier trapping to states outside a PbS QD. Using our model, we estimate the lowest exciton splitting energy and lifetimes of the dark and bright exciton states of PbS QDs. Consistent with our model, the PL transition energy of PbS QDs deviates at higher temperatures from the one predicted based on the bulk PbS band-gap dependence due to the lowest 1S-1S exciton state splitting. Temperature-induced broadening of the PL spectrum of PbS QDs is explained by the exciton-phonon interaction.
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1 publication, 0.87%
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1 publication, 0.87%
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Journal of Electronic Materials
1 publication, 0.87%
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Citations by publishers
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American Chemical Society (ACS)
36 publications, 31.3%
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Elsevier
18 publications, 15.65%
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Wiley
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IOP Publishing
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Springer Nature
5 publications, 4.35%
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American Physical Society (APS)
4 publications, 3.48%
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Optical Society of America
3 publications, 2.61%
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Materials Research Society
2 publications, 1.74%
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Pleiades Publishing
1 publication, 0.87%
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Optical Society of India
1 publication, 0.87%
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1 publication, 0.87%
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Oxford University Press
1 publication, 0.87%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Gaponenko M. S. et al. Temperature-dependent photoluminescence of PbS quantum dots in glass: Evidence of exciton state splitting and carrier trapping // Physical Review B. 2010. Vol. 82. No. 12. 125320
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Gaponenko M. S., Lutich A. A., Tolstik N. A., Onushchenko A. A., Malyarevich A. M., Petrov E. P., Petrov E., Yumashev K. V. Temperature-dependent photoluminescence of PbS quantum dots in glass: Evidence of exciton state splitting and carrier trapping // Physical Review B. 2010. Vol. 82. No. 12. 125320
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TY - JOUR
DO - 10.1103/physrevb.82.125320
UR - https://doi.org/10.1103/physrevb.82.125320
TI - Temperature-dependent photoluminescence of PbS quantum dots in glass: Evidence of exciton state splitting and carrier trapping
T2 - Physical Review B
AU - Gaponenko, Maxim S.
AU - Lutich, Andrey A.
AU - Tolstik, Nikolai A.
AU - Onushchenko, Alexei A.
AU - Malyarevich, Alexander M.
AU - Petrov, Eugene P
AU - Yumashev, Konstantin V.
AU - Petrov, E.P
PY - 2010
DA - 2010/09/17 00:00:00
PB - American Physical Society (APS)
IS - 12
VL - 82
SN - 2469-9950
SN - 2469-9969
SN - 1098-0121
SN - 1550-235X
ER -
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@article{2010_Gaponenko,
author = {Maxim S. Gaponenko and Andrey A. Lutich and Nikolai A. Tolstik and Alexei A. Onushchenko and Alexander M. Malyarevich and Eugene P Petrov and Konstantin V. Yumashev and E.P Petrov},
title = {Temperature-dependent photoluminescence of PbS quantum dots in glass: Evidence of exciton state splitting and carrier trapping},
journal = {Physical Review B},
year = {2010},
volume = {82},
publisher = {American Physical Society (APS)},
month = {sep},
url = {https://doi.org/10.1103/physrevb.82.125320},
number = {12},
doi = {10.1103/physrevb.82.125320}
}