Physical Review B, volume 60, issue 4, pages R2177-R2180
Ultrafast dynamics of inter- and intraband transitions in semiconductor nanocrystals: Implications for quantum-dot lasers
Victor I. Klimov
1
,
V. I. KLIMOV
1
,
Ch. J. Schwarz
1
,
D.W. McBranch
1
,
C. A. Leatherdale
2, 3
,
Moungi G. Bawendi
2, 3
,
M G Bawendi
2, 3
1
Chemical Sciences and Technology Division, CST-6, MS-J585, Los Alamos National Laboratory, Los Alamos, New Mexico 87545
|
2
Department of Chemistry and Center for Materials Science and Engineering
Publication type: Journal Article
Publication date: 1999-07-15
Journal:
Physical Review B
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.7
ISSN: 24699950, 24699969, 10980121, 1550235X
Abstract
Application of femtosecond transient absorption in the visible and near-IR spectral ranges and time-resolved photoluminescence allows us to separate electron and hole relaxation paths and to map the structure of interband and intraband optical transitions in CdSe and CdS nanocrystals (NC's) with a wide range of surface properties. In contrast to electron relaxation, which is controlled by NC surface passivation, depopulation of hole quantized states is extremely fast (sub-ps-to-ps time scales) in all types samples, independent of NC surface treatment (including NC's overcoated with a ZnS layer). Our results suggest that ultrafast hole dynamics are not due to trapping at localized surface defects such as a vacancy, but rather arise from relaxation into intrinsic NC states or intrinsically unpassivated interface states.
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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KLIMOV V. I. et al. Ultrafast dynamics of inter- and intraband transitions in semiconductor nanocrystals: Implications for quantum-dot lasers // Physical Review B. 1999. Vol. 60. No. 4. p. R2177-R2180.
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KLIMOV V. I., Klimov V. I., Schwarz C. J., McBranch D., Leatherdale C. A., Bawendi M. G., Bawendi M. G. Ultrafast dynamics of inter- and intraband transitions in semiconductor nanocrystals: Implications for quantum-dot lasers // Physical Review B. 1999. Vol. 60. No. 4. p. R2177-R2180.
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TY - JOUR
DO - 10.1103/physrevb.60.r2177
UR - https://doi.org/10.1103/physrevb.60.r2177
TI - Ultrafast dynamics of inter- and intraband transitions in semiconductor nanocrystals: Implications for quantum-dot lasers
T2 - Physical Review B
AU - KLIMOV, V. I.
AU - Schwarz, Ch. J.
AU - McBranch, D.W.
AU - Leatherdale, C. A.
AU - Bawendi, M G
AU - Klimov, Victor I.
AU - Bawendi, Moungi G.
PY - 1999
DA - 1999/07/15 00:00:00
PB - American Physical Society (APS)
SP - R2177-R2180
IS - 4
VL - 60
SN - 2469-9950
SN - 2469-9969
SN - 1098-0121
SN - 1550-235X
ER -
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@article{1999_KLIMOV,
author = {V. I. KLIMOV and Ch. J. Schwarz and D.W. McBranch and C. A. Leatherdale and M G Bawendi and Victor I. Klimov and Moungi G. Bawendi},
title = {Ultrafast dynamics of inter- and intraband transitions in semiconductor nanocrystals: Implications for quantum-dot lasers},
journal = {Physical Review B},
year = {1999},
volume = {60},
publisher = {American Physical Society (APS)},
month = {jul},
url = {https://doi.org/10.1103/physrevb.60.r2177},
number = {4},
pages = {R2177--R2180},
doi = {10.1103/physrevb.60.r2177}
}
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KLIMOV, V. I., et al. “Ultrafast dynamics of inter- and intraband transitions in semiconductor nanocrystals: Implications for quantum-dot lasers.” Physical Review B, vol. 60, no. 4, Jul. 1999, pp. R2177-R2180. https://doi.org/10.1103/physrevb.60.r2177.
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