Physical Review B, volume 61, issue 20, pages R13349-R13352
Mechanisms for intraband energy relaxation in semiconductor quantum dots: The role of electron-hole interactions
Victor I. Klimov
1
,
V. I. KLIMOV
1
,
A A Mikhailovsky
1
,
A. A. Mikhailovsky
1
,
D.W. McBranch
1
,
C. A. Leatherdale
2
,
M G Bawendi
2
1
Chemical Science and Technology Division, CST-6, MS-J585, Los Alamos National Laboratory, Los Alamos, New Mexico 87545
|
Publication type: Journal Article
Publication date: 2000-05-15
Journal:
Physical Review B
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.7
ISSN: 24699950, 24699969, 10980121, 1550235X
Abstract
To evaluate the role of nonphonon energy relaxation mechanisms in quantum dots and in particular the role of electron-hole (e-h) interactions, we have studied femtosecond carrier dynamics in CdSe colloidal nanoparticles in which the e-h separation (coupling) is controlled using different types of surface ligands. In dots capped with hole accepting molecules, the e-h coupling is strongly reduced after the hole is transferred to a capping group. By re-exciting an electron within the conduction band at different stages of hole transfer and monitoring its relaxation back into the ground state, we observe a more than tenfold increase in the electron relaxation time (from 250 fs to 3 ps) after the completion of the hole transfer to the capping molecule. This strongly indicates that electron relaxation in quantum dots is dominated not by phonon emission but by the e-h energy transfer.
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Citations by publishers
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20
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120
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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KLIMOV V. I. et al. Mechanisms for intraband energy relaxation in semiconductor quantum dots: The role of electron-hole interactions // Physical Review B. 2000. Vol. 61. No. 20. p. R13349-R13352.
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KLIMOV V. I., Klimov V. I., Mikhailovsky A. A., Mikhailovsky A. A., McBranch D., Leatherdale C. A., Bawendi M. G., Bawendi M. G. Mechanisms for intraband energy relaxation in semiconductor quantum dots: The role of electron-hole interactions // Physical Review B. 2000. Vol. 61. No. 20. p. R13349-R13352.
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TY - JOUR
DO - 10.1103/physrevb.61.r13349
UR - https://doi.org/10.1103/physrevb.61.r13349
TI - Mechanisms for intraband energy relaxation in semiconductor quantum dots: The role of electron-hole interactions
T2 - Physical Review B
AU - KLIMOV, V. I.
AU - Mikhailovsky, A A
AU - McBranch, D.W.
AU - Leatherdale, C. A.
AU - Bawendi, M G
AU - Klimov, Victor I.
AU - Mikhailovsky, A. A.
AU - Bawendi, Moungi G.
PY - 2000
DA - 2000/05/15 00:00:00
PB - American Physical Society (APS)
SP - R13349-R13352
IS - 20
VL - 61
SN - 2469-9950
SN - 2469-9969
SN - 1098-0121
SN - 1550-235X
ER -
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@article{2000_KLIMOV,
author = {V. I. KLIMOV and A A Mikhailovsky and D.W. McBranch and C. A. Leatherdale and M G Bawendi and Victor I. Klimov and A. A. Mikhailovsky and Moungi G. Bawendi},
title = {Mechanisms for intraband energy relaxation in semiconductor quantum dots: The role of electron-hole interactions},
journal = {Physical Review B},
year = {2000},
volume = {61},
publisher = {American Physical Society (APS)},
month = {may},
url = {https://doi.org/10.1103/physrevb.61.r13349},
number = {20},
pages = {R13349--R13352},
doi = {10.1103/physrevb.61.r13349}
}
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KLIMOV, V. I., et al. “Mechanisms for intraband energy relaxation in semiconductor quantum dots: The role of electron-hole interactions.” Physical Review B, vol. 61, no. 20, May. 2000, pp. R13349-R13352. https://doi.org/10.1103/physrevb.61.r13349.
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