Physical Review B, volume 63, issue 20, publication number 205316
Blinking statistics in single semiconductor nanocrystal quantum dots
Publication type: Journal Article
Publication date: 2001-05-02
Journal:
Physical Review B
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.7
ISSN: 24699950, 24699969, 10980121, 1550235X
Abstract
Statistical studies of fluorescence intermittency in single CdSe nanocrystal quantum dots (QD's) reveal a temperature-independent power-law distribution in the histogram of on and off times---the time periods before the QD turns from emitting to nonemitting (bright to dark) and vice versa. Every QD shows a similar power-law behavior for the off-time distribution regardless of temperature, excitation intensity, surface morphology or size. We propose a dynamic model of tunneling between core and trapped charged states to explain the universal power-law statistics of the blinking events observed. The on-time probability distributions show evidence of both a tunneling mechanism similar to the off-time statistics and a secondary, photoinduced process that leads to a truncation of the power law. The same blinking statistics are also observed for single CdTe nanocrystal QD's.
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Citations by publishers
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American Chemical Society (ACS)
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American Physical Society (APS)
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1 publication, 0.2%
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Biophysical Society
1 publication, 0.2%
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IEEE
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Shimizu K. T. et al. Blinking statistics in single semiconductor nanocrystal quantum dots // Physical Review B. 2001. Vol. 63. No. 20. 205316
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Shimizu K. T., Neuhauser R. G., Leatherdale C. A., Empedocles S. A., Woo W. K., Bawendi M. G., Bawendi M. G. Blinking statistics in single semiconductor nanocrystal quantum dots // Physical Review B. 2001. Vol. 63. No. 20. 205316
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TY - JOUR
DO - 10.1103/PhysRevB.63.205316
UR - https://doi.org/10.1103/PhysRevB.63.205316
TI - Blinking statistics in single semiconductor nanocrystal quantum dots
T2 - Physical Review B
AU - Shimizu, K T
AU - Neuhauser, R. G.
AU - Leatherdale, C. A.
AU - Empedocles, S. A.
AU - Bawendi, M G
AU - Woo, W. K.
AU - Bawendi, Moungi G.
PY - 2001
DA - 2001/05/02 00:00:00
PB - American Physical Society (APS)
IS - 20
VL - 63
SN - 2469-9950
SN - 2469-9969
SN - 1098-0121
SN - 1550-235X
ER -
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@article{2001_Shimizu,
author = {K T Shimizu and R. G. Neuhauser and C. A. Leatherdale and S. A. Empedocles and M G Bawendi and W. K. Woo and Moungi G. Bawendi},
title = {Blinking statistics in single semiconductor nanocrystal quantum dots},
journal = {Physical Review B},
year = {2001},
volume = {63},
publisher = {American Physical Society (APS)},
month = {may},
url = {https://doi.org/10.1103/PhysRevB.63.205316},
number = {20},
doi = {10.1103/PhysRevB.63.205316}
}
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