Physical Review B, volume 72, issue 19, publication number 195312

Time-resolved intraband relaxation of strongly confined electrons and holes in colloidal PbSe nanocrystals

Jeffrey M. Harbold ¹

Hui Du ²

Todd D Krauss ²

Todd Krauss ²

Kyung-Sang Cho ³

Chris B Murray ³

Chris Murray ³

Frank W Wise ¹

Frank Wise Frank Wise ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

Department of applied physics, Cornell University, Ithaca, New York 14853, USA |

Department of Chemistry, University of Rochester, Rochester, New York 14627, USA |

IBM, T. J. Watson Research Center, Yorktown Heights, New York 10598, USA |

Publication type: Journal Article

Publication date: 2005-11-08

American Physical Society (APS)

Journal: Physical Review B

Quartile SCImago

Quartile WOS

Impact factor: 3.7

ISSN: 24699950, 24699969, 10980121, 1550235X

DOI: 10.1103/physrevb.72.195312

Copy DOI

Electronic, Optical and Magnetic Materials

Condensed Matter Physics

Abstract

The relaxation of strongly-confined electrons and holes between 1P and 1S levels in colloidal PbSe nanocrystals has been time-resolved using femtosecond transient absorption spectroscopy. In contrast to II-VI and III-V semiconductor nanocrystals, both electrons and holes are strongly confined in PbSe nanocrystals. Despite the large electron and hole energy level spacings (at least 12 times the optical phonon energy), we consistently observe picosecond time-scale relaxation. Existing theories of carrier relaxation cannot account for these experimental results. Mechanisms that could possibly circumvent the phonon bottleneck in IV-VI quantum dots are discussed.

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Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 1.5% Journal of the American Chemical Society 2 publications, 1.5%
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Applied Optics	Applied Optics, 2, 1.5% Applied Optics 2 publications, 1.5%
ACS Symposium Series	ACS Symposium Series, 2, 1.5% ACS Symposium Series 2 publications, 1.5%
Physical Review Letters	Physical Review Letters, 1, 0.75% Physical Review Letters 1 publication, 0.75%
EPJ Web of Conferences	EPJ Web of Conferences, 1, 0.75% EPJ Web of Conferences 1 publication, 0.75%
Uspekhi Fizicheskih Nauk	Uspekhi Fizicheskih Nauk, 1, 0.75% Uspekhi Fizicheskih Nauk 1 publication, 0.75%
Scientific Reports	Scientific Reports, 1, 0.75% Scientific Reports 1 publication, 0.75%
Nature	Nature, 1, 0.75% Nature 1 publication, 0.75%
Nature Communications	Nature Communications, 1, 0.75% Nature Communications 1 publication, 0.75%
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Journal of Nanostructure in Chemistry	Journal of Nanostructure in Chemistry, 1, 0.75% Journal of Nanostructure in Chemistry 1 publication, 0.75%
Journal of Physics: Conference Series	Journal of Physics: Conference Series, 1, 0.75% Journal of Physics: Conference Series 1 publication, 0.75%
Nanotechnology	Nanotechnology, 1, 0.75% Nanotechnology 1 publication, 0.75%
Chemical Physics Letters	Chemical Physics Letters, 1, 0.75% Chemical Physics Letters 1 publication, 0.75%
Optik	Optik, 1, 0.75% Optik 1 publication, 0.75%
	5 10 15 20 25

Citations by publishers

	10 20 30 40 50 60
American Chemical Society (ACS)	American Chemical Society (ACS), 57, 42.86% American Chemical Society (ACS) 57 publications, 42.86%
American Physical Society (APS)	American Physical Society (APS), 26, 19.55% American Physical Society (APS) 26 publications, 19.55%
Elsevier	Elsevier, 11, 8.27% Elsevier 11 publications, 8.27%
Springer Nature	Springer Nature, 7, 5.26% Springer Nature 7 publications, 5.26%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 7, 5.26% Royal Society of Chemistry (RSC) 7 publications, 5.26%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 4, 3.01% American Institute of Physics (AIP) 4 publications, 3.01%
Wiley	Wiley, 4, 3.01% Wiley 4 publications, 3.01%
Optical Society of America	Optical Society of America, 4, 3.01% Optical Society of America 4 publications, 3.01%
Pleiades Publishing	Pleiades Publishing, 3, 2.26% Pleiades Publishing 3 publications, 2.26%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 1.5% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 1.5%
IOP Publishing	IOP Publishing, 2, 1.5% IOP Publishing 2 publications, 1.5%
EDP Sciences	EDP Sciences, 1, 0.75% EDP Sciences 1 publication, 0.75%
Uspekhi Fizicheskikh Nauk Journal	Uspekhi Fizicheskikh Nauk Journal, 1, 0.75% Uspekhi Fizicheskikh Nauk Journal 1 publication, 0.75%
Walter de Gruyter	Walter de Gruyter, 1, 0.75% Walter de Gruyter 1 publication, 0.75%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.75% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.75%
	10 20 30 40 50 60

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Harbold J. M. et al. Time-resolved intraband relaxation of strongly confined electrons and holes in colloidal PbSe nanocrystals // Physical Review B. 2005. Vol. 72. No. 19. 195312

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Harbold J. M., Du H., Du H., Krauss T. D., Krauss T., Cho K., Murray C. B., Murray C., Wise F. W., Frank Wise F. W. Time-resolved intraband relaxation of strongly confined electrons and holes in colloidal PbSe nanocrystals // Physical Review B. 2005. Vol. 72. No. 19. 195312

RIS |

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RIS Copy

TY - JOUR

DO - 10.1103/physrevb.72.195312

UR - https://doi.org/10.1103/physrevb.72.195312

TI - Time-resolved intraband relaxation of strongly confined electrons and holes in colloidal PbSe nanocrystals

T2 - Physical Review B

AU - Harbold, Jeffrey M.

AU - Du, Hui

AU - Krauss, Todd D

AU - Cho, Kyung-Sang

AU - Murray, Chris B

AU - Wise, Frank W

AU - Du, Hui

AU - Krauss, Todd

AU - Murray, Chris

AU - Frank Wise, Frank Wise

PY - 2005

DA - 2005/11/08 00:00:00

PB - American Physical Society (APS)

IS - 19

VL - 72

SN - 2469-9950

SN - 2469-9969

SN - 1098-0121

SN - 1550-235X

ER -

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@article{2005_Harbold,

author = {Jeffrey M. Harbold and Hui Du and Todd D Krauss and Kyung-Sang Cho and Chris B Murray and Frank W Wise and Hui Du and Todd Krauss and Chris Murray and Frank Wise Frank Wise},

title = {Time-resolved intraband relaxation of strongly confined electrons and holes in colloidal PbSe nanocrystals},

journal = {Physical Review B},

year = {2005},

volume = {72},

publisher = {American Physical Society (APS)},

month = {nov},

url = {https://doi.org/10.1103/physrevb.72.195312},

number = {19},

doi = {10.1103/physrevb.72.195312}

}

Found error?

Publisher

American Physical Society (APS)

Journal

Physical Review B

Quartile SCImago

Quartile WOS

Impact factor

3.7

ISSN

24699950 (Print)
24699969 (Electronic)
10980121 (Print)
1550235X (Electronic)