Open Access

Physical Review Letters, volume 106, issue 18, publication number 187401

Near-Unity Quantum Yields of Biexciton Emission fromCdSe/CdSNanocrystals Measured Using Single-Particle Spectroscopy

Y.-S. Park ^{1, 2}

A V Malko ³

A. Malko ³

J. Vela ^{1, 2}

J Vela ^{1, 2}

Y. Chen ^{1, 2}

Y. Ghosh ^{1, 2}

F. García-Santamaría ²

J.A. Hollingsworth ^{1, 2}

Jennifer A. Hollingsworth ^{1, 2}

Victor I. Klimov ^{2, 4}

V. I. KLIMOV ^{2, 4}

H. HTOON ^{1, 2}

Han Htoon ^{1, 2}

Hide authors affiliations Show authors affiliations: 4 affiliations

Center for integrated Nanotechnologies, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA |

Chemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA |

Department of Physics, The University of Texas at Dallas, Richardson, Texas 75080, USA |

⁴

Center for Advanced Solar Photophysics, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA |

Publication type: Journal Article

Publication date: 2011-05-03

American Physical Society (APS)

Journal: Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor: 8.6

ISSN: 00319007, 10797114

DOI: 10.1103/PhysRevLett.106.187401

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General Physics and Astronomy

Abstract

Biexciton photoluminescence (PL) quantum yields (Q(2X)) of individual CdSe/CdS core-shell nanocrystal quantum dots with various shell thicknesses are derived from independent PL saturation and two-photon correlation measurements. We observe a near-unity Q(2X) for some nanocrystals with an ultrathick 19-monolayer shell. High Q(2X)'s are, however, not universal and vary widely among nominally identical nanocrystals indicating a significant dependence of Q(2X) upon subtle structural differences. Interestingly, our measurements indicate that high Q(2X)'s are not required to achieve complete suppression of PL intensity fluctuations in individual nanocrystals.

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Nature	Nature, 2, 1.05% Nature 2 publications, 1.05%
Small	Small, 2, 1.05% Small 2 publications, 1.05%
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Citations by publishers

	10 20 30 40 50 60 70 80 90 100
American Chemical Society (ACS)	American Chemical Society (ACS), 91, 47.89% American Chemical Society (ACS) 91 publications, 47.89%
Springer Nature	Springer Nature, 20, 10.53% Springer Nature 20 publications, 10.53%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 20, 10.53% Royal Society of Chemistry (RSC) 20 publications, 10.53%
Wiley	Wiley, 13, 6.84% Wiley 13 publications, 6.84%
American Physical Society (APS)	American Physical Society (APS), 12, 6.32% American Physical Society (APS) 12 publications, 6.32%
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Elsevier	Elsevier, 6, 3.16% Elsevier 6 publications, 3.16%
Optical Society of America	Optical Society of America, 5, 2.63% Optical Society of America 5 publications, 2.63%
Pleiades Publishing	Pleiades Publishing, 2, 1.05% Pleiades Publishing 2 publications, 1.05%
SPIE	SPIE, 2, 1.05% SPIE 2 publications, 1.05%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 0.53% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 0.53%
Cambridge University Press	Cambridge University Press, 1, 0.53% Cambridge University Press 1 publication, 0.53%
IOP Publishing	IOP Publishing, 1, 0.53% IOP Publishing 1 publication, 0.53%
Taylor & Francis	Taylor & Francis, 1, 0.53% Taylor & Francis 1 publication, 0.53%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.53% American Association for the Advancement of Science (AAAS) 1 publication, 0.53%
Annual Reviews	Annual Reviews, 1, 0.53% Annual Reviews 1 publication, 0.53%
IEEE	IEEE, 1, 0.53% IEEE 1 publication, 0.53%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.53% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.53%
	10 20 30 40 50 60 70 80 90 100

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Park Y. et al. Near-Unity Quantum Yields of Biexciton Emission fromCdSe/CdSNanocrystals Measured Using Single-Particle Spectroscopy // Physical Review Letters. 2011. Vol. 106. No. 18. 187401

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Park Y., Malko A. V., Malko A., Vela J., Vela J., Chen Y., Ghosh Y., García-Santamaría F., Hollingsworth J., Hollingsworth J. A., KLIMOV V. I., Klimov V. I., HTOON H., Htoon H. Near-Unity Quantum Yields of Biexciton Emission fromCdSe/CdSNanocrystals Measured Using Single-Particle Spectroscopy // Physical Review Letters. 2011. Vol. 106. No. 18. 187401

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TY - JOUR

DO - 10.1103/PhysRevLett.106.187401

UR - https://doi.org/10.1103/PhysRevLett.106.187401

TI - Near-Unity Quantum Yields of Biexciton Emission fromCdSe/CdSNanocrystals Measured Using Single-Particle Spectroscopy

T2 - Physical Review Letters

AU - Park, Y.-S.

AU - Malko, A V

AU - Vela, J.

AU - Chen, Y.

AU - Ghosh, Y.

AU - García-Santamaría, F.

AU - Hollingsworth, J.A.

AU - KLIMOV, V. I.

AU - HTOON, H.

AU - Malko, A.

AU - Vela, J

AU - Hollingsworth, Jennifer A.

AU - Klimov, Victor I.

AU - Htoon, Han

PY - 2011

DA - 2011/05/03 00:00:00

PB - American Physical Society (APS)

IS - 18

VL - 106

SN - 0031-9007

SN - 1079-7114

ER -

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@article{2011_Park,

author = {Y.-S. Park and A V Malko and J. Vela and Y. Chen and Y. Ghosh and F. García-Santamaría and J.A. Hollingsworth and V. I. KLIMOV and H. HTOON and A. Malko and J Vela and Jennifer A. Hollingsworth and Victor I. Klimov and Han Htoon},

title = {Near-Unity Quantum Yields of Biexciton Emission fromCdSe/CdSNanocrystals Measured Using Single-Particle Spectroscopy},

journal = {Physical Review Letters},

year = {2011},

volume = {106},

publisher = {American Physical Society (APS)},

month = {may},

url = {https://doi.org/10.1103/PhysRevLett.106.187401},

number = {18},

doi = {10.1103/PhysRevLett.106.187401}

}

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Publisher

American Physical Society (APS)

Journal

Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor

8.6

ISSN

00319007 (Print)
10797114 (Electronic)