Open Access

Physical Review Letters, volume 85, issue 15, pages 3301-3304

Correlation between Fluorescence Intermittency and Spectral Diffusion in Single Semiconductor Quantum Dots

R. G. Neuhauser ¹

K T Shimizu ¹

W. K. Woo ¹

S. A. Empedocles ¹

Moungi G. Bawendi ¹

M G Bawendi ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139 |

Publication type: Journal Article

Publication date: 2000-10-09

American Physical Society (APS)

Journal: Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor: 8.6

ISSN: 00319007, 10797114

DOI: 10.1103/PhysRevLett.85.3301

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General Physics and Astronomy

Abstract

We find a correlation between the dynamics of fluorescence intermittency and spectral diffusion in the spectroscopy of single CdSe nanocrystal quantum dots (QD). A statistical analysis of the data suggests two populations of blinking events: blinking followed by large spectral diffusion shifts and blinking with small or no spectral shifts. Although unexpected from earlier studies, the correlation between blinking and spectral shifting is consistent with a model of QD ionization as the mechanism for the blinking event, followed by a redistribution of local electric fields that results in spectral shifting.

By date By citations

Top-30

Citations by journals

	5 10 15 20 25 30
Physical Review B	Physical Review B, 30, 8.82% Physical Review B 30 publications, 8.82%
Nano Letters	Nano Letters, 22, 6.47% Nano Letters 22 publications, 6.47%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 22, 6.47% Journal of Physical Chemistry C 22 publications, 6.47%
Journal of Physical Chemistry B	Journal of Physical Chemistry B, 17, 5% Journal of Physical Chemistry B 17 publications, 5%
Physical Review Letters	Physical Review Letters, 13, 3.82% Physical Review Letters 13 publications, 3.82%
Applied Physics Letters	Applied Physics Letters, 11, 3.24% Applied Physics Letters 11 publications, 3.24%
ACS Nano	ACS Nano, 10, 2.94% ACS Nano 10 publications, 2.94%
Journal of Chemical Physics	Journal of Chemical Physics, 7, 2.06% Journal of Chemical Physics 7 publications, 2.06%
ChemPhysChem	ChemPhysChem, 7, 2.06% ChemPhysChem 7 publications, 2.06%
Advanced Materials	Advanced Materials, 7, 2.06% Advanced Materials 7 publications, 2.06%
Journal of Luminescence	Journal of Luminescence, 6, 1.76% Journal of Luminescence 6 publications, 1.76%
Chemical Physics Letters	Chemical Physics Letters, 5, 1.47% Chemical Physics Letters 5 publications, 1.47%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 5, 1.47% Physical Chemistry Chemical Physics 5 publications, 1.47%
Physical Review E	Physical Review E, 4, 1.18% Physical Review E 4 publications, 1.18%
Nanotechnology	Nanotechnology, 4, 1.18% Nanotechnology 4 publications, 1.18%
Small	Small, 4, 1.18% Small 4 publications, 1.18%
Journal of the American Chemical Society	Journal of the American Chemical Society, 4, 1.18% Journal of the American Chemical Society 4 publications, 1.18%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 4, 1.18% Journal of Physical Chemistry Letters 4 publications, 1.18%
Nanoscale	Nanoscale, 4, 1.18% Nanoscale 4 publications, 1.18%
Proceedings of SPIE - The International Society for Optical Engineering	Proceedings of SPIE - The International Society for Optical Engineering, 4, 1.18% Proceedings of SPIE - The International Society for Optical Engineering 4 publications, 1.18%
Journal of Applied Physics	Journal of Applied Physics, 3, 0.88% Journal of Applied Physics 3 publications, 0.88%
Superlattices and Microstructures	Superlattices and Microstructures, 3, 0.88% Superlattices and Microstructures 3 publications, 0.88%
Chemical Physics	Chemical Physics, 3, 0.88% Chemical Physics 3 publications, 0.88%
Physica Status Solidi (B): Basic Research	Physica Status Solidi (B): Basic Research, 3, 0.88% Physica Status Solidi (B): Basic Research 3 publications, 0.88%
ACS Photonics	ACS Photonics, 3, 0.88% ACS Photonics 3 publications, 0.88%
Chemical Society Reviews	Chemical Society Reviews, 3, 0.88% Chemical Society Reviews 3 publications, 0.88%
Science	Science, 3, 0.88% Science 3 publications, 0.88%
Semiconductor Science and Technology	Semiconductor Science and Technology, 2, 0.59% Semiconductor Science and Technology 2 publications, 0.59%
Physical Review A	Physical Review A, 2, 0.59% Physical Review A 2 publications, 0.59%
	5 10 15 20 25 30

Citations by publishers

	10 20 30 40 50 60 70 80 90 100
American Chemical Society (ACS)	American Chemical Society (ACS), 91, 26.76% American Chemical Society (ACS) 91 publications, 26.76%
American Physical Society (APS)	American Physical Society (APS), 49, 14.41% American Physical Society (APS) 49 publications, 14.41%
Wiley	Wiley, 36, 10.59% Wiley 36 publications, 10.59%
Elsevier	Elsevier, 34, 10% Elsevier 34 publications, 10%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 23, 6.76% American Institute of Physics (AIP) 23 publications, 6.76%
Springer Nature	Springer Nature, 21, 6.18% Springer Nature 21 publications, 6.18%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 14, 4.12% Royal Society of Chemistry (RSC) 14 publications, 4.12%
IOP Publishing	IOP Publishing, 12, 3.53% IOP Publishing 12 publications, 3.53%
SPIE	SPIE, 6, 1.76% SPIE 6 publications, 1.76%
Optical Society of America	Optical Society of America, 5, 1.47% Optical Society of America 5 publications, 1.47%
Walter de Gruyter	Walter de Gruyter, 3, 0.88% Walter de Gruyter 3 publications, 0.88%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 3, 0.88% American Association for the Advancement of Science (AAAS) 3 publications, 0.88%
Annual Reviews	Annual Reviews, 3, 0.88% Annual Reviews 3 publications, 0.88%
Japan Society of Applied Physics	Japan Society of Applied Physics, 2, 0.59% Japan Society of Applied Physics 2 publications, 0.59%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 2, 0.59% Proceedings of the National Academy of Sciences (PNAS) 2 publications, 0.59%
Beilstein-Institut	Beilstein-Institut, 1, 0.29% Beilstein-Institut 1 publication, 0.29%
The Royal Society	The Royal Society, 1, 0.29% The Royal Society 1 publication, 0.29%
Uspekhi Fizicheskikh Nauk Journal	Uspekhi Fizicheskikh Nauk Journal, 1, 0.29% Uspekhi Fizicheskikh Nauk Journal 1 publication, 0.29%
Physical Society of Japan	Physical Society of Japan, 1, 0.29% Physical Society of Japan 1 publication, 0.29%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.29% Frontiers Media S.A. 1 publication, 0.29%
Materials Research Society	Materials Research Society, 1, 0.29% Materials Research Society 1 publication, 0.29%
Pleiades Publishing	Pleiades Publishing, 1, 0.29% Pleiades Publishing 1 publication, 0.29%
Taylor & Francis	Taylor & Francis, 1, 0.29% Taylor & Francis 1 publication, 0.29%
Verein zur Forderung des Open Access Publizierens in den Quantenwissenschaften	Verein zur Forderung des Open Access Publizierens in den Quantenwissenschaften, 1, 0.29% Verein zur Forderung des Open Access Publizierens in den Quantenwissenschaften 1 publication, 0.29%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.29% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.29%
	10 20 30 40 50 60 70 80 90 100

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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GOST |

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GOST Copy

Neuhauser R. G. et al. Correlation between Fluorescence Intermittency and Spectral Diffusion in Single Semiconductor Quantum Dots // Physical Review Letters. 2000. Vol. 85. No. 15. pp. 3301-3304.

GOST all authors (up to 50) Copy

Neuhauser R. G., Shimizu K. T., Woo W. K., Empedocles S. A., Bawendi M. G., Bawendi M. G. Correlation between Fluorescence Intermittency and Spectral Diffusion in Single Semiconductor Quantum Dots // Physical Review Letters. 2000. Vol. 85. No. 15. pp. 3301-3304.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1103/PhysRevLett.85.3301

UR - https://doi.org/10.1103/PhysRevLett.85.3301

TI - Correlation between Fluorescence Intermittency and Spectral Diffusion in Single Semiconductor Quantum Dots

T2 - Physical Review Letters

AU - Neuhauser, R. G.

AU - Shimizu, K T

AU - Empedocles, S. A.

AU - Bawendi, M G

AU - Woo, W. K.

AU - Bawendi, Moungi G.

PY - 2000

DA - 2000/10/09 00:00:00

PB - American Physical Society (APS)

SP - 3301-3304

IS - 15

VL - 85

SN - 0031-9007

SN - 1079-7114

ER -

BibTex |

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BibTex Copy

@article{2000_Neuhauser,

author = {R. G. Neuhauser and K T Shimizu and S. A. Empedocles and M G Bawendi and W. K. Woo and Moungi G. Bawendi},

title = {Correlation between Fluorescence Intermittency and Spectral Diffusion in Single Semiconductor Quantum Dots},

journal = {Physical Review Letters},

year = {2000},

volume = {85},

publisher = {American Physical Society (APS)},

month = {oct},

url = {https://doi.org/10.1103/PhysRevLett.85.3301},

number = {15},

pages = {3301--3304},

doi = {10.1103/PhysRevLett.85.3301}

}

MLA

Cite this

MLA Copy

Neuhauser, R. G., et al. “Correlation between Fluorescence Intermittency and Spectral Diffusion in Single Semiconductor Quantum Dots.” Physical Review Letters, vol. 85, no. 15, Oct. 2000, pp. 3301-3304. https://doi.org/10.1103/PhysRevLett.85.3301.

Found error?

Publisher

American Physical Society (APS)

Journal

Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor

8.6

ISSN

00319007 (Print)
10797114 (Electronic)

Profiles

Bawendi, Moungi G