Open Access

Physical Review Letters, volume 93, issue 18, publication number 187402

Structure of Excited-State Transitions of Individual Semiconductor Nanocrystals Probed by Photoluminescence Excitation Spectroscopy

Han Htoon ¹

Paris J. Cox ¹

Victor I. Klimov ¹

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Chemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA |

Publication type: Journal Article

Publication date: 2004-10-28

American Physical Society (APS)

Journal: Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor: 8.6

ISSN: 00319007, 10797114

DOI: 10.1103/physrevlett.93.187402

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General Physics and Astronomy

Abstract

We perform for the first time photoluminescence excitation (PLE) studies of individual nanocrystals (NCs) that reveal the structure of excited-state transitions not obscured by ensemble averaging. Single-NC PLE spectra strongly deviate from a traditional idealized picture of sharp, quasiatomic resonances. We detect only a few relatively narrow transitions (3-4 meV) at the band edge, while at higher spectral energies, we observe a broad structureless feature separated from the band-edge peaks by a >50 meV "minigap." These observations can be rationalized by analyzing hole intraband relaxation behavior.

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Citations by journals

	1 2 3 4 5 6 7
Physical Review B	Physical Review B, 7, 15.91% Physical Review B 7 publications, 15.91%
Nano Letters	Nano Letters, 4, 9.09% Nano Letters 4 publications, 9.09%
Physical Review Letters	Physical Review Letters, 3, 6.82% Physical Review Letters 3 publications, 6.82%
Journal of Chemical Physics	Journal of Chemical Physics, 2, 4.55% Journal of Chemical Physics 2 publications, 4.55%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 2, 4.55% Journal of Physical Chemistry Letters 2 publications, 4.55%
Beilstein Journal of Nanotechnology	Beilstein Journal of Nanotechnology, 1, 2.27% Beilstein Journal of Nanotechnology 1 publication, 2.27%
Applied Physics Letters	Applied Physics Letters, 1, 2.27% Applied Physics Letters 1 publication, 2.27%
Nanomaterials	Nanomaterials, 1, 2.27% Nanomaterials 1 publication, 2.27%
Nature Physics	Nature Physics, 1, 2.27% Nature Physics 1 publication, 2.27%
Light: Science and Applications	Light: Science and Applications, 1, 2.27% Light: Science and Applications 1 publication, 2.27%
Journal of Luminescence	Journal of Luminescence, 1, 2.27% Journal of Luminescence 1 publication, 2.27%
ACS Photonics	ACS Photonics, 1, 2.27% ACS Photonics 1 publication, 2.27%
Nachrichten aus der Chemie	Nachrichten aus der Chemie, 1, 2.27% Nachrichten aus der Chemie 1 publication, 2.27%
Journal of Physical Chemistry B	Journal of Physical Chemistry B, 1, 2.27% Journal of Physical Chemistry B 1 publication, 2.27%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 1, 2.27% Journal of Physical Chemistry C 1 publication, 2.27%
ACS Nano	ACS Nano, 1, 2.27% ACS Nano 1 publication, 2.27%
Chemical Reviews	Chemical Reviews, 1, 2.27% Chemical Reviews 1 publication, 2.27%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 1, 2.27% Physical Chemistry Chemical Physics 1 publication, 2.27%
Chemical Society Reviews	Chemical Society Reviews, 1, 2.27% Chemical Society Reviews 1 publication, 2.27%
Laser Physics	Laser Physics, 1, 2.27% Laser Physics 1 publication, 2.27%
Springer Series in Optical Sciences	Springer Series in Optical Sciences, 1, 2.27% Springer Series in Optical Sciences 1 publication, 2.27%
Journal of Biological Education	Journal of Biological Education, 1, 2.27% Journal of Biological Education 1 publication, 2.27%
Topics in Applied Physics	Topics in Applied Physics, 1, 2.27% Topics in Applied Physics 1 publication, 2.27%
Science	Science, 1, 2.27% Science 1 publication, 2.27%
Annual Review of Physical Chemistry	Annual Review of Physical Chemistry, 1, 2.27% Annual Review of Physical Chemistry 1 publication, 2.27%
Russian Chemical Reviews	Russian Chemical Reviews, 1, 2.27% Russian Chemical Reviews 1 publication, 2.27%
	1 2 3 4 5 6 7

Citations by publishers

	2 4 6 8 10 12
American Chemical Society (ACS)	American Chemical Society (ACS), 11, 25% American Chemical Society (ACS) 11 publications, 25%
American Physical Society (APS)	American Physical Society (APS), 10, 22.73% American Physical Society (APS) 10 publications, 22.73%
Springer Nature	Springer Nature, 4, 9.09% Springer Nature 4 publications, 9.09%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 3, 6.82% American Institute of Physics (AIP) 3 publications, 6.82%
Elsevier	Elsevier, 2, 4.55% Elsevier 2 publications, 4.55%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 2, 4.55% Royal Society of Chemistry (RSC) 2 publications, 4.55%
Beilstein-Institut	Beilstein-Institut, 1, 2.27% Beilstein-Institut 1 publication, 2.27%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 1, 2.27% Multidisciplinary Digital Publishing Institute (MDPI) 1 publication, 2.27%
Wiley	Wiley, 1, 2.27% Wiley 1 publication, 2.27%
IOP Publishing	IOP Publishing, 1, 2.27% IOP Publishing 1 publication, 2.27%
Taylor & Francis	Taylor & Francis, 1, 2.27% Taylor & Francis 1 publication, 2.27%
Cambridge University Press	Cambridge University Press, 1, 2.27% Cambridge University Press 1 publication, 2.27%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 2.27% American Association for the Advancement of Science (AAAS) 1 publication, 2.27%
Annual Reviews	Annual Reviews, 1, 2.27% Annual Reviews 1 publication, 2.27%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 2.27% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 2.27%
	2 4 6 8 10 12

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Htoon H., Cox P. J., Klimov V. I. Structure of Excited-State Transitions of Individual Semiconductor Nanocrystals Probed by Photoluminescence Excitation Spectroscopy // Physical Review Letters. 2004. Vol. 93. No. 18. 187402

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TY - JOUR

DO - 10.1103/physrevlett.93.187402

UR - https://doi.org/10.1103/physrevlett.93.187402

TI - Structure of Excited-State Transitions of Individual Semiconductor Nanocrystals Probed by Photoluminescence Excitation Spectroscopy

T2 - Physical Review Letters

AU - Htoon, Han

AU - Cox, Paris J.

AU - Klimov, Victor I.

PY - 2004

DA - 2004/10/28 00:00:00

PB - American Physical Society (APS)

IS - 18

VL - 93

SN - 0031-9007

SN - 1079-7114

ER -

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@article{2004_Htoon,

author = {Han Htoon and Paris J. Cox and Victor I. Klimov},

title = {Structure of Excited-State Transitions of Individual Semiconductor Nanocrystals Probed by Photoluminescence Excitation Spectroscopy},

journal = {Physical Review Letters},

year = {2004},

volume = {93},

publisher = {American Physical Society (APS)},

month = {oct},

url = {https://doi.org/10.1103/physrevlett.93.187402},

number = {18},

doi = {10.1103/physrevlett.93.187402}

}

Found error?

Publisher

American Physical Society (APS)

Journal

Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor

8.6

ISSN

00319007 (Print)
10797114 (Electronic)