International Union of Crystallography (IUCr)

Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials

, том 72 , издание 5 , страницы 716-722

CH3NH3PbI3: precise structural consequences of water absorption at ambient conditions.

Alla Arakcheeva ¹

D. O. Chernyshov ²

Massimo Spina ¹

László Forró ¹

Endre Horvath ¹

Endre Horváth ¹

Скрыть аффилиации авторов Показать аффилиации авторов: 2 аффилиации

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland |

SNBL, ESRF, 71 Avenue des Martyrs, 38043 Grenoble CEDEX 9, France |

Тип публикации: Journal Article

Дата публикации: 2016-09-16

International Union of Crystallography (IUCr)

Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials

scimago Q2

wos Q3

БС1

SJR: 0.300

CiteScore: 2.8

Impact factor: 1.3

ISSN: 20525192, 20525206

DOI: 10.1107/S2052520616010428

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PubMed ID: 27698312

Materials Chemistry

Metals and Alloys

Electronic, Optical and Magnetic Materials

Atomic and Molecular Physics, and Optics

Краткое описание

The crystal structure of the pristine (I) and aged (II) crystals of CH₃NH₃PbI₃(hereafter MAPbI₃) hybrid organic–inorganic lead iodide has been studied at 293 K with high-precision single-crystal X-ray diffraction using a synchrotron light source. We show that (I) and (II) are characterized by an identical tetragonal unit cell but different space groups:I422 for (I) andP4₂2₁2 for (II). Both space groups are subgroups ofI4/mcm, which is widely used for MAPbI₃. The main difference between (I) and (II) comes from the difference in hydrogen bonds between the MA⁺cation and the PbI₃framework which is the direct consequence of H₂O insertion in the aged crystal (II).

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Arakcheeva A. et al. CH3NH3PbI3: precise structural consequences of water absorption at ambient conditions. // Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials. 2016. Vol. 72. No. 5. pp. 716-722.

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Arakcheeva A., Chernyshov D. O., Spina M., Forró L., Horvath E., Horváth E. CH3NH3PbI3: precise structural consequences of water absorption at ambient conditions. // Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials. 2016. Vol. 72. No. 5. pp. 716-722.

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TY - JOUR

DO - 10.1107/S2052520616010428

UR - https://doi.org/10.1107/S2052520616010428

TI - CH3NH3PbI3: precise structural consequences of water absorption at ambient conditions.

T2 - Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials

AU - Arakcheeva, Alla

AU - Chernyshov, D. O.

AU - Spina, Massimo

AU - Forró, László

AU - Horvath, Endre

AU - Horváth, Endre

PY - 2016

DA - 2016/09/16

PB - International Union of Crystallography (IUCr)

SP - 716-722

IS - 5

VL - 72

PMID - 27698312

SN - 2052-5192

SN - 2052-5206

ER -

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@article{2016_Arakcheeva,

author = {Alla Arakcheeva and D. O. Chernyshov and Massimo Spina and László Forró and Endre Horvath and Endre Horváth},

title = {CH3NH3PbI3: precise structural consequences of water absorption at ambient conditions.},

journal = {Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials},

year = {2016},

volume = {72},

publisher = {International Union of Crystallography (IUCr)},

month = {sep},

url = {https://doi.org/10.1107/S2052520616010428},

number = {5},

pages = {716--722},

doi = {10.1107/S2052520616010428}

}

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Arakcheeva, Alla, et al. “CH3NH3PbI3: precise structural consequences of water absorption at ambient conditions..” Acta Crystallographica Section B: Structural Science, Crystal Engineering and Materials, vol. 72, no. 5, Sep. 2016, pp. 716-722. https://doi.org/10.1107/S2052520616010428.