Journal of the American Ceramic Society, volume 86, issue 3, pages 437-440

Novel Fast Lithium Ion Conduction in Garnet‐Type Li5La3M2O12 (M = Nb, Ta)

Venkataraman Thangadurai ¹

Heiko Kaack ¹

Werner J.F. Weppner ¹

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Chair for Sensors and Solid State Ionics, Faculty of Engineering, University of Kiel, Kaiserstrasse 2, 24143 Kiel, Germany. |

Publication type: Journal Article

Publication date: 2003-03-01

Wiley

Journal: Journal of the American Ceramic Society

Quartile SCImago

Quartile WOS

Impact factor: 3.9

ISSN: 00027820, 15512916

DOI: 10.1111/j.1151-2916.2003.tb03318.x

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Materials Chemistry

Ceramics and Composites

Abstract

Lithium metal oxides with the nominal composition Li5La3M2O12 (M = Nb, Ta), possessing a garnetlike structure, have been investigated with regard to their electrical properties. These compounds form a new class of solid-state lithium ion conductors with a different crystal structure compared with all those known so far. The materials are prepared by solid-state reaction and characterized by powder XRD and ac impedance to determine their lithium ionic conductivity. Both the niobium and tantalum members exhibit the same order of magnitude of bulk conductivity (∼10−6 S/cm at 25°C). The activation energies for ionic conductivity (<300°C) are 0.43 and 0.56 eV for Li5La3Nb2O12 and Li5La3Ta2O12, respectively, which are comparable to those of other solid lithium conductors, such as Lisicon, Li14ZnGe4O16. Among the investigated materials, the tantalum compound Li5La3Ta2O12 is stable against reaction with molten lithium. Further tailoring of the compositions by appropriate chemical substitutions and improved synthesizing methods, especially with regard to minimizing grain-boundary resistance, are important issues in view of the potential use of the new class of compounds as electrolytes in practical lithium ion batteries.

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	5 10 15 20 25 30 35 40

Citations by publishers

	50 100 150 200 250
Elsevier	Elsevier, 209, 31.57% Elsevier 209 publications, 31.57%
American Chemical Society (ACS)	American Chemical Society (ACS), 95, 14.35% American Chemical Society (ACS) 95 publications, 14.35%
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Canadian Science Publishing	Canadian Science Publishing, 2, 0.3% Canadian Science Publishing 2 publications, 0.3%
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Materials Research Society	Materials Research Society, 2, 0.3% Materials Research Society 2 publications, 0.3%
Chinese Ceramic Society	Chinese Ceramic Society, 2, 0.3% Chinese Ceramic Society 2 publications, 0.3%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 2, 0.3% American Association for the Advancement of Science (AAAS) 2 publications, 0.3%
Walter de Gruyter	Walter de Gruyter, 2, 0.3% Walter de Gruyter 2 publications, 0.3%
Trans Tech Publications	Trans Tech Publications, 2, 0.3% Trans Tech Publications 2 publications, 0.3%
Annual Reviews	Annual Reviews, 2, 0.3% Annual Reviews 2 publications, 0.3%
ASME	ASME, 1, 0.15% ASME 1 publication, 0.15%
Bentham Science	Bentham Science, 1, 0.15% Bentham Science 1 publication, 0.15%
The Royal Society	The Royal Society, 1, 0.15% The Royal Society 1 publication, 0.15%
Japan Institute of Metals and Materials	Japan Institute of Metals and Materials, 1, 0.15% Japan Institute of Metals and Materials 1 publication, 0.15%
	50 100 150 200 250

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Thangadurai V., Kaack H., Weppner W. J. Novel Fast Lithium Ion Conduction in Garnet‐Type Li5La3M2O12 (M = Nb, Ta) // Journal of the American Ceramic Society. 2003. Vol. 86. No. 3. pp. 437-440.

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Thangadurai V., Kaack H., Weppner W. J. Novel Fast Lithium Ion Conduction in Garnet‐Type Li5La3M2O12 (M = Nb, Ta) // Journal of the American Ceramic Society. 2003. Vol. 86. No. 3. pp. 437-440.

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RIS Copy

TY - JOUR

DO - 10.1111/j.1151-2916.2003.tb03318.x

UR - https://doi.org/10.1111/j.1151-2916.2003.tb03318.x

TI - Novel Fast Lithium Ion Conduction in Garnet‐Type Li5La3M2O12 (M = Nb, Ta)

T2 - Journal of the American Ceramic Society

AU - Thangadurai, Venkataraman

AU - Kaack, Heiko

AU - Weppner, Werner J.F.

PY - 2003

DA - 2003/03/01 00:00:00

PB - Wiley

SP - 437-440

IS - 3

VL - 86

SN - 0002-7820

SN - 1551-2916

ER -

BibTex |

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BibTex Copy

@article{2003_Thangadurai,

author = {Venkataraman Thangadurai and Heiko Kaack and Werner J.F. Weppner},

title = {Novel Fast Lithium Ion Conduction in Garnet‐Type Li5La3M2O12 (M = Nb, Ta)},

journal = {Journal of the American Ceramic Society},

year = {2003},

volume = {86},

publisher = {Wiley},

month = {mar},

url = {https://doi.org/10.1111/j.1151-2916.2003.tb03318.x},

number = {3},

pages = {437--440},

doi = {10.1111/j.1151-2916.2003.tb03318.x}

}

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MLA Copy

Thangadurai, Venkataraman, et al. “Novel Fast Lithium Ion Conduction in Garnet‐Type Li5La3M2O12 (M = Nb, Ta).” Journal of the American Ceramic Society, vol. 86, no. 3, Mar. 2003, pp. 437-440. https://doi.org/10.1111/j.1151-2916.2003.tb03318.x.

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Publisher

Wiley

Journal

Journal of the American Ceramic Society

Quartile SCImago

Quartile WOS

Impact factor

3.9

ISSN

00027820 (Print)
15512916 (Electronic)