Open Access
Science, volume 290, issue 5490, pages 314-317
Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots
V. I. KLIMOV
1
,
A A Mikhailovsky
1
,
Su Xu
1
,
A. Malko
1
,
J.A. Hollingsworth
1
,
C. A. Leatherdale
2
,
H.-J. Eisler
2
,
M G Bawendi
2
Publication type: Journal Article
Publication date: 2000-10-13
Multidisciplinary
Abstract
The development of optical gain in chemically synthesized semiconductor nanoparticles (nanocrystal quantum dots) has been intensely studied as the first step toward nanocrystal quantum dot lasers. We examined the competing dynamical processes involved in optical amplification and lasing in nanocrystal quantum dots and found that, despite a highly efficient intrinsic nonradiative Auger recombination, large optical gain can be developed at the wavelength of the emitting transition for close-packed solids of these dots. Narrowband stimulated emission with a pronounced gain threshold at wavelengths tunable with the size of the nanocrystal was observed, as expected from quantum confinement effects. These results unambiguously demonstrate the feasibility of nanocrystal quantum dot lasers.
Top-30
Citations by journals
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Journal of Physical Chemistry C
140 publications, 5.68%
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Nano Letters
127 publications, 5.16%
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Physical Review B
79 publications, 3.21%
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Applied Physics Letters
76 publications, 3.09%
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ACS Nano
71 publications, 2.88%
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Journal of the American Chemical Society
64 publications, 2.6%
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Chemistry of Materials
51 publications, 2.07%
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Advanced Materials
50 publications, 2.03%
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Journal of Physical Chemistry B
46 publications, 1.87%
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Nanoscale
43 publications, 1.75%
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Nanotechnology
38 publications, 1.54%
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Journal of Physical Chemistry Letters
37 publications, 1.5%
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Physical Review Letters
34 publications, 1.38%
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Journal of Luminescence
27 publications, 1.1%
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Physical Chemistry Chemical Physics
27 publications, 1.1%
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ACS Photonics
26 publications, 1.06%
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Advanced Optical Materials
26 publications, 1.06%
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Optics Express
26 publications, 1.06%
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Journal of Applied Physics
25 publications, 1.02%
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Journal of Materials Chemistry A
24 publications, 0.97%
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Journal of Chemical Physics
23 publications, 0.93%
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Advanced Functional Materials
23 publications, 0.93%
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Langmuir
21 publications, 0.85%
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Journal of Materials Chemistry C
21 publications, 0.85%
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Chemical Communications
19 publications, 0.77%
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Chemical Reviews
18 publications, 0.73%
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RSC Advances
18 publications, 0.73%
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Physica E: Low-Dimensional Systems and Nanostructures
17 publications, 0.69%
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ACS applied materials & interfaces
16 publications, 0.65%
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140
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Citations by publishers
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700
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American Chemical Society (ACS)
667 publications, 27.08%
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Elsevier
334 publications, 13.56%
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Wiley
272 publications, 11.04%
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Springer Nature
198 publications, 8.04%
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Royal Society of Chemistry (RSC)
194 publications, 7.88%
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American Institute of Physics (AIP)
136 publications, 5.52%
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American Physical Society (APS)
123 publications, 4.99%
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IOP Publishing
100 publications, 4.06%
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Optical Society of America
48 publications, 1.95%
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Taylor & Francis
30 publications, 1.22%
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Multidisciplinary Digital Publishing Institute (MDPI)
28 publications, 1.14%
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IEEE
22 publications, 0.89%
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Pleiades Publishing
20 publications, 0.81%
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SPIE
19 publications, 0.77%
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Materials Research Society
15 publications, 0.61%
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World Scientific
12 publications, 0.49%
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The Chemical Society of Japan
11 publications, 0.45%
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Walter de Gruyter
10 publications, 0.41%
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Cambridge University Press
9 publications, 0.37%
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Hindawi Limited
9 publications, 0.37%
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American Association for the Advancement of Science (AAAS)
8 publications, 0.32%
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Trans Tech Publications
8 publications, 0.32%
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Japan Society of Applied Physics
6 publications, 0.24%
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American Vacuum Society
5 publications, 0.2%
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Chinese Physical Society
5 publications, 0.2%
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Proceedings of the National Academy of Sciences (PNAS)
5 publications, 0.2%
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Annual Reviews
5 publications, 0.2%
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EDP Sciences
4 publications, 0.16%
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The Electrochemical Society
4 publications, 0.16%
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100
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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KLIMOV V. I. et al. Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots // Science. 2000. Vol. 290. No. 5490. pp. 314-317.
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KLIMOV V. I., Mikhailovsky A. A., Xu S., Malko A., Hollingsworth J., Leatherdale C. A., Eisler H., Bawendi M. G. Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots // Science. 2000. Vol. 290. No. 5490. pp. 314-317.
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TY - JOUR
DO - 10.1126/science.290.5490.314
UR - https://doi.org/10.1126/science.290.5490.314
TI - Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots
T2 - Science
AU - KLIMOV, V. I.
AU - Mikhailovsky, A A
AU - Xu, Su
AU - Malko, A.
AU - Hollingsworth, J.A.
AU - Leatherdale, C. A.
AU - Eisler, H.-J.
AU - Bawendi, M G
PY - 2000
DA - 2000/10/13 00:00:00
PB - American Association for the Advancement of Science (AAAS)
SP - 314-317
IS - 5490
VL - 290
SN - 0036-8075
SN - 1095-9203
ER -
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@article{2000_KLIMOV,
author = {V. I. KLIMOV and A A Mikhailovsky and Su Xu and A. Malko and J.A. Hollingsworth and C. A. Leatherdale and H.-J. Eisler and M G Bawendi},
title = {Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots},
journal = {Science},
year = {2000},
volume = {290},
publisher = {American Association for the Advancement of Science (AAAS)},
month = {oct},
url = {https://doi.org/10.1126/science.290.5490.314},
number = {5490},
pages = {314--317},
doi = {10.1126/science.290.5490.314}
}
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KLIMOV, V. I., et al. “Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots.” Science, vol. 290, no. 5490, Oct. 2000, pp. 314-317. https://doi.org/10.1126/science.290.5490.314.